Absence of Magnetic Thermal Conductivity in the Quantum Spin Liquid Candidate EtMe3Sb[Pd(dmit)2]2

We present the ultralow-temperature specific heat and thermal conductivity measurements on single crystals of triangular-lattice compound EtMe3Sb[Pd(dmit)2]2, which has long been considered as a gapless quantum spin liquid candidate. In specific heat measurements, a finite linear term is observed, c...

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Veröffentlicht in:Physical review letters 2019-12, Vol.123 (24), p.1
Hauptverfasser: Ni, J M, Pan, B L, Song, B Q, Huang, Y Y, Zeng, J Y, Yu, Y J, Cheng, E J, Wang, L S, Dai, D Z, Kato, R, Li, S Y
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container_issue 24
container_start_page 1
container_title Physical review letters
container_volume 123
creator Ni, J M
Pan, B L
Song, B Q
Huang, Y Y
Zeng, J Y
Yu, Y J
Cheng, E J
Wang, L S
Dai, D Z
Kato, R
Li, S Y
description We present the ultralow-temperature specific heat and thermal conductivity measurements on single crystals of triangular-lattice compound EtMe3Sb[Pd(dmit)2]2, which has long been considered as a gapless quantum spin liquid candidate. In specific heat measurements, a finite linear term is observed, consistent with the previous work [S. Yamashita et al., Nat. Commun. 2, 275 (2011)]. However, we do not observe a finite residual linear term in the thermal conductivity measurements, and the thermal conductivity does not change in a magnetic field of 6 T. These results are in sharp contrast to previous thermal conductivity measurements on EtMe3Sb[Pd(dmit)2]2 [M. Yamashita et al., Science 328, 1246 (2010)], in which a huge residual linear term was observed and attributed to highly mobile gapless excitations, likely the spinons of a quantum spin liquid. In this context, the true ground state of EtMe3Sb[Pd(dmit)2]2 has to be reconsidered.
doi_str_mv 10.1103/PhysRevLett.123.247204
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In specific heat measurements, a finite linear term is observed, consistent with the previous work [S. Yamashita et al., Nat. Commun. 2, 275 (2011)]. However, we do not observe a finite residual linear term in the thermal conductivity measurements, and the thermal conductivity does not change in a magnetic field of 6 T. These results are in sharp contrast to previous thermal conductivity measurements on EtMe3Sb[Pd(dmit)2]2 [M. Yamashita et al., Science 328, 1246 (2010)], in which a huge residual linear term was observed and attributed to highly mobile gapless excitations, likely the spinons of a quantum spin liquid. 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subjects Crystal lattices
Heat conductivity
Heat transfer
Single crystals
Specific heat
Spin liquid
Thermal conductivity
title Absence of Magnetic Thermal Conductivity in the Quantum Spin Liquid Candidate EtMe3Sb[Pd(dmit)2]2
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