Geochromatographic migration of oil pollution from a heating plant to river sediments
Many pollution sources are difficult to identify because pollutants are transported far away into complex environments. In particular, the mechanisms of petroleum migration in sediments are poorly known. Here, we studied two sediments from the circuit of a heating plant and three sediments located a...
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| Veröffentlicht in: | Environmental chemistry letters 2020-03, Vol.18 (2), p.459-466 |
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| creator | Samelak, Ivan Balaban, Milica Antić, Mališa Šolević Knudsen, Tatjana Jovančićević, Branimir |
| description | Many pollution sources are difficult to identify because pollutants are transported far away into complex environments. In particular, the mechanisms of petroleum migration in sediments are poorly known. Here, we studied two sediments from the circuit of a heating plant and three sediments located at 100, 200 and 300 m away from the plant. Saturated hydrocarbons were isolated and group composition was determined by column chromatography.
n
-Alkanes, terpanes and steranes were analyzed by gas chromatography-mass spectrometry. Results show that the amount of short
n
-alkanes increases during migration, which indicates the migration mechanism. Results on steranes reveal a geochromatographic migration of the oil, where the fastest eluting stereoisomers display the longest migration path. Changes in the distribution of biological markers are explained by migration in water. |
| doi_str_mv | 10.1007/s10311-019-00937-2 |
| format | Article |
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n
-Alkanes, terpanes and steranes were analyzed by gas chromatography-mass spectrometry. Results show that the amount of short
n
-alkanes increases during migration, which indicates the migration mechanism. Results on steranes reveal a geochromatographic migration of the oil, where the fastest eluting stereoisomers display the longest migration path. Changes in the distribution of biological markers are explained by migration in water.</description><identifier>ISSN: 1610-3653</identifier><identifier>EISSN: 1610-3661</identifier><identifier>DOI: 10.1007/s10311-019-00937-2</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Alkanes ; Analytical Chemistry ; Biomarkers ; Chromatography ; Circuits ; Column chromatography ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Fluvial sediments ; Gas chromatography ; Geochemistry ; Heating ; Heating equipment ; Mass spectrometry ; Mass spectroscopy ; Oil pollution ; Original Paper ; Petroleum ; Pollutants ; Pollution ; Pollution sources ; Rivers ; Saturated hydrocarbons ; Sediment ; Sediments ; Stereoisomers ; Water analysis ; Water pollution</subject><ispartof>Environmental chemistry letters, 2020-03, Vol.18 (2), p.459-466</ispartof><rights>Springer Nature Switzerland AG 2019</rights><rights>Environmental Chemistry Letters is a copyright of Springer, (2019). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c363t-c155cf814ad2b2843e6c27201578d4924aa8fbbdb83246828a77ae2d8c4b84503</citedby><cites>FETCH-LOGICAL-c363t-c155cf814ad2b2843e6c27201578d4924aa8fbbdb83246828a77ae2d8c4b84503</cites><orcidid>0000-0001-7095-4764</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10311-019-00937-2$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10311-019-00937-2$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27903,27904,41467,42536,51297</link.rule.ids></links><search><creatorcontrib>Samelak, Ivan</creatorcontrib><creatorcontrib>Balaban, Milica</creatorcontrib><creatorcontrib>Antić, Mališa</creatorcontrib><creatorcontrib>Šolević Knudsen, Tatjana</creatorcontrib><creatorcontrib>Jovančićević, Branimir</creatorcontrib><title>Geochromatographic migration of oil pollution from a heating plant to river sediments</title><title>Environmental chemistry letters</title><addtitle>Environ Chem Lett</addtitle><description>Many pollution sources are difficult to identify because pollutants are transported far away into complex environments. In particular, the mechanisms of petroleum migration in sediments are poorly known. Here, we studied two sediments from the circuit of a heating plant and three sediments located at 100, 200 and 300 m away from the plant. Saturated hydrocarbons were isolated and group composition was determined by column chromatography.
n
-Alkanes, terpanes and steranes were analyzed by gas chromatography-mass spectrometry. Results show that the amount of short
n
-alkanes increases during migration, which indicates the migration mechanism. Results on steranes reveal a geochromatographic migration of the oil, where the fastest eluting stereoisomers display the longest migration path. Changes in the distribution of biological markers are explained by migration in water.</description><subject>Alkanes</subject><subject>Analytical Chemistry</subject><subject>Biomarkers</subject><subject>Chromatography</subject><subject>Circuits</subject><subject>Column chromatography</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Fluvial sediments</subject><subject>Gas chromatography</subject><subject>Geochemistry</subject><subject>Heating</subject><subject>Heating equipment</subject><subject>Mass spectrometry</subject><subject>Mass spectroscopy</subject><subject>Oil pollution</subject><subject>Original Paper</subject><subject>Petroleum</subject><subject>Pollutants</subject><subject>Pollution</subject><subject>Pollution sources</subject><subject>Rivers</subject><subject>Saturated hydrocarbons</subject><subject>Sediment</subject><subject>Sediments</subject><subject>Stereoisomers</subject><subject>Water analysis</subject><subject>Water pollution</subject><issn>1610-3653</issn><issn>1610-3661</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp9UMtOwzAQtBBIlMIPcLLE2eBXHOeIKihIlbjQs-U4TusqiYPtIPH3uA2CG6cd7c7M7g4AtwTfE4zLh0gwIwRhUiGMK1YiegYWRBCMmBDk_BcX7BJcxXjAmNKS0gXYrq03--B7nfwu6HHvDOxdRsn5AfoWetfB0XfddGq0mQk13Ns8H3Zw7PSQYPIwuE8bYLSN6-2Q4jW4aHUX7c1PXYLt89P76gVt3tavq8cNMkywhAwpCtNKwnVDayo5s8LkszApStnwinKtZVvXTS0Z5UJSqctSW9pIw2vJC8yW4G72HYP_mGxM6uCnMOSVih4frzAXNLPozDLBxxhsq8bgeh2-FMHqGJ-a41M5PnWKTx1FbBbFTB52NvxZ_6P6Bv9Lcs4</recordid><startdate>20200301</startdate><enddate>20200301</enddate><creator>Samelak, Ivan</creator><creator>Balaban, Milica</creator><creator>Antić, Mališa</creator><creator>Šolević Knudsen, Tatjana</creator><creator>Jovančićević, Branimir</creator><general>Springer International Publishing</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QH</scope><scope>7ST</scope><scope>7UA</scope><scope>7XB</scope><scope>88I</scope><scope>8AO</scope><scope>8FE</scope><scope>8FG</scope><scope>8FK</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>BHPHI</scope><scope>BKSAR</scope><scope>C1K</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>F1W</scope><scope>GNUQQ</scope><scope>H97</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>L.G</scope><scope>M2P</scope><scope>PATMY</scope><scope>PCBAR</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>SOI</scope><orcidid>https://orcid.org/0000-0001-7095-4764</orcidid></search><sort><creationdate>20200301</creationdate><title>Geochromatographic migration of oil pollution from a heating plant to river sediments</title><author>Samelak, Ivan ; 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In particular, the mechanisms of petroleum migration in sediments are poorly known. Here, we studied two sediments from the circuit of a heating plant and three sediments located at 100, 200 and 300 m away from the plant. Saturated hydrocarbons were isolated and group composition was determined by column chromatography.
n
-Alkanes, terpanes and steranes were analyzed by gas chromatography-mass spectrometry. Results show that the amount of short
n
-alkanes increases during migration, which indicates the migration mechanism. Results on steranes reveal a geochromatographic migration of the oil, where the fastest eluting stereoisomers display the longest migration path. Changes in the distribution of biological markers are explained by migration in water.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s10311-019-00937-2</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0001-7095-4764</orcidid><oa>free_for_read</oa></addata></record> |
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| subjects | Alkanes Analytical Chemistry Biomarkers Chromatography Circuits Column chromatography Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Fluvial sediments Gas chromatography Geochemistry Heating Heating equipment Mass spectrometry Mass spectroscopy Oil pollution Original Paper Petroleum Pollutants Pollution Pollution sources Rivers Saturated hydrocarbons Sediment Sediments Stereoisomers Water analysis Water pollution |
| title | Geochromatographic migration of oil pollution from a heating plant to river sediments |
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