Formation of Nitrosodipropylamine from Nitrogenous Contaminants (Amines and Amine-Based Pesticides) in Water During Chloramination
Chloramination of drinking water and wastewater can generate carcinogenic nitrosamines, among which, nitrosodipropylamine (NDPA) with large molecular weight and weak polarity has been commonly found. However, knowledge on the formation of NDPA remains highly limited. Laboratory tests were conducted...
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| Veröffentlicht in: | Water, air, and soil pollution air, and soil pollution, 2020-04, Vol.231 (4), Article 141 |
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| creator | Zhou, Chao Bai, Jinchao He, Changxuan Wang, Hao Sun, Jianhai Yang, Yiqiong Gao, Naiyun Zhang, Xiaodong |
| description | Chloramination of drinking water and wastewater can generate carcinogenic nitrosamines, among which, nitrosodipropylamine (NDPA) with large molecular weight and weak polarity has been commonly found. However, knowledge on the formation of NDPA remains highly limited. Laboratory tests were conducted to quantify NDPA formation during chloramination of nitrogenous precursors, including dipropylamine and methyldipropylamine, and pesticides such as trifluralin, oryzalin, and vernolat. Results showed that all precursors exhibited > 10.0% NDPA yields after 24 h. Oryzalin and trifluralin accomplished the highest (13.63%) and lowest (11.31%) yield, respectively. Maximal yields of all precursors were observed at pH 9.0 and temperature 288 K. Maximums of NDPA yield from oryzalin (18.27%) and vernolat (19.54%) were formed at Cl:N of 0.7:1.0, but maximal yields of dipropylamine (18.44%), methyldipropylamine (22.98%), and trifluralin (33.06%) were achieved at Cl:N of 1.2:1.0. Maximal NDPA yields of dipropylamine (37.14%), methyldipropylamine (32.84%), and vernolat (49.02%) were observed at [NH
2
Cl]
0
:[precursor]
0
= 500, but highest yields of trifluralin (30.24%) and oryzalin (25.53%) were accomplished at [NH
2
Cl]
0
:[precursor]
0
= 50. Bromide and organic contents in tap and raw water reduced NDPA due to competition for NH
2
Cl. Chloramination of water impacted by amines and pesticides should be careful of NDPA formation. |
| doi_str_mv | 10.1007/s11270-020-04519-9 |
| format | Article |
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2
Cl]
0
:[precursor]
0
= 500, but highest yields of trifluralin (30.24%) and oryzalin (25.53%) were accomplished at [NH
2
Cl]
0
:[precursor]
0
= 50. Bromide and organic contents in tap and raw water reduced NDPA due to competition for NH
2
Cl. Chloramination of water impacted by amines and pesticides should be careful of NDPA formation.</description><identifier>ISSN: 0049-6979</identifier><identifier>EISSN: 1573-2932</identifier><identifier>DOI: 10.1007/s11270-020-04519-9</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Amines ; Atmospheric Protection/Air Quality Control/Air Pollution ; Carcinogens ; Climate Change/Climate Change Impacts ; Contaminants ; Doxylamine ; Drinking water ; Earth and Environmental Science ; Environment ; Environmental monitoring ; Hydrogeology ; Laboratory tests ; Molecular weight ; Nitrosamines ; Nitrosoamines ; Oryzalin ; Pesticides ; Polarity ; Precursors ; Raw water ; Soil Science & Conservation ; Tetracycline ; Tetracyclines ; Trifluralin ; Wastewater ; Water Quality/Water Pollution</subject><ispartof>Water, air, and soil pollution, 2020-04, Vol.231 (4), Article 141</ispartof><rights>Springer Nature Switzerland AG 2020</rights><rights>COPYRIGHT 2020 Springer</rights><rights>Water, Air, and Soil Pollution is a copyright of Springer, (2020). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c386t-e185779ead2754e62922e17ac8d361dcb374ff78cbdfc1b47abbfaeeca11eed53</citedby><cites>FETCH-LOGICAL-c386t-e185779ead2754e62922e17ac8d361dcb374ff78cbdfc1b47abbfaeeca11eed53</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11270-020-04519-9$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11270-020-04519-9$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Zhou, Chao</creatorcontrib><creatorcontrib>Bai, Jinchao</creatorcontrib><creatorcontrib>He, Changxuan</creatorcontrib><creatorcontrib>Wang, Hao</creatorcontrib><creatorcontrib>Sun, Jianhai</creatorcontrib><creatorcontrib>Yang, Yiqiong</creatorcontrib><creatorcontrib>Gao, Naiyun</creatorcontrib><creatorcontrib>Zhang, Xiaodong</creatorcontrib><title>Formation of Nitrosodipropylamine from Nitrogenous Contaminants (Amines and Amine-Based Pesticides) in Water During Chloramination</title><title>Water, air, and soil pollution</title><addtitle>Water Air Soil Pollut</addtitle><description>Chloramination of drinking water and wastewater can generate carcinogenic nitrosamines, among which, nitrosodipropylamine (NDPA) with large molecular weight and weak polarity has been commonly found. However, knowledge on the formation of NDPA remains highly limited. Laboratory tests were conducted to quantify NDPA formation during chloramination of nitrogenous precursors, including dipropylamine and methyldipropylamine, and pesticides such as trifluralin, oryzalin, and vernolat. Results showed that all precursors exhibited > 10.0% NDPA yields after 24 h. Oryzalin and trifluralin accomplished the highest (13.63%) and lowest (11.31%) yield, respectively. Maximal yields of all precursors were observed at pH 9.0 and temperature 288 K. Maximums of NDPA yield from oryzalin (18.27%) and vernolat (19.54%) were formed at Cl:N of 0.7:1.0, but maximal yields of dipropylamine (18.44%), methyldipropylamine (22.98%), and trifluralin (33.06%) were achieved at Cl:N of 1.2:1.0. Maximal NDPA yields of dipropylamine (37.14%), methyldipropylamine (32.84%), and vernolat (49.02%) were observed at [NH
2
Cl]
0
:[precursor]
0
= 500, but highest yields of trifluralin (30.24%) and oryzalin (25.53%) were accomplished at [NH
2
Cl]
0
:[precursor]
0
= 50. Bromide and organic contents in tap and raw water reduced NDPA due to competition for NH
2
Cl. 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Xiaodong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Formation of Nitrosodipropylamine from Nitrogenous Contaminants (Amines and Amine-Based Pesticides) in Water During Chloramination</atitle><jtitle>Water, air, and soil pollution</jtitle><stitle>Water Air Soil Pollut</stitle><date>2020-04-01</date><risdate>2020</risdate><volume>231</volume><issue>4</issue><artnum>141</artnum><issn>0049-6979</issn><eissn>1573-2932</eissn><abstract>Chloramination of drinking water and wastewater can generate carcinogenic nitrosamines, among which, nitrosodipropylamine (NDPA) with large molecular weight and weak polarity has been commonly found. However, knowledge on the formation of NDPA remains highly limited. Laboratory tests were conducted to quantify NDPA formation during chloramination of nitrogenous precursors, including dipropylamine and methyldipropylamine, and pesticides such as trifluralin, oryzalin, and vernolat. Results showed that all precursors exhibited > 10.0% NDPA yields after 24 h. Oryzalin and trifluralin accomplished the highest (13.63%) and lowest (11.31%) yield, respectively. Maximal yields of all precursors were observed at pH 9.0 and temperature 288 K. Maximums of NDPA yield from oryzalin (18.27%) and vernolat (19.54%) were formed at Cl:N of 0.7:1.0, but maximal yields of dipropylamine (18.44%), methyldipropylamine (22.98%), and trifluralin (33.06%) were achieved at Cl:N of 1.2:1.0. Maximal NDPA yields of dipropylamine (37.14%), methyldipropylamine (32.84%), and vernolat (49.02%) were observed at [NH
2
Cl]
0
:[precursor]
0
= 500, but highest yields of trifluralin (30.24%) and oryzalin (25.53%) were accomplished at [NH
2
Cl]
0
:[precursor]
0
= 50. Bromide and organic contents in tap and raw water reduced NDPA due to competition for NH
2
Cl. Chloramination of water impacted by amines and pesticides should be careful of NDPA formation.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s11270-020-04519-9</doi></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0049-6979 |
| ispartof | Water, air, and soil pollution, 2020-04, Vol.231 (4), Article 141 |
| issn | 0049-6979 1573-2932 |
| language | eng |
| recordid | cdi_proquest_journals_2378613231 |
| source | Springer Nature - Complete Springer Journals |
| subjects | Amines Atmospheric Protection/Air Quality Control/Air Pollution Carcinogens Climate Change/Climate Change Impacts Contaminants Doxylamine Drinking water Earth and Environmental Science Environment Environmental monitoring Hydrogeology Laboratory tests Molecular weight Nitrosamines Nitrosoamines Oryzalin Pesticides Polarity Precursors Raw water Soil Science & Conservation Tetracycline Tetracyclines Trifluralin Wastewater Water Quality/Water Pollution |
| title | Formation of Nitrosodipropylamine from Nitrogenous Contaminants (Amines and Amine-Based Pesticides) in Water During Chloramination |
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