Facet-dependent catalytic activities of Pd/rGO: Exploring dehydrogenation mechanism of dodecahydro-N-ethylcarbazole

[Display omitted] •Pd nanoparticles enclosed by {100}, {110} and {111} facets were successfully synthesized in-situ on rGO.•Facet effect in the dehydrogenation of LOHC was proposed for the first time.•Restriction mechanism of the macrokinetic and thermodynamic rate-determining step was preliminarily...

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Veröffentlicht in:	Applied catalysis. B, Environmental Environmental, 2020-06, Vol.266, p.118658, Article 118658
Hauptverfasser:	Wang, Bin, Chen, You-Tao, Chang, Tie-Yan, Jiang, Zhao, Huang, Zheng-Qing, Wang, Si-Yao, Chang, Chun-Ran, Chen, Yu-Sheng, Wei, Jin-Jia, Yang, Sen, Fang, Tao
Format:	Artikel
Sprache:	eng
Schlagworte:	Catalysts Dehydrogenation Dehydrogenation kinetics Dehydrogenation Mechanism Dodecahydro-N-ethylcarbazole Graphene Hydrogen bonds Liquid organic hydrogen carrier N-ethylcarbazole Nanoparticles Selectivity Shape-control synthesis
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