Photocatalytic and electrocatalytic hydrogen production using nickel complexes supported by hemilabile and non-innocent ligands
Nickel complexes with non-innocent ligands generated by one-electron reduction of octahedral Schiff base nickel( ii ) complexes with hemilabile ligands exhibited excellent catalytic activities of over 5000 TONs through a metal-ligand cooperation mechanism for hydrogen evolution from water under visi...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2020-03, Vol.56 (19), p.2829-2832 |
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| container_title | Chemical communications (Cambridge, England) |
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| creator | Inoue, Satoshi Yan, Yin-Nan Yamanishi, Katsunori Kataoka, Yusuke Kawamoto, Tatsuya |
| description | Nickel complexes with non-innocent ligands generated by one-electron reduction of octahedral Schiff base nickel(
ii
) complexes with hemilabile ligands exhibited excellent catalytic activities of over 5000 TONs through a metal-ligand cooperation mechanism for hydrogen evolution from water under visible light irradiation.
Square-planar Ni complexes with non-innocent ligands generated by one-electron reduction of octahedral Ni(
ii
) complexes with Schiff base ligands exhibited excellent catalytic activities
via
proton-coupled electron transfer for the H
2
evolution reaction. |
| doi_str_mv | 10.1039/c9cc09568c |
| format | Article |
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ii
) complexes with hemilabile ligands exhibited excellent catalytic activities of over 5000 TONs through a metal-ligand cooperation mechanism for hydrogen evolution from water under visible light irradiation.
Square-planar Ni complexes with non-innocent ligands generated by one-electron reduction of octahedral Ni(
ii
) complexes with Schiff base ligands exhibited excellent catalytic activities
via
proton-coupled electron transfer for the H
2
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ii
) complexes with hemilabile ligands exhibited excellent catalytic activities of over 5000 TONs through a metal-ligand cooperation mechanism for hydrogen evolution from water under visible light irradiation.
Square-planar Ni complexes with non-innocent ligands generated by one-electron reduction of octahedral Ni(
ii
) complexes with Schiff base ligands exhibited excellent catalytic activities
via
proton-coupled electron transfer for the H
2
evolution reaction.</description><subject>Coordination compounds</subject><subject>Crystallography</subject><subject>Hydrogen evolution</subject><subject>Hydrogen production</subject><subject>Imines</subject><subject>Ligands</subject><subject>Light irradiation</subject><subject>Nickel</subject><subject>Physical properties</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNp9kc-L1TAQx4so7rp68a5EvIhQTZqmaY5L8Rcs6EHBW0kn0_eypklNUvCd_NfN7ltX8eBcMsz3w5fJfKvqMaOvGOXqNSgAqkTXw53qlPGurUXbf7171QtVS96Kk-pBSpe0FBP9_eqEN1RyKvhp9fPTPuQAOmt3yBaI9oagQ8jxr-H-YGLYoSdrDGaDbIMnW7J-R7yFb-gIhGV1-AMTSdu6hpjRkOlA9rhYpyfr8NrXB19b7wOgz8TZXZmlh9W9WbuEj27es-rL2zefh_f1xcd3H4bzixraRuW6RdFJoFpT07SoOEjTKs214R2bUZsZuJTMqAYpa5iYKfaT7qcOBNfzPEl-Vr04-pYvfN8w5XGxCdA57TFsaWy46IWkraQFff4Pehm26Mt2hZKsXK6ctVAvjxTEkFLEeVyjXXQ8jIyOV7GMgxqG61iGAj-9sdymBc0t-juHAjw5AjHBrfon16I_-58-rmbmvwCSV6Cy</recordid><startdate>20200305</startdate><enddate>20200305</enddate><creator>Inoue, Satoshi</creator><creator>Yan, Yin-Nan</creator><creator>Yamanishi, Katsunori</creator><creator>Kataoka, Yusuke</creator><creator>Kawamoto, Tatsuya</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-3141-1991</orcidid><orcidid>https://orcid.org/0000-0002-3572-1225</orcidid><orcidid>https://orcid.org/0000-0002-3587-3974</orcidid></search><sort><creationdate>20200305</creationdate><title>Photocatalytic and electrocatalytic hydrogen production using nickel complexes supported by hemilabile and non-innocent ligands</title><author>Inoue, Satoshi ; Yan, Yin-Nan ; Yamanishi, Katsunori ; Kataoka, Yusuke ; Kawamoto, Tatsuya</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c429t-4e567c0aa0d24e93c7d49a3ad361feadfc3771d92e01215f0e8ba8b6c53affb73</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Coordination compounds</topic><topic>Crystallography</topic><topic>Hydrogen evolution</topic><topic>Hydrogen production</topic><topic>Imines</topic><topic>Ligands</topic><topic>Light irradiation</topic><topic>Nickel</topic><topic>Physical properties</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Inoue, Satoshi</creatorcontrib><creatorcontrib>Yan, Yin-Nan</creatorcontrib><creatorcontrib>Yamanishi, Katsunori</creatorcontrib><creatorcontrib>Kataoka, Yusuke</creatorcontrib><creatorcontrib>Kawamoto, Tatsuya</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Inoue, Satoshi</au><au>Yan, Yin-Nan</au><au>Yamanishi, Katsunori</au><au>Kataoka, Yusuke</au><au>Kawamoto, Tatsuya</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Photocatalytic and electrocatalytic hydrogen production using nickel complexes supported by hemilabile and non-innocent ligands</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2020-03-05</date><risdate>2020</risdate><volume>56</volume><issue>19</issue><spage>2829</spage><epage>2832</epage><pages>2829-2832</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>Nickel complexes with non-innocent ligands generated by one-electron reduction of octahedral Schiff base nickel(
ii
) complexes with hemilabile ligands exhibited excellent catalytic activities of over 5000 TONs through a metal-ligand cooperation mechanism for hydrogen evolution from water under visible light irradiation.
Square-planar Ni complexes with non-innocent ligands generated by one-electron reduction of octahedral Ni(
ii
) complexes with Schiff base ligands exhibited excellent catalytic activities
via
proton-coupled electron transfer for the H
2
evolution reaction.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>32073053</pmid><doi>10.1039/c9cc09568c</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0002-3141-1991</orcidid><orcidid>https://orcid.org/0000-0002-3572-1225</orcidid><orcidid>https://orcid.org/0000-0002-3587-3974</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2020-03, Vol.56 (19), p.2829-2832 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_proquest_journals_2371073359 |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Coordination compounds Crystallography Hydrogen evolution Hydrogen production Imines Ligands Light irradiation Nickel Physical properties |
| title | Photocatalytic and electrocatalytic hydrogen production using nickel complexes supported by hemilabile and non-innocent ligands |
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