Generalized Kinetic Equation for Interaction between Liquid-Phase Silicon and Pyrolytic Carbon Surface
An interaction between the surface of pyrolytic carbon and silicon melt within the temperature range of 1600–2000°C is studied in this work. We showed that this process is multistage and consists of kinetic, diffusion, and transition stages. We found that growth of β-silicon carbide during the liqui...
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| Veröffentlicht in: | Protection of metals and physical chemistry of surfaces 2019-12, Vol.55 (7), p.1277-1279 |
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| container_title | Protection of metals and physical chemistry of surfaces |
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| creator | Sinani, I. L. Bushuev, V. M. Lunegov, S. G. |
| description | An interaction between the surface of pyrolytic carbon and silicon melt within the temperature range of 1600–2000°C is studied in this work. We showed that this process is multistage and consists of kinetic, diffusion, and transition stages. We found that growth of β-silicon carbide during the liquid-phase interaction between silicon and the surface of pyrolytic carbon obeys kinetic law and we found the duration of the kinetic stage within the temperature range. We showed that there is an increase in the exponent when the stages of the process are changed, the thickness of the carbide layer increases in the range 1 ≤
n
≤ 2, and the activation energy increases from the kinetic stage to the diffusion one. This leads to control of the process by the diffusion stage being the longest in time parameter. |
| doi_str_mv | 10.1134/S2070205119070177 |
| format | Article |
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n
≤ 2, and the activation energy increases from the kinetic stage to the diffusion one. This leads to control of the process by the diffusion stage being the longest in time parameter.</description><identifier>ISSN: 2070-2051</identifier><identifier>EISSN: 2070-206X</identifier><identifier>DOI: 10.1134/S2070205119070177</identifier><language>eng</language><publisher>Moscow: Pleiades Publishing</publisher><subject>Carbon ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Corrosion and Coatings ; Diffusion ; General Issues of Corrosion ; Industrial Chemistry/Chemical Engineering ; Inorganic Chemistry ; Kinetic equations ; Liquid phases ; Materials Science ; Metallic Materials ; Silicon ; Silicon carbide ; Thickness ; Tribology</subject><ispartof>Protection of metals and physical chemistry of surfaces, 2019-12, Vol.55 (7), p.1277-1279</ispartof><rights>Pleiades Publishing, Ltd. 2019</rights><rights>2019© Pleiades Publishing, Ltd. 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c305t-d0295e5de24fd08c36665f475bb4a5d59800c10daad6182e88fdb958f6d785d53</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1134/S2070205119070177$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1134/S2070205119070177$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Sinani, I. L.</creatorcontrib><creatorcontrib>Bushuev, V. M.</creatorcontrib><creatorcontrib>Lunegov, S. G.</creatorcontrib><title>Generalized Kinetic Equation for Interaction between Liquid-Phase Silicon and Pyrolytic Carbon Surface</title><title>Protection of metals and physical chemistry of surfaces</title><addtitle>Prot Met Phys Chem Surf</addtitle><description>An interaction between the surface of pyrolytic carbon and silicon melt within the temperature range of 1600–2000°C is studied in this work. We showed that this process is multistage and consists of kinetic, diffusion, and transition stages. We found that growth of β-silicon carbide during the liquid-phase interaction between silicon and the surface of pyrolytic carbon obeys kinetic law and we found the duration of the kinetic stage within the temperature range. We showed that there is an increase in the exponent when the stages of the process are changed, the thickness of the carbide layer increases in the range 1 ≤
n
≤ 2, and the activation energy increases from the kinetic stage to the diffusion one. This leads to control of the process by the diffusion stage being the longest in time parameter.</description><subject>Carbon</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Corrosion and Coatings</subject><subject>Diffusion</subject><subject>General Issues of Corrosion</subject><subject>Industrial Chemistry/Chemical Engineering</subject><subject>Inorganic Chemistry</subject><subject>Kinetic equations</subject><subject>Liquid phases</subject><subject>Materials Science</subject><subject>Metallic Materials</subject><subject>Silicon</subject><subject>Silicon carbide</subject><subject>Thickness</subject><subject>Tribology</subject><issn>2070-2051</issn><issn>2070-206X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNp1UE1LAzEQDaJgrf4AbwueV5Ps5mOPUqoWCxaq4G3JJhNNWbNtsovUX29qRQ_iad7M-xh4CJ0TfElIUV4tKRaYYkZIlQAR4gCNdqecYv58-IMZOUYnMa4w5lxIMUL2FjwE1boPMNm989A7nU03g-pd5zPbhWzm-yTQX3sD_TuAz-ZuMziTL15VhGzpWqcTqbzJFtvQtdtdxkSFJh2XQ7BKwyk6sqqNcPY9x-jpZvo4ucvnD7ezyfU81wVmfW4wrRgwA7S0BktdcM6ZLQVrmlIxwyqJsSbYKGU4kRSktKapmLTcCJn4Yowu9rnr0G0GiH296obg08uaFmVBJZccJxXZq3ToYgxg63Vwbypsa4LrXZ31nzqTh-49MWn9C4Tf5P9Nn5sqdzw</recordid><startdate>20191201</startdate><enddate>20191201</enddate><creator>Sinani, I. L.</creator><creator>Bushuev, V. M.</creator><creator>Lunegov, S. G.</creator><general>Pleiades Publishing</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope></search><sort><creationdate>20191201</creationdate><title>Generalized Kinetic Equation for Interaction between Liquid-Phase Silicon and Pyrolytic Carbon Surface</title><author>Sinani, I. L. ; Bushuev, V. M. ; Lunegov, S. G.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c305t-d0295e5de24fd08c36665f475bb4a5d59800c10daad6182e88fdb958f6d785d53</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Carbon</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Corrosion and Coatings</topic><topic>Diffusion</topic><topic>General Issues of Corrosion</topic><topic>Industrial Chemistry/Chemical Engineering</topic><topic>Inorganic Chemistry</topic><topic>Kinetic equations</topic><topic>Liquid phases</topic><topic>Materials Science</topic><topic>Metallic Materials</topic><topic>Silicon</topic><topic>Silicon carbide</topic><topic>Thickness</topic><topic>Tribology</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Sinani, I. L.</creatorcontrib><creatorcontrib>Bushuev, V. M.</creatorcontrib><creatorcontrib>Lunegov, S. G.</creatorcontrib><collection>CrossRef</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><jtitle>Protection of metals and physical chemistry of surfaces</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Sinani, I. L.</au><au>Bushuev, V. M.</au><au>Lunegov, S. G.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Generalized Kinetic Equation for Interaction between Liquid-Phase Silicon and Pyrolytic Carbon Surface</atitle><jtitle>Protection of metals and physical chemistry of surfaces</jtitle><stitle>Prot Met Phys Chem Surf</stitle><date>2019-12-01</date><risdate>2019</risdate><volume>55</volume><issue>7</issue><spage>1277</spage><epage>1279</epage><pages>1277-1279</pages><issn>2070-2051</issn><eissn>2070-206X</eissn><abstract>An interaction between the surface of pyrolytic carbon and silicon melt within the temperature range of 1600–2000°C is studied in this work. We showed that this process is multistage and consists of kinetic, diffusion, and transition stages. We found that growth of β-silicon carbide during the liquid-phase interaction between silicon and the surface of pyrolytic carbon obeys kinetic law and we found the duration of the kinetic stage within the temperature range. We showed that there is an increase in the exponent when the stages of the process are changed, the thickness of the carbide layer increases in the range 1 ≤
n
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| subjects | Carbon Characterization and Evaluation of Materials Chemistry and Materials Science Corrosion and Coatings Diffusion General Issues of Corrosion Industrial Chemistry/Chemical Engineering Inorganic Chemistry Kinetic equations Liquid phases Materials Science Metallic Materials Silicon Silicon carbide Thickness Tribology |
| title | Generalized Kinetic Equation for Interaction between Liquid-Phase Silicon and Pyrolytic Carbon Surface |
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