Evaluating uranium radiochronometry by single-collector mass spectrometry for nuclear forensics: a multi-instrument investigation
Radiochronometric data, a key signature in evaluating the provenance and process history of nuclear material out of regulatory control, are conventionally acquired via multi-collector mass spectrometry. Here we explore the potential of age-dating by single-collector mass spectrometry. To evaluate mo...
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| Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2019-12, Vol.322 (3), p.1627-1640 |
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| container_title | Journal of radioanalytical and nuclear chemistry |
| container_volume | 322 |
| creator | Treinen, Kerri C. Samperton, Kyle M. Lindvall, Rachel E. Wimpenny, Josh B. Gaffney, Amy M. Bavio, Marta Baransky, Eva J. Williams, Ross W. |
| description | Radiochronometric data, a key signature in evaluating the provenance and process history of nuclear material out of regulatory control, are conventionally acquired via multi-collector mass spectrometry. Here we explore the potential of age-dating by single-collector mass spectrometry. To evaluate model age accuracy/precision across different instrument designs, we performed
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Th–
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U and
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Pa–
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U radiochronometry of CRM 125-A using two single-collector and one multi-collector plasma source mass spectrometers. Single-collector instruments produce accurate model ages for this uranium standard and thus hold promise for nuclear forensics radiochronometry. Increased acquisition of age information via multiple instrument designs will bolster the global response to nuclear interdictions. |
| doi_str_mv | 10.1007/s10967-019-06832-y |
| format | Article |
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230
Th–
234
U and
231
Pa–
235
U radiochronometry of CRM 125-A using two single-collector and one multi-collector plasma source mass spectrometers. Single-collector instruments produce accurate model ages for this uranium standard and thus hold promise for nuclear forensics radiochronometry. Increased acquisition of age information via multiple instrument designs will bolster the global response to nuclear interdictions.</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-019-06832-y</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Age ; Chemistry ; Chemistry and Materials Science ; Customer relationship management software ; Diagnostic Radiology ; Forensic sciences ; Hadrons ; Heavy Ions ; Inorganic Chemistry ; Ions ; Mass spectrometers ; Mass spectrometry ; Model accuracy ; Nuclear Chemistry ; Nuclear Physics ; Physical Chemistry ; Plasma physics ; Scientific imaging ; Spectrometers ; Spectroscopy ; Spectrum analysis ; Uranium</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2019-12, Vol.322 (3), p.1627-1640</ispartof><rights>Akadémiai Kiadó, Budapest, Hungary 2019</rights><rights>COPYRIGHT 2019 Springer</rights><rights>Copyright Springer Nature B.V. 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c358t-74b227f91ca6a512a35197add0244e208465f88e711bbc828206ffe5e774b53d3</citedby><cites>FETCH-LOGICAL-c358t-74b227f91ca6a512a35197add0244e208465f88e711bbc828206ffe5e774b53d3</cites><orcidid>0000-0003-0177-5978 ; 0000-0003-0645-6810</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10967-019-06832-y$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10967-019-06832-y$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,777,781,27905,27906,41469,42538,51300</link.rule.ids></links><search><creatorcontrib>Treinen, Kerri C.</creatorcontrib><creatorcontrib>Samperton, Kyle M.</creatorcontrib><creatorcontrib>Lindvall, Rachel E.</creatorcontrib><creatorcontrib>Wimpenny, Josh B.</creatorcontrib><creatorcontrib>Gaffney, Amy M.</creatorcontrib><creatorcontrib>Bavio, Marta</creatorcontrib><creatorcontrib>Baransky, Eva J.</creatorcontrib><creatorcontrib>Williams, Ross W.</creatorcontrib><title>Evaluating uranium radiochronometry by single-collector mass spectrometry for nuclear forensics: a multi-instrument investigation</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>Radiochronometric data, a key signature in evaluating the provenance and process history of nuclear material out of regulatory control, are conventionally acquired via multi-collector mass spectrometry. Here we explore the potential of age-dating by single-collector mass spectrometry. To evaluate model age accuracy/precision across different instrument designs, we performed
230
Th–
234
U and
231
Pa–
235
U radiochronometry of CRM 125-A using two single-collector and one multi-collector plasma source mass spectrometers. Single-collector instruments produce accurate model ages for this uranium standard and thus hold promise for nuclear forensics radiochronometry. 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230
Th–
234
U and
231
Pa–
235
U radiochronometry of CRM 125-A using two single-collector and one multi-collector plasma source mass spectrometers. Single-collector instruments produce accurate model ages for this uranium standard and thus hold promise for nuclear forensics radiochronometry. Increased acquisition of age information via multiple instrument designs will bolster the global response to nuclear interdictions.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s10967-019-06832-y</doi><tpages>14</tpages><orcidid>https://orcid.org/0000-0003-0177-5978</orcidid><orcidid>https://orcid.org/0000-0003-0645-6810</orcidid></addata></record> |
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| subjects | Age Chemistry Chemistry and Materials Science Customer relationship management software Diagnostic Radiology Forensic sciences Hadrons Heavy Ions Inorganic Chemistry Ions Mass spectrometers Mass spectrometry Model accuracy Nuclear Chemistry Nuclear Physics Physical Chemistry Plasma physics Scientific imaging Spectrometers Spectroscopy Spectrum analysis Uranium |
| title | Evaluating uranium radiochronometry by single-collector mass spectrometry for nuclear forensics: a multi-instrument investigation |
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