Highly flexible, stable and transparent capacitors with enhanced performances by composite electrodes of AZO and metallic nanomeshes
Transparent and flexible capacitors with composite electrodes consisting of ZnO:Al(AZO) and Cr–Au nanomeshes and dielectric ZrO2 films were directly prepared on plastic substrates. The transparent composite electrodes exhibited an ultralow sheet resistance (5.6 Ω·square−1) and good flexural properti...
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Veröffentlicht in: | Journal of alloys and compounds 2020-04, Vol.819, p.152973, Article 152973 |
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creator | Guo, Tao Zhang, Guozhen Zhang, Heng Su, Xi Chen, Xue Wan, Jiaxian Wu, Hao Liu, Chang |
description | Transparent and flexible capacitors with composite electrodes consisting of ZnO:Al(AZO) and Cr–Au nanomeshes and dielectric ZrO2 films were directly prepared on plastic substrates. The transparent composite electrodes exhibited an ultralow sheet resistance (5.6 Ω·square−1) and good flexural properties. ZrO2 thin films were grown by atomic layer deposition to serve as dielectric layers. The capacitors showed a higher capacitance density (17.8 fF μm−2) than that capacitors with AZO electrodes (9.8 fF μm−2) while maintained an extra-low leakage current density (1.3 × 10−9 A cm−2 at 1 V). Additionally, the quality factor was increased from 9.6 to 80.5 at a frequency of 1 MHz with the incorporation of Cr–Au nanomeshes, which greatly reduced the power consumptions. More importantly, the capacitors with the composite electrodes exhibited excellent bendability, good cycling stability, and relatively high transparency. It is, therefore, a promising route for application in developing transparent, flexible, high-performance and low-cost integrated circuits.
•Flexible and transparent capacitors were directly fabricated on low-cost plastic substrate.•A high quality factor of 80.5 was obtained, meaning an extremely low power consumptions.•The electrodes involved in Cr–Au nanomesh can effectively improve the flexible properties of capacitors. |
doi_str_mv | 10.1016/j.jallcom.2019.152973 |
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•Flexible and transparent capacitors were directly fabricated on low-cost plastic substrate.•A high quality factor of 80.5 was obtained, meaning an extremely low power consumptions.•The electrodes involved in Cr–Au nanomesh can effectively improve the flexible properties of capacitors.</description><identifier>ISSN: 0925-8388</identifier><identifier>EISSN: 1873-4669</identifier><identifier>DOI: 10.1016/j.jallcom.2019.152973</identifier><language>eng</language><publisher>Lausanne: Elsevier B.V</publisher><subject>Atomic layer deposition ; Atomic layer epitaxy ; Capacitors ; Electrodes ; Flexible electronic devices ; Integrated circuits ; Leakage current ; Performance enhancement ; Power consumption ; Q factors ; Substrates ; Thin films ; Transparent conductive films ; Zinc oxide ; Zirconium dioxide</subject><ispartof>Journal of alloys and compounds, 2020-04, Vol.819, p.152973, Article 152973</ispartof><rights>2019 Elsevier B.V.</rights><rights>Copyright Elsevier BV Apr 5, 2020</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c337t-45a001eac4a14c349a310d606fa567c32f2d7fcfb216dfb3d407d42c674aaf553</citedby><cites>FETCH-LOGICAL-c337t-45a001eac4a14c349a310d606fa567c32f2d7fcfb216dfb3d407d42c674aaf553</cites><orcidid>0000-0002-6232-5551 ; 0000-0002-5010-3986</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.jallcom.2019.152973$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids></links><search><creatorcontrib>Guo, Tao</creatorcontrib><creatorcontrib>Zhang, Guozhen</creatorcontrib><creatorcontrib>Zhang, Heng</creatorcontrib><creatorcontrib>Su, Xi</creatorcontrib><creatorcontrib>Chen, Xue</creatorcontrib><creatorcontrib>Wan, Jiaxian</creatorcontrib><creatorcontrib>Wu, Hao</creatorcontrib><creatorcontrib>Liu, Chang</creatorcontrib><title>Highly flexible, stable and transparent capacitors with enhanced performances by composite electrodes of AZO and metallic nanomeshes</title><title>Journal of alloys and compounds</title><description>Transparent and flexible capacitors with composite electrodes consisting of ZnO:Al(AZO) and Cr–Au nanomeshes and dielectric ZrO2 films were directly prepared on plastic substrates. The transparent composite electrodes exhibited an ultralow sheet resistance (5.6 Ω·square−1) and good flexural properties. ZrO2 thin films were grown by atomic layer deposition to serve as dielectric layers. The capacitors showed a higher capacitance density (17.8 fF μm−2) than that capacitors with AZO electrodes (9.8 fF μm−2) while maintained an extra-low leakage current density (1.3 × 10−9 A cm−2 at 1 V). Additionally, the quality factor was increased from 9.6 to 80.5 at a frequency of 1 MHz with the incorporation of Cr–Au nanomeshes, which greatly reduced the power consumptions. More importantly, the capacitors with the composite electrodes exhibited excellent bendability, good cycling stability, and relatively high transparency. It is, therefore, a promising route for application in developing transparent, flexible, high-performance and low-cost integrated circuits.
•Flexible and transparent capacitors were directly fabricated on low-cost plastic substrate.•A high quality factor of 80.5 was obtained, meaning an extremely low power consumptions.•The electrodes involved in Cr–Au nanomesh can effectively improve the flexible properties of capacitors.</description><subject>Atomic layer deposition</subject><subject>Atomic layer epitaxy</subject><subject>Capacitors</subject><subject>Electrodes</subject><subject>Flexible electronic devices</subject><subject>Integrated circuits</subject><subject>Leakage current</subject><subject>Performance enhancement</subject><subject>Power consumption</subject><subject>Q factors</subject><subject>Substrates</subject><subject>Thin films</subject><subject>Transparent conductive films</subject><subject>Zinc oxide</subject><subject>Zirconium dioxide</subject><issn>0925-8388</issn><issn>1873-4669</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNqFkE9v1DAQxa2KSl1aPgKSJa5k8b84yQlVFVCkSr3QSy_WrD1mHSVxsF3o3vvB8bK9cxrN6M2bNz9C3nO25YzrT-N2hGmycd4Kxoctb8XQyTOy4X0nG6X18IZs2CDappd9f0He5jwyVpWSb8jLbfi5nw7UT_gcdhN-pLlArRQWR0uCJa-QcCnUwgo2lJgy_RPKnuKyh8WioysmH9N8bDLdHWjNscYcClKc0JYUXZ1HT68f7_-Zzlhq2mDpAkucMe8xX5FzD1PGd6_1kjx8_fLj5ra5u__2_eb6rrFSdqVRLdTYCFYBV1aqASRnTjPtodWdlcIL13nrd4Jr53fSKdY5JazuFIBvW3lJPpx81xR_PWEuZoxPaaknjZCt6oWWkldVe1LZFHNO6M2awgzpYDgzR-BmNK_AzRG4OQGve59Pe1hf-B0wmWwDHhmFVEEYF8N_HP4CtKGO1Q</recordid><startdate>20200405</startdate><enddate>20200405</enddate><creator>Guo, Tao</creator><creator>Zhang, Guozhen</creator><creator>Zhang, Heng</creator><creator>Su, Xi</creator><creator>Chen, Xue</creator><creator>Wan, Jiaxian</creator><creator>Wu, Hao</creator><creator>Liu, Chang</creator><general>Elsevier B.V</general><general>Elsevier BV</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><orcidid>https://orcid.org/0000-0002-6232-5551</orcidid><orcidid>https://orcid.org/0000-0002-5010-3986</orcidid></search><sort><creationdate>20200405</creationdate><title>Highly flexible, stable and transparent capacitors with enhanced performances by composite electrodes of AZO and metallic nanomeshes</title><author>Guo, Tao ; Zhang, Guozhen ; Zhang, Heng ; Su, Xi ; Chen, Xue ; Wan, Jiaxian ; Wu, Hao ; Liu, Chang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c337t-45a001eac4a14c349a310d606fa567c32f2d7fcfb216dfb3d407d42c674aaf553</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Atomic layer deposition</topic><topic>Atomic layer epitaxy</topic><topic>Capacitors</topic><topic>Electrodes</topic><topic>Flexible electronic devices</topic><topic>Integrated circuits</topic><topic>Leakage current</topic><topic>Performance enhancement</topic><topic>Power consumption</topic><topic>Q factors</topic><topic>Substrates</topic><topic>Thin films</topic><topic>Transparent conductive films</topic><topic>Zinc oxide</topic><topic>Zirconium dioxide</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Guo, Tao</creatorcontrib><creatorcontrib>Zhang, Guozhen</creatorcontrib><creatorcontrib>Zhang, Heng</creatorcontrib><creatorcontrib>Su, Xi</creatorcontrib><creatorcontrib>Chen, Xue</creatorcontrib><creatorcontrib>Wan, Jiaxian</creatorcontrib><creatorcontrib>Wu, Hao</creatorcontrib><creatorcontrib>Liu, Chang</creatorcontrib><collection>CrossRef</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><jtitle>Journal of alloys and compounds</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Guo, Tao</au><au>Zhang, Guozhen</au><au>Zhang, Heng</au><au>Su, Xi</au><au>Chen, Xue</au><au>Wan, Jiaxian</au><au>Wu, Hao</au><au>Liu, Chang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Highly flexible, stable and transparent capacitors with enhanced performances by composite electrodes of AZO and metallic nanomeshes</atitle><jtitle>Journal of alloys and compounds</jtitle><date>2020-04-05</date><risdate>2020</risdate><volume>819</volume><spage>152973</spage><pages>152973-</pages><artnum>152973</artnum><issn>0925-8388</issn><eissn>1873-4669</eissn><abstract>Transparent and flexible capacitors with composite electrodes consisting of ZnO:Al(AZO) and Cr–Au nanomeshes and dielectric ZrO2 films were directly prepared on plastic substrates. The transparent composite electrodes exhibited an ultralow sheet resistance (5.6 Ω·square−1) and good flexural properties. ZrO2 thin films were grown by atomic layer deposition to serve as dielectric layers. The capacitors showed a higher capacitance density (17.8 fF μm−2) than that capacitors with AZO electrodes (9.8 fF μm−2) while maintained an extra-low leakage current density (1.3 × 10−9 A cm−2 at 1 V). Additionally, the quality factor was increased from 9.6 to 80.5 at a frequency of 1 MHz with the incorporation of Cr–Au nanomeshes, which greatly reduced the power consumptions. More importantly, the capacitors with the composite electrodes exhibited excellent bendability, good cycling stability, and relatively high transparency. It is, therefore, a promising route for application in developing transparent, flexible, high-performance and low-cost integrated circuits.
•Flexible and transparent capacitors were directly fabricated on low-cost plastic substrate.•A high quality factor of 80.5 was obtained, meaning an extremely low power consumptions.•The electrodes involved in Cr–Au nanomesh can effectively improve the flexible properties of capacitors.</abstract><cop>Lausanne</cop><pub>Elsevier B.V</pub><doi>10.1016/j.jallcom.2019.152973</doi><orcidid>https://orcid.org/0000-0002-6232-5551</orcidid><orcidid>https://orcid.org/0000-0002-5010-3986</orcidid></addata></record> |
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subjects | Atomic layer deposition Atomic layer epitaxy Capacitors Electrodes Flexible electronic devices Integrated circuits Leakage current Performance enhancement Power consumption Q factors Substrates Thin films Transparent conductive films Zinc oxide Zirconium dioxide |
title | Highly flexible, stable and transparent capacitors with enhanced performances by composite electrodes of AZO and metallic nanomeshes |
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