Absence of Magnetic Thermal Conductivity in the Quantum Spin Liquid Candidate EtMe3Sb[Pd(dmit)2]2
We present the ultralow-temperature specific heat and thermal conductivity measurements on single crystals of triangular-lattice compound EtMe3Sb[Pd(dmit)2]2, which has long been considered as a gapless quantum spin liquid candidate. In specific heat measurements, a finite linear term is observed, c...
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Veröffentlicht in: | Physical review letters 2019-12, Vol.123 (24), p.1 |
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description | We present the ultralow-temperature specific heat and thermal conductivity measurements on single crystals of triangular-lattice compound EtMe3Sb[Pd(dmit)2]2, which has long been considered as a gapless quantum spin liquid candidate. In specific heat measurements, a finite linear term is observed, consistent with the previous work [S. Yamashita et al., Nat. Commun. 2, 275 (2011)]. However, we do not observe a finite residual linear term in the thermal conductivity measurements, and the thermal conductivity does not change in a magnetic field of 6 T. These results are in sharp contrast to previous thermal conductivity measurements on EtMe3Sb[Pd(dmit)2]2 [M. Yamashita et al., Science 328, 1246 (2010)], in which a huge residual linear term was observed and attributed to highly mobile gapless excitations, likely the spinons of a quantum spin liquid. In this context, the true ground state of EtMe3Sb[Pd(dmit)2]2 has to be reconsidered. |
doi_str_mv | 10.1103/PhysRevLett.123.247204 |
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In specific heat measurements, a finite linear term is observed, consistent with the previous work [S. Yamashita et al., Nat. Commun. 2, 275 (2011)]. However, we do not observe a finite residual linear term in the thermal conductivity measurements, and the thermal conductivity does not change in a magnetic field of 6 T. These results are in sharp contrast to previous thermal conductivity measurements on EtMe3Sb[Pd(dmit)2]2 [M. Yamashita et al., Science 328, 1246 (2010)], in which a huge residual linear term was observed and attributed to highly mobile gapless excitations, likely the spinons of a quantum spin liquid. In this context, the true ground state of EtMe3Sb[Pd(dmit)2]2 has to be reconsidered.</description><identifier>ISSN: 0031-9007</identifier><identifier>EISSN: 1079-7114</identifier><identifier>DOI: 10.1103/PhysRevLett.123.247204</identifier><language>eng</language><publisher>College Park: American Physical Society</publisher><subject>Crystal lattices ; Heat conductivity ; Heat transfer ; Single crystals ; Specific heat ; Spin liquid ; Thermal conductivity</subject><ispartof>Physical review letters, 2019-12, Vol.123 (24), p.1</ispartof><rights>Copyright American Physical Society Dec 13, 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids></links><search><creatorcontrib>Ni, J M</creatorcontrib><creatorcontrib>Pan, B L</creatorcontrib><creatorcontrib>Song, B Q</creatorcontrib><creatorcontrib>Huang, Y Y</creatorcontrib><creatorcontrib>Zeng, J Y</creatorcontrib><creatorcontrib>Yu, Y J</creatorcontrib><creatorcontrib>Cheng, E J</creatorcontrib><creatorcontrib>Wang, L S</creatorcontrib><creatorcontrib>Dai, D Z</creatorcontrib><creatorcontrib>Kato, R</creatorcontrib><creatorcontrib>Li, S Y</creatorcontrib><title>Absence of Magnetic Thermal Conductivity in the Quantum Spin Liquid Candidate EtMe3Sb[Pd(dmit)2]2</title><title>Physical review letters</title><description>We present the ultralow-temperature specific heat and thermal conductivity measurements on single crystals of triangular-lattice compound EtMe3Sb[Pd(dmit)2]2, which has long been considered as a gapless quantum spin liquid candidate. In specific heat measurements, a finite linear term is observed, consistent with the previous work [S. Yamashita et al., Nat. Commun. 2, 275 (2011)]. However, we do not observe a finite residual linear term in the thermal conductivity measurements, and the thermal conductivity does not change in a magnetic field of 6 T. These results are in sharp contrast to previous thermal conductivity measurements on EtMe3Sb[Pd(dmit)2]2 [M. Yamashita et al., Science 328, 1246 (2010)], in which a huge residual linear term was observed and attributed to highly mobile gapless excitations, likely the spinons of a quantum spin liquid. In this context, the true ground state of EtMe3Sb[Pd(dmit)2]2 has to be reconsidered.</description><subject>Crystal lattices</subject><subject>Heat conductivity</subject><subject>Heat transfer</subject><subject>Single crystals</subject><subject>Specific heat</subject><subject>Spin liquid</subject><subject>Thermal conductivity</subject><issn>0031-9007</issn><issn>1079-7114</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNotjU1Lw0AUABdRsFb_gix40UPqe2-T7uZYQv2AFKutJ5Gyyb7YLW3SNptC_70FPQ3MYUaIW4QBIqjH6fLYfvAh5xAGSGpAsSaIz0QPQaeRRozPRQ9AYZQC6Etx1bYrAEAamp6wo6LlumTZVHJif2oOvpTzJe83di2zpnZdGfzBh6P0tQxLlu-drUO3kbPtSeR-13knM1s772xgOQ4TVrPia-ru3caHB_qma3FR2XXLN__si8-n8Tx7ifK359dslEdbNCpEZNFQbAuqiA2lRlVQFdoZg6lOMWFWiU6GCVChQbGKyzTF2ClCSqqSC1B9cffX3e6bXcdtWKyabl-flgtSpE0KSYLqF4sOWAg</recordid><startdate>20191210</startdate><enddate>20191210</enddate><creator>Ni, J M</creator><creator>Pan, B L</creator><creator>Song, B Q</creator><creator>Huang, Y Y</creator><creator>Zeng, J Y</creator><creator>Yu, Y J</creator><creator>Cheng, E J</creator><creator>Wang, L S</creator><creator>Dai, D Z</creator><creator>Kato, R</creator><creator>Li, S Y</creator><general>American Physical Society</general><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>20191210</creationdate><title>Absence of Magnetic Thermal Conductivity in the Quantum Spin Liquid Candidate EtMe3Sb[Pd(dmit)2]2</title><author>Ni, J M ; Pan, B L ; Song, B Q ; Huang, Y Y ; Zeng, J Y ; Yu, Y J ; Cheng, E J ; Wang, L S ; Dai, D Z ; Kato, R ; Li, S Y</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-p183t-2a1824ab2f2e82983f0fb7d88197915ee35756502b703e34c9914d32125fceb03</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Crystal lattices</topic><topic>Heat conductivity</topic><topic>Heat transfer</topic><topic>Single crystals</topic><topic>Specific heat</topic><topic>Spin liquid</topic><topic>Thermal conductivity</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ni, J M</creatorcontrib><creatorcontrib>Pan, B L</creatorcontrib><creatorcontrib>Song, B Q</creatorcontrib><creatorcontrib>Huang, Y Y</creatorcontrib><creatorcontrib>Zeng, J Y</creatorcontrib><creatorcontrib>Yu, Y J</creatorcontrib><creatorcontrib>Cheng, E J</creatorcontrib><creatorcontrib>Wang, L S</creatorcontrib><creatorcontrib>Dai, D Z</creatorcontrib><creatorcontrib>Kato, R</creatorcontrib><creatorcontrib>Li, S Y</creatorcontrib><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Physical review letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ni, J M</au><au>Pan, B L</au><au>Song, B Q</au><au>Huang, Y Y</au><au>Zeng, J Y</au><au>Yu, Y J</au><au>Cheng, E J</au><au>Wang, L S</au><au>Dai, D Z</au><au>Kato, R</au><au>Li, S Y</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Absence of Magnetic Thermal Conductivity in the Quantum Spin Liquid Candidate EtMe3Sb[Pd(dmit)2]2</atitle><jtitle>Physical review letters</jtitle><date>2019-12-10</date><risdate>2019</risdate><volume>123</volume><issue>24</issue><spage>1</spage><pages>1-</pages><issn>0031-9007</issn><eissn>1079-7114</eissn><abstract>We present the ultralow-temperature specific heat and thermal conductivity measurements on single crystals of triangular-lattice compound EtMe3Sb[Pd(dmit)2]2, which has long been considered as a gapless quantum spin liquid candidate. In specific heat measurements, a finite linear term is observed, consistent with the previous work [S. Yamashita et al., Nat. Commun. 2, 275 (2011)]. However, we do not observe a finite residual linear term in the thermal conductivity measurements, and the thermal conductivity does not change in a magnetic field of 6 T. These results are in sharp contrast to previous thermal conductivity measurements on EtMe3Sb[Pd(dmit)2]2 [M. Yamashita et al., Science 328, 1246 (2010)], in which a huge residual linear term was observed and attributed to highly mobile gapless excitations, likely the spinons of a quantum spin liquid. In this context, the true ground state of EtMe3Sb[Pd(dmit)2]2 has to be reconsidered.</abstract><cop>College Park</cop><pub>American Physical Society</pub><doi>10.1103/PhysRevLett.123.247204</doi></addata></record> |
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subjects | Crystal lattices Heat conductivity Heat transfer Single crystals Specific heat Spin liquid Thermal conductivity |
title | Absence of Magnetic Thermal Conductivity in the Quantum Spin Liquid Candidate EtMe3Sb[Pd(dmit)2]2 |
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