UV-cured gel polymer electrolytes with improved stability for advanced aqueous Li-ion batteries
We report the development of a new class of "water-in-salt" electrolytes based on UV photopolymerized acrylic polymers. Incorporation of "water-in-bisalt" in a polymer matrix reduces water activity, expands the electrochemical stability window to 4.1 V, and dramatically improves...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2019-10, Vol.55 (87), p.1385-1388 |
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| container_title | Chemical communications (Cambridge, England) |
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| creator | Langevin, Spencer A Tan, Bing Freeman, Adam W Gagnon, Jarod C Hoffman, Christopher M Logan, Matthew W Maranchi, Jeffrey P Gerasopoulos, Konstantinos |
| description | We report the development of a new class of "water-in-salt" electrolytes based on UV photopolymerized acrylic polymers. Incorporation of "water-in-bisalt" in a polymer matrix reduces water activity, expands the electrochemical stability window to 4.1 V, and dramatically improves cycle life in full cells with lithium titanate anodes compared to liquid water-based electrolytes.
We report UV-photopolymerized "water-in-bisalt" electrolytes that expand the electrochemical stability window, improving "water-in-bisalt" cycle life in lithium titanate full cells. |
| doi_str_mv | 10.1039/c9cc06207f |
| format | Article |
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We report UV-photopolymerized "water-in-bisalt" electrolytes that expand the electrochemical stability window, improving "water-in-bisalt" cycle life in lithium titanate full cells.</description><subject>Electrolytes</subject><subject>Electrolytic cells</subject><subject>Flammability</subject><subject>Lithium-ion batteries</subject><subject>Rechargeable batteries</subject><subject>Stability</subject><subject>Water</subject><subject>Water activity</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNpd0ctLwzAABvAgCs7pxbsQ8CJCNc-2OUpxKgy8OPFW8qpG-phJOtl_b-pEwVzy4Efy8QWAU4yuMKLiWgutUU5Q0eyBGaY5yzgrX_anNRdZQRk_BEchvKM0MC9noF49Z3r01sBX28L10G4766FtrY4-baIN8NPFN-i6tR82iYUolWtd3MJm8FCajex1OpYfox3GAJcuc0MPlYzRemfDMThoZBvsyc88B6vF7VN1ny0f7x6qm2WmKWYxI0hLRYXJDZICE6pyRguiCkoIZkQiZKnUzApFGo5LjozUBceGSGwYVlTTObjY3Ztipigh1p0L2rat7KdcNaGIsyJPjyV6_o--D6PvU7pJCYHK1GRSlzul_RCCt0299q6TfltjVE9d15Woqu-uFwmf7bAP-tf9_QX9AoS5ez4</recordid><startdate>20191029</startdate><enddate>20191029</enddate><creator>Langevin, Spencer A</creator><creator>Tan, Bing</creator><creator>Freeman, Adam W</creator><creator>Gagnon, Jarod C</creator><creator>Hoffman, Christopher M</creator><creator>Logan, Matthew W</creator><creator>Maranchi, Jeffrey P</creator><creator>Gerasopoulos, Konstantinos</creator><general>Royal Society of Chemistry</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0003-2259-4703</orcidid></search><sort><creationdate>20191029</creationdate><title>UV-cured gel polymer electrolytes with improved stability for advanced aqueous Li-ion batteries</title><author>Langevin, Spencer A ; Tan, Bing ; Freeman, Adam W ; Gagnon, Jarod C ; Hoffman, Christopher M ; Logan, Matthew W ; Maranchi, Jeffrey P ; Gerasopoulos, Konstantinos</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c314t-20cab39d6d0a9123b64372b7322142a00e3ac4e9b2f51850dac751d2a1d41b3c3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Electrolytes</topic><topic>Electrolytic cells</topic><topic>Flammability</topic><topic>Lithium-ion batteries</topic><topic>Rechargeable batteries</topic><topic>Stability</topic><topic>Water</topic><topic>Water activity</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Langevin, Spencer A</creatorcontrib><creatorcontrib>Tan, Bing</creatorcontrib><creatorcontrib>Freeman, Adam W</creatorcontrib><creatorcontrib>Gagnon, Jarod C</creatorcontrib><creatorcontrib>Hoffman, Christopher M</creatorcontrib><creatorcontrib>Logan, Matthew W</creatorcontrib><creatorcontrib>Maranchi, Jeffrey P</creatorcontrib><creatorcontrib>Gerasopoulos, Konstantinos</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Langevin, Spencer A</au><au>Tan, Bing</au><au>Freeman, Adam W</au><au>Gagnon, Jarod C</au><au>Hoffman, Christopher M</au><au>Logan, Matthew W</au><au>Maranchi, Jeffrey P</au><au>Gerasopoulos, Konstantinos</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>UV-cured gel polymer electrolytes with improved stability for advanced aqueous Li-ion batteries</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><date>2019-10-29</date><risdate>2019</risdate><volume>55</volume><issue>87</issue><spage>1385</spage><epage>1388</epage><pages>1385-1388</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>We report the development of a new class of "water-in-salt" electrolytes based on UV photopolymerized acrylic polymers. Incorporation of "water-in-bisalt" in a polymer matrix reduces water activity, expands the electrochemical stability window to 4.1 V, and dramatically improves cycle life in full cells with lithium titanate anodes compared to liquid water-based electrolytes.
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| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2019-10, Vol.55 (87), p.1385-1388 |
| issn | 1359-7345 1364-548X |
| language | eng |
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| source | Royal Society Of Chemistry Journals; Alma/SFX Local Collection |
| subjects | Electrolytes Electrolytic cells Flammability Lithium-ion batteries Rechargeable batteries Stability Water Water activity |
| title | UV-cured gel polymer electrolytes with improved stability for advanced aqueous Li-ion batteries |
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