Magnon Pairs and Spin-Nematic Correlation in the Spin Seebeck Effect
Investigating exotic magnetic materials with spintronic techniques is effective at advancing magnetism as well as spintronics. In this work, we report unusual field-induced suppression of the spin Seebeck effect (SSE) in a quasi-one-dimensional frustrated spin-12 magnet LiCuVO4, known to exhibit spi...
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Veröffentlicht in: | Physical review letters 2019-09, Vol.123 (11), p.1, Article 117202 |
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creator | Hirobe, Daichi Sato, Masahiro Hagihala, Masato Shiomi, Yuki Masuda, Takatsugu Saitoh, Eiji |
description | Investigating exotic magnetic materials with spintronic techniques is effective at advancing magnetism as well as spintronics. In this work, we report unusual field-induced suppression of the spin Seebeck effect (SSE) in a quasi-one-dimensional frustrated spin-12 magnet LiCuVO4, known to exhibit spin-nematic correlation in a wide range of external magnetic field B. The suppression takes place above |B|≳2 T in spite of the B-linear isothermal magnetization curves in the same B range. The result can be attributed to the growth of the spin-nematic correlation while increasing B. The correlation stabilizes magnon pairs carrying spin 2, thereby suppressing the interfacial spin injection of SSE by preventing the spin-1 exchange between single magnons and conduction electrons at the interface. This interpretation is supported by integrating thermodynamic measurements and theoretical analysis on the SSE. |
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In this work, we report unusual field-induced suppression of the spin Seebeck effect (SSE) in a quasi-one-dimensional frustrated spin-12 magnet LiCuVO4, known to exhibit spin-nematic correlation in a wide range of external magnetic field B. The suppression takes place above |B|≳2 T in spite of the B-linear isothermal magnetization curves in the same B range. The result can be attributed to the growth of the spin-nematic correlation while increasing B. The correlation stabilizes magnon pairs carrying spin 2, thereby suppressing the interfacial spin injection of SSE by preventing the spin-1 exchange between single magnons and conduction electrons at the interface. This interpretation is supported by integrating thermodynamic measurements and theoretical analysis on the SSE.</description><identifier>ISSN: 0031-9007</identifier><identifier>EISSN: 1079-7114</identifier><identifier>DOI: 10.1103/PhysRevLett.123.117202</identifier><language>eng</language><publisher>College Park: American Physical Society</publisher><subject>Conduction electrons ; Correlation ; Magnetic materials ; Magnetism ; Magnetization curves ; Magnons ; Seebeck effect ; Spintronics</subject><ispartof>Physical review letters, 2019-09, Vol.123 (11), p.1, Article 117202</ispartof><rights>Copyright American Physical Society Sep 13, 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c283t-7d73d9226c448505fe067917720fff21bf2e4a21d31838da77e340f49534e3573</citedby><cites>FETCH-LOGICAL-c283t-7d73d9226c448505fe067917720fff21bf2e4a21d31838da77e340f49534e3573</cites><orcidid>0000-0002-1469-8847</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,2876,2877,27924,27925</link.rule.ids></links><search><creatorcontrib>Hirobe, Daichi</creatorcontrib><creatorcontrib>Sato, Masahiro</creatorcontrib><creatorcontrib>Hagihala, Masato</creatorcontrib><creatorcontrib>Shiomi, Yuki</creatorcontrib><creatorcontrib>Masuda, Takatsugu</creatorcontrib><creatorcontrib>Saitoh, Eiji</creatorcontrib><title>Magnon Pairs and Spin-Nematic Correlation in the Spin Seebeck Effect</title><title>Physical review letters</title><description>Investigating exotic magnetic materials with spintronic techniques is effective at advancing magnetism as well as spintronics. In this work, we report unusual field-induced suppression of the spin Seebeck effect (SSE) in a quasi-one-dimensional frustrated spin-12 magnet LiCuVO4, known to exhibit spin-nematic correlation in a wide range of external magnetic field B. The suppression takes place above |B|≳2 T in spite of the B-linear isothermal magnetization curves in the same B range. The result can be attributed to the growth of the spin-nematic correlation while increasing B. The correlation stabilizes magnon pairs carrying spin 2, thereby suppressing the interfacial spin injection of SSE by preventing the spin-1 exchange between single magnons and conduction electrons at the interface. This interpretation is supported by integrating thermodynamic measurements and theoretical analysis on the SSE.</description><subject>Conduction electrons</subject><subject>Correlation</subject><subject>Magnetic materials</subject><subject>Magnetism</subject><subject>Magnetization curves</subject><subject>Magnons</subject><subject>Seebeck effect</subject><subject>Spintronics</subject><issn>0031-9007</issn><issn>1079-7114</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNpNkE1PwzAMhiMEEmPwF1AkzgU7aZvmiMb4kAZMDM5R1jqsY2tHkiHt3xMYB062_D6yrYexc4RLRJBX08UuvNDXhGK8RCHTUAkQB2yAoHSmEPNDNgCQmGkAdcxOQlgCAIqyGrCbR_ve9R2f2tYHbruGzzZtlz3R2sa25qPee1qlNiFtx-OCfnM-I5pT_cHHzlEdT9mRs6tAZ391yN5ux6-j-2zyfPcwup5ktahkzFSjZKOFKOs8rwooHEGpNKr0rnNO4NwJyq3ARmIlq8YqRTIHl-tC5iQLJYfsYr934_vPLYVolv3Wd-mkEUJrVZSoIVHlnqp9H4InZza-XVu_Mwjmx5j5Z8wkY2ZvTH4D_ZBfqA</recordid><startdate>20190912</startdate><enddate>20190912</enddate><creator>Hirobe, Daichi</creator><creator>Sato, Masahiro</creator><creator>Hagihala, Masato</creator><creator>Shiomi, Yuki</creator><creator>Masuda, Takatsugu</creator><creator>Saitoh, Eiji</creator><general>American Physical Society</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0002-1469-8847</orcidid></search><sort><creationdate>20190912</creationdate><title>Magnon Pairs and Spin-Nematic Correlation in the Spin Seebeck Effect</title><author>Hirobe, Daichi ; Sato, Masahiro ; Hagihala, Masato ; Shiomi, Yuki ; Masuda, Takatsugu ; Saitoh, Eiji</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c283t-7d73d9226c448505fe067917720fff21bf2e4a21d31838da77e340f49534e3573</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Conduction electrons</topic><topic>Correlation</topic><topic>Magnetic materials</topic><topic>Magnetism</topic><topic>Magnetization curves</topic><topic>Magnons</topic><topic>Seebeck effect</topic><topic>Spintronics</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Hirobe, Daichi</creatorcontrib><creatorcontrib>Sato, Masahiro</creatorcontrib><creatorcontrib>Hagihala, Masato</creatorcontrib><creatorcontrib>Shiomi, Yuki</creatorcontrib><creatorcontrib>Masuda, Takatsugu</creatorcontrib><creatorcontrib>Saitoh, Eiji</creatorcontrib><collection>CrossRef</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Physical review letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Hirobe, Daichi</au><au>Sato, Masahiro</au><au>Hagihala, Masato</au><au>Shiomi, Yuki</au><au>Masuda, Takatsugu</au><au>Saitoh, Eiji</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Magnon Pairs and Spin-Nematic Correlation in the Spin Seebeck Effect</atitle><jtitle>Physical review letters</jtitle><date>2019-09-12</date><risdate>2019</risdate><volume>123</volume><issue>11</issue><spage>1</spage><pages>1-</pages><artnum>117202</artnum><issn>0031-9007</issn><eissn>1079-7114</eissn><abstract>Investigating exotic magnetic materials with spintronic techniques is effective at advancing magnetism as well as spintronics. In this work, we report unusual field-induced suppression of the spin Seebeck effect (SSE) in a quasi-one-dimensional frustrated spin-12 magnet LiCuVO4, known to exhibit spin-nematic correlation in a wide range of external magnetic field B. The suppression takes place above |B|≳2 T in spite of the B-linear isothermal magnetization curves in the same B range. The result can be attributed to the growth of the spin-nematic correlation while increasing B. The correlation stabilizes magnon pairs carrying spin 2, thereby suppressing the interfacial spin injection of SSE by preventing the spin-1 exchange between single magnons and conduction electrons at the interface. This interpretation is supported by integrating thermodynamic measurements and theoretical analysis on the SSE.</abstract><cop>College Park</cop><pub>American Physical Society</pub><doi>10.1103/PhysRevLett.123.117202</doi><orcidid>https://orcid.org/0000-0002-1469-8847</orcidid></addata></record> |
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subjects | Conduction electrons Correlation Magnetic materials Magnetism Magnetization curves Magnons Seebeck effect Spintronics |
title | Magnon Pairs and Spin-Nematic Correlation in the Spin Seebeck Effect |
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