Degradation of high-concentration simulated organic wastewater by DBD plasma

In this study, a high-concentration simulated organic wastewater, made by dissolving methyl violet in water, was degraded using dielectric barrier discharge (DBD) plasma generated in air and O respectively. The decoloration rate and chemical oxygen demand (COD) of wastewater were evaluated during pl...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Water science and technology 2019-10, Vol.80 (8), p.1413-1420
Hauptverfasser: Wang, Xing-Quan, Li, Xing, Zhou, Ren-Wu, Huang, Jun, Chen, Wei, Wang, Feng-Peng, Lu, Xiu-Yuan, Wen, Qian
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 1420
container_issue 8
container_start_page 1413
container_title Water science and technology
container_volume 80
creator Wang, Xing-Quan
Li, Xing
Zhou, Ren-Wu
Huang, Jun
Chen, Wei
Wang, Feng-Peng
Lu, Xiu-Yuan
Wen, Qian
description In this study, a high-concentration simulated organic wastewater, made by dissolving methyl violet in water, was degraded using dielectric barrier discharge (DBD) plasma generated in air and O respectively. The decoloration rate and chemical oxygen demand (COD) of wastewater were evaluated during plasma treatments with the initial concentration of methyl violet of 300 mg L . Results showed that the highest decoloration rate of around 100% within 10 min and the highest COD decrease of 33% within 60 min could be achieved with the O plasma treatment at the discharge voltage of 10 kV, while air plasma treatment showed lower efficiency in decolorizing the methyl violet solution and lower COD decrease (24%) after 60 min treatment. UV-Vis spectroscopy and chemical analysis of generated by-products during the plasma-enabled degradation process revealed that the methyl violet molecules could be completely decomposed into some refractory organics in the solution. Based on the experimental results and literature review, a pathway of methyl violet degradation attributed to energetic electrons and highly reactive species generated by DBD was proposed.
doi_str_mv 10.2166/wst.2019.389
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2350183381</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2350183381</sourcerecordid><originalsourceid>FETCH-LOGICAL-c319t-b4da86e5a4d4e8bfe8172f2d3c2da7601d9c0aaa076433af23431da92afa36973</originalsourceid><addsrcrecordid>eNo9kN9LwzAUhYMobk7ffJaCr7YmuVnaPOrmLxj4os_htkm2jrWdScvYf2_Gpk8XDh_ncD9CbhnNOJPycRf6jFOmMijUGRkzpWSqcuDnZEx5DinjHEbkKoQ1pTQHQS_JCJiSrKBiTBZzu_RosK-7NulcsqqXq7Tq2sq2vT-moW6GDfbWJJ1fYltXyQ5Db3cx8km5T-bP82S7wdDgNblwuAn25nQn5Pv15Wv2ni4-3z5mT4u0isN9WgqDhbRTFEbYonS2YDl33EDFDeaSMqMqiog0lwIAHQcBzKDi6BBk_G1C7o-9W9_9DDb0et0Nvo2TmsOUsgKgYJF6OFKV70Lw1umtrxv0e82oPqjTUZ0-qNNRXcTvTqVD2VjzD_-5gl-1O2oh</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2350183381</pqid></control><display><type>article</type><title>Degradation of high-concentration simulated organic wastewater by DBD plasma</title><source>MEDLINE</source><source>EZB Electronic Journals Library</source><creator>Wang, Xing-Quan ; Li, Xing ; Zhou, Ren-Wu ; Huang, Jun ; Chen, Wei ; Wang, Feng-Peng ; Lu, Xiu-Yuan ; Wen, Qian</creator><creatorcontrib>Wang, Xing-Quan ; Li, Xing ; Zhou, Ren-Wu ; Huang, Jun ; Chen, Wei ; Wang, Feng-Peng ; Lu, Xiu-Yuan ; Wen, Qian</creatorcontrib><description>In this study, a high-concentration simulated organic wastewater, made by dissolving methyl violet in water, was degraded using dielectric barrier discharge (DBD) plasma generated in air and O respectively. The decoloration rate and chemical oxygen demand (COD) of wastewater were evaluated during plasma treatments with the initial concentration of methyl violet of 300 mg L . Results showed that the highest decoloration rate of around 100% within 10 min and the highest COD decrease of 33% within 60 min could be achieved with the O plasma treatment at the discharge voltage of 10 kV, while air plasma treatment showed lower efficiency in decolorizing the methyl violet solution and lower COD decrease (24%) after 60 min treatment. UV-Vis spectroscopy and chemical analysis of generated by-products during the plasma-enabled degradation process revealed that the methyl violet molecules could be completely decomposed into some refractory organics in the solution. Based on the experimental results and literature review, a pathway of methyl violet degradation attributed to energetic electrons and highly reactive species generated by DBD was proposed.</description><identifier>ISSN: 0273-1223</identifier><identifier>EISSN: 1996-9732</identifier><identifier>DOI: 10.2166/wst.2019.389</identifier><identifier>PMID: 31961804</identifier><language>eng</language><publisher>England: IWA Publishing</publisher><subject>Air plasma ; Analytical methods ; Biological Oxygen Demand Analysis ; By-products ; Chemical analysis ; Chemical oxygen demand ; Color removal ; Decoloring ; Degradation ; Dielectric barrier discharge ; Drinking water ; Efficiency ; Electrodes ; Gases ; Gentian Violet ; Literature reviews ; Organic chemistry ; Organic wastes ; Pharmaceutical industry ; Phenols ; Plasma ; Pollutants ; Power supply ; Spectroscopy ; Ultraviolet spectroscopy ; Waste Water ; Wastewater ; Water Pollutants, Chemical ; Water Purification ; Water treatment</subject><ispartof>Water science and technology, 2019-10, Vol.80 (8), p.1413-1420</ispartof><rights>Copyright IWA Publishing Oct 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-b4da86e5a4d4e8bfe8172f2d3c2da7601d9c0aaa076433af23431da92afa36973</citedby><cites>FETCH-LOGICAL-c319t-b4da86e5a4d4e8bfe8172f2d3c2da7601d9c0aaa076433af23431da92afa36973</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/31961804$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Wang, Xing-Quan</creatorcontrib><creatorcontrib>Li, Xing</creatorcontrib><creatorcontrib>Zhou, Ren-Wu</creatorcontrib><creatorcontrib>Huang, Jun</creatorcontrib><creatorcontrib>Chen, Wei</creatorcontrib><creatorcontrib>Wang, Feng-Peng</creatorcontrib><creatorcontrib>Lu, Xiu-Yuan</creatorcontrib><creatorcontrib>Wen, Qian</creatorcontrib><title>Degradation of high-concentration simulated organic wastewater by DBD plasma</title><title>Water science and technology</title><addtitle>Water Sci Technol</addtitle><description>In this study, a high-concentration simulated organic wastewater, made by dissolving methyl violet in water, was degraded using dielectric barrier discharge (DBD) plasma generated in air and O respectively. The decoloration rate and chemical oxygen demand (COD) of wastewater were evaluated during plasma treatments with the initial concentration of methyl violet of 300 mg L . Results showed that the highest decoloration rate of around 100% within 10 min and the highest COD decrease of 33% within 60 min could be achieved with the O plasma treatment at the discharge voltage of 10 kV, while air plasma treatment showed lower efficiency in decolorizing the methyl violet solution and lower COD decrease (24%) after 60 min treatment. UV-Vis spectroscopy and chemical analysis of generated by-products during the plasma-enabled degradation process revealed that the methyl violet molecules could be completely decomposed into some refractory organics in the solution. Based on the experimental results and literature review, a pathway of methyl violet degradation attributed to energetic electrons and highly reactive species generated by DBD was proposed.</description><subject>Air plasma</subject><subject>Analytical methods</subject><subject>Biological Oxygen Demand Analysis</subject><subject>By-products</subject><subject>Chemical analysis</subject><subject>Chemical oxygen demand</subject><subject>Color removal</subject><subject>Decoloring</subject><subject>Degradation</subject><subject>Dielectric barrier discharge</subject><subject>Drinking water</subject><subject>Efficiency</subject><subject>Electrodes</subject><subject>Gases</subject><subject>Gentian Violet</subject><subject>Literature reviews</subject><subject>Organic chemistry</subject><subject>Organic wastes</subject><subject>Pharmaceutical industry</subject><subject>Phenols</subject><subject>Plasma</subject><subject>Pollutants</subject><subject>Power supply</subject><subject>Spectroscopy</subject><subject>Ultraviolet spectroscopy</subject><subject>Waste Water</subject><subject>Wastewater</subject><subject>Water Pollutants, Chemical</subject><subject>Water Purification</subject><subject>Water treatment</subject><issn>0273-1223</issn><issn>1996-9732</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNo9kN9LwzAUhYMobk7ffJaCr7YmuVnaPOrmLxj4os_htkm2jrWdScvYf2_Gpk8XDh_ncD9CbhnNOJPycRf6jFOmMijUGRkzpWSqcuDnZEx5DinjHEbkKoQ1pTQHQS_JCJiSrKBiTBZzu_RosK-7NulcsqqXq7Tq2sq2vT-moW6GDfbWJJ1fYltXyQ5Db3cx8km5T-bP82S7wdDgNblwuAn25nQn5Pv15Wv2ni4-3z5mT4u0isN9WgqDhbRTFEbYonS2YDl33EDFDeaSMqMqiog0lwIAHQcBzKDi6BBk_G1C7o-9W9_9DDb0et0Nvo2TmsOUsgKgYJF6OFKV70Lw1umtrxv0e82oPqjTUZ0-qNNRXcTvTqVD2VjzD_-5gl-1O2oh</recordid><startdate>20191015</startdate><enddate>20191015</enddate><creator>Wang, Xing-Quan</creator><creator>Li, Xing</creator><creator>Zhou, Ren-Wu</creator><creator>Huang, Jun</creator><creator>Chen, Wei</creator><creator>Wang, Feng-Peng</creator><creator>Lu, Xiu-Yuan</creator><creator>Wen, Qian</creator><general>IWA Publishing</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QH</scope><scope>7UA</scope><scope>7X7</scope><scope>7XB</scope><scope>88E</scope><scope>8FE</scope><scope>8FG</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>BHPHI</scope><scope>BKSAR</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>F1W</scope><scope>FYUFA</scope><scope>GHDGH</scope><scope>H96</scope><scope>H97</scope><scope>HCIFZ</scope><scope>K9.</scope><scope>L.G</scope><scope>L6V</scope><scope>M0S</scope><scope>M1P</scope><scope>M7S</scope><scope>PCBAR</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PTHSS</scope></search><sort><creationdate>20191015</creationdate><title>Degradation of high-concentration simulated organic wastewater by DBD plasma</title><author>Wang, Xing-Quan ; Li, Xing ; Zhou, Ren-Wu ; Huang, Jun ; Chen, Wei ; Wang, Feng-Peng ; Lu, Xiu-Yuan ; Wen, Qian</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-b4da86e5a4d4e8bfe8172f2d3c2da7601d9c0aaa076433af23431da92afa36973</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Air plasma</topic><topic>Analytical methods</topic><topic>Biological Oxygen Demand Analysis</topic><topic>By-products</topic><topic>Chemical analysis</topic><topic>Chemical oxygen demand</topic><topic>Color removal</topic><topic>Decoloring</topic><topic>Degradation</topic><topic>Dielectric barrier discharge</topic><topic>Drinking water</topic><topic>Efficiency</topic><topic>Electrodes</topic><topic>Gases</topic><topic>Gentian Violet</topic><topic>Literature reviews</topic><topic>Organic chemistry</topic><topic>Organic wastes</topic><topic>Pharmaceutical industry</topic><topic>Phenols</topic><topic>Plasma</topic><topic>Pollutants</topic><topic>Power supply</topic><topic>Spectroscopy</topic><topic>Ultraviolet spectroscopy</topic><topic>Waste Water</topic><topic>Wastewater</topic><topic>Water Pollutants, Chemical</topic><topic>Water Purification</topic><topic>Water treatment</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Xing-Quan</creatorcontrib><creatorcontrib>Li, Xing</creatorcontrib><creatorcontrib>Zhou, Ren-Wu</creatorcontrib><creatorcontrib>Huang, Jun</creatorcontrib><creatorcontrib>Chen, Wei</creatorcontrib><creatorcontrib>Wang, Feng-Peng</creatorcontrib><creatorcontrib>Lu, Xiu-Yuan</creatorcontrib><creatorcontrib>Wen, Qian</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Aqualine</collection><collection>Water Resources Abstracts</collection><collection>Health &amp; Medical Collection (Proquest)</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Medical Database (Alumni Edition)</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>Materials Science &amp; Engineering Collection</collection><collection>ProQuest Central (Alumni)</collection><collection>ProQuest One Sustainability</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest Natural Science Collection</collection><collection>Earth, Atmospheric &amp; Aquatic Science Collection</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Health Research Premium Collection</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>Aquatic Science &amp; Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy &amp; Non-Living Resources</collection><collection>Aquatic Science &amp; Fisheries Abstracts (ASFA) 3: Aquatic Pollution &amp; Environmental Quality</collection><collection>SciTech Premium Collection (Proquest) (PQ_SDU_P3)</collection><collection>ProQuest Health &amp; Medical Complete (Alumni)</collection><collection>Aquatic Science &amp; Fisheries Abstracts (ASFA) Professional</collection><collection>ProQuest Engineering Collection</collection><collection>Health &amp; Medical Collection (Alumni Edition)</collection><collection>PML(ProQuest Medical Library)</collection><collection>Engineering Database</collection><collection>Earth, Atmospheric &amp; Aquatic Science Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Engineering Collection</collection><jtitle>Water science and technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wang, Xing-Quan</au><au>Li, Xing</au><au>Zhou, Ren-Wu</au><au>Huang, Jun</au><au>Chen, Wei</au><au>Wang, Feng-Peng</au><au>Lu, Xiu-Yuan</au><au>Wen, Qian</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Degradation of high-concentration simulated organic wastewater by DBD plasma</atitle><jtitle>Water science and technology</jtitle><addtitle>Water Sci Technol</addtitle><date>2019-10-15</date><risdate>2019</risdate><volume>80</volume><issue>8</issue><spage>1413</spage><epage>1420</epage><pages>1413-1420</pages><issn>0273-1223</issn><eissn>1996-9732</eissn><abstract>In this study, a high-concentration simulated organic wastewater, made by dissolving methyl violet in water, was degraded using dielectric barrier discharge (DBD) plasma generated in air and O respectively. The decoloration rate and chemical oxygen demand (COD) of wastewater were evaluated during plasma treatments with the initial concentration of methyl violet of 300 mg L . Results showed that the highest decoloration rate of around 100% within 10 min and the highest COD decrease of 33% within 60 min could be achieved with the O plasma treatment at the discharge voltage of 10 kV, while air plasma treatment showed lower efficiency in decolorizing the methyl violet solution and lower COD decrease (24%) after 60 min treatment. UV-Vis spectroscopy and chemical analysis of generated by-products during the plasma-enabled degradation process revealed that the methyl violet molecules could be completely decomposed into some refractory organics in the solution. Based on the experimental results and literature review, a pathway of methyl violet degradation attributed to energetic electrons and highly reactive species generated by DBD was proposed.</abstract><cop>England</cop><pub>IWA Publishing</pub><pmid>31961804</pmid><doi>10.2166/wst.2019.389</doi><tpages>8</tpages></addata></record>
fulltext fulltext
identifier ISSN: 0273-1223
ispartof Water science and technology, 2019-10, Vol.80 (8), p.1413-1420
issn 0273-1223
1996-9732
language eng
recordid cdi_proquest_journals_2350183381
source MEDLINE; EZB Electronic Journals Library
subjects Air plasma
Analytical methods
Biological Oxygen Demand Analysis
By-products
Chemical analysis
Chemical oxygen demand
Color removal
Decoloring
Degradation
Dielectric barrier discharge
Drinking water
Efficiency
Electrodes
Gases
Gentian Violet
Literature reviews
Organic chemistry
Organic wastes
Pharmaceutical industry
Phenols
Plasma
Pollutants
Power supply
Spectroscopy
Ultraviolet spectroscopy
Waste Water
Wastewater
Water Pollutants, Chemical
Water Purification
Water treatment
title Degradation of high-concentration simulated organic wastewater by DBD plasma
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-07T18%3A28%3A51IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Degradation%20of%20high-concentration%20simulated%20organic%20wastewater%20by%20DBD%20plasma&rft.jtitle=Water%20science%20and%20technology&rft.au=Wang,%20Xing-Quan&rft.date=2019-10-15&rft.volume=80&rft.issue=8&rft.spage=1413&rft.epage=1420&rft.pages=1413-1420&rft.issn=0273-1223&rft.eissn=1996-9732&rft_id=info:doi/10.2166/wst.2019.389&rft_dat=%3Cproquest_cross%3E2350183381%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2350183381&rft_id=info:pmid/31961804&rfr_iscdi=true