In-situ synthesis of organic-inorganic hybrid thin film of PEDOT/V2O5 as hole transport layer for polymer solar cells
•Hybrid film of PEDOT/V2O5 was obtained via an in-situ synthesis method.•A higher PCE of 3.76% is achieved using PEDOT/V2O5, which increased by 8% than that of the regular PEDOT:PSS device.•Devices with PEDOT/V2O5 show better stability. Here, an organic-inorganic hybrid thin film of PEDOT/V2O5 compl...
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| Veröffentlicht in: | Solar energy 2019-09, Vol.190, p.63-68 |
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| creator | Ling, Hanbing Zhang, Rui Ye, Xiaoqin Wen, Zhiyue Xia, Jiangbin Lu, Xing |
| description | •Hybrid film of PEDOT/V2O5 was obtained via an in-situ synthesis method.•A higher PCE of 3.76% is achieved using PEDOT/V2O5, which increased by 8% than that of the regular PEDOT:PSS device.•Devices with PEDOT/V2O5 show better stability.
Here, an organic-inorganic hybrid thin film of PEDOT/V2O5 complex was successfully obtained via an in-situ synthesis method. In detail, PEDOT buffer layer was prepared by in-situ oxidative polymerization. Then, a layer of V2O5 nanoparticles was deposited on it. V2O5 nanoparticles can closely combine with PEDOT and modifying the surface defects of PEDOT. For the control polymer solar cells (PSCs) with a PEDOT:PSS hole transport layer (HTL), a power conversion efficiency (PCE) of 3.50% is obtained. Encouragingly, a higher PCE of 3.76% is achieved for the cell using the as-prepared PEDOT/V2O5 as the HTL, which increased by 8% than that of the control device. Furthermore, the devices with PEDOT/V2O5 show a better stability than the control devices using PEDOT:PSS as HTL. The results indicate that PEDOT/V2O5 is an excellent HTL for efficient and stable PSCs. |
| doi_str_mv | 10.1016/j.solener.2019.07.095 |
| format | Article |
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Here, an organic-inorganic hybrid thin film of PEDOT/V2O5 complex was successfully obtained via an in-situ synthesis method. In detail, PEDOT buffer layer was prepared by in-situ oxidative polymerization. Then, a layer of V2O5 nanoparticles was deposited on it. V2O5 nanoparticles can closely combine with PEDOT and modifying the surface defects of PEDOT. For the control polymer solar cells (PSCs) with a PEDOT:PSS hole transport layer (HTL), a power conversion efficiency (PCE) of 3.50% is obtained. Encouragingly, a higher PCE of 3.76% is achieved for the cell using the as-prepared PEDOT/V2O5 as the HTL, which increased by 8% than that of the control device. Furthermore, the devices with PEDOT/V2O5 show a better stability than the control devices using PEDOT:PSS as HTL. The results indicate that PEDOT/V2O5 is an excellent HTL for efficient and stable PSCs.</description><identifier>ISSN: 0038-092X</identifier><identifier>EISSN: 1471-1257</identifier><identifier>DOI: 10.1016/j.solener.2019.07.095</identifier><language>eng</language><publisher>New York: Elsevier Ltd</publisher><subject>Buffer layers ; Control stability ; Energy conversion efficiency ; Hole transport layer ; In-situ synthesis ; Nanoparticles ; PEDOT/V2O5 ; Photovoltaic cells ; Polymer solar cell ; Polymerization ; Polymers ; Solar cells ; Solar energy ; Surface defects ; Synthesis ; Thin films ; Transport ; Vanadium pentoxide</subject><ispartof>Solar energy, 2019-09, Vol.190, p.63-68</ispartof><rights>2019 International Solar Energy Society</rights><rights>Copyright Pergamon Press Inc. Sep 15, 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c376t-f3aaad02875593765c3d97adc1016cefcf0c6a4efd21d53ded0536fd7d3de8ac3</citedby><cites>FETCH-LOGICAL-c376t-f3aaad02875593765c3d97adc1016cefcf0c6a4efd21d53ded0536fd7d3de8ac3</cites><orcidid>0000-0001-6238-4992</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0038092X19307674$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3536,27903,27904,65309</link.rule.ids></links><search><creatorcontrib>Ling, Hanbing</creatorcontrib><creatorcontrib>Zhang, Rui</creatorcontrib><creatorcontrib>Ye, Xiaoqin</creatorcontrib><creatorcontrib>Wen, Zhiyue</creatorcontrib><creatorcontrib>Xia, Jiangbin</creatorcontrib><creatorcontrib>Lu, Xing</creatorcontrib><title>In-situ synthesis of organic-inorganic hybrid thin film of PEDOT/V2O5 as hole transport layer for polymer solar cells</title><title>Solar energy</title><description>•Hybrid film of PEDOT/V2O5 was obtained via an in-situ synthesis method.•A higher PCE of 3.76% is achieved using PEDOT/V2O5, which increased by 8% than that of the regular PEDOT:PSS device.•Devices with PEDOT/V2O5 show better stability.
Here, an organic-inorganic hybrid thin film of PEDOT/V2O5 complex was successfully obtained via an in-situ synthesis method. In detail, PEDOT buffer layer was prepared by in-situ oxidative polymerization. Then, a layer of V2O5 nanoparticles was deposited on it. V2O5 nanoparticles can closely combine with PEDOT and modifying the surface defects of PEDOT. For the control polymer solar cells (PSCs) with a PEDOT:PSS hole transport layer (HTL), a power conversion efficiency (PCE) of 3.50% is obtained. Encouragingly, a higher PCE of 3.76% is achieved for the cell using the as-prepared PEDOT/V2O5 as the HTL, which increased by 8% than that of the control device. Furthermore, the devices with PEDOT/V2O5 show a better stability than the control devices using PEDOT:PSS as HTL. The results indicate that PEDOT/V2O5 is an excellent HTL for efficient and stable PSCs.</description><subject>Buffer layers</subject><subject>Control stability</subject><subject>Energy conversion efficiency</subject><subject>Hole transport layer</subject><subject>In-situ synthesis</subject><subject>Nanoparticles</subject><subject>PEDOT/V2O5</subject><subject>Photovoltaic cells</subject><subject>Polymer solar cell</subject><subject>Polymerization</subject><subject>Polymers</subject><subject>Solar cells</subject><subject>Solar energy</subject><subject>Surface defects</subject><subject>Synthesis</subject><subject>Thin films</subject><subject>Transport</subject><subject>Vanadium pentoxide</subject><issn>0038-092X</issn><issn>1471-1257</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNqFUMtOwzAQtBBIlMInIFninNR26jg5IVRelSqVQ0HcLOMHcZTawU6R8vc4au-cdrQ7uzM7ANxilGOEy0WbR99pp0NOEK5zxHJU0zMww0uGM0woOwczhIoqQzX5vARXMbYIYYYrNgOHtcuiHQ4wjm5odLQRegN9-BbOysy6E4LN-BWsgkNjHTS220-st6fH7W7xQbYUigib5AEOQbjY-zDATow6QOMD7H037hNOJkWAUnddvAYXRnRR35zqHLw_P-1Wr9lm-7JePWwyWbByyEwhhFCIVIzSOnWoLFTNhJLT21IbaZAsxVIbRbCihdIK0aI0iqmEKyGLObg73u2D_znoOPDWH4JLkpyQumIlYcs6seiRJYOPMWjD-2D3IowcIz5J8ZafEuZTwhwxnhJOe_fHPZ1e-LVpGqXVTmplg5YDV97-c-EPjO-Jgw</recordid><startdate>20190915</startdate><enddate>20190915</enddate><creator>Ling, Hanbing</creator><creator>Zhang, Rui</creator><creator>Ye, Xiaoqin</creator><creator>Wen, Zhiyue</creator><creator>Xia, Jiangbin</creator><creator>Lu, Xing</creator><general>Elsevier Ltd</general><general>Pergamon Press Inc</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7ST</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>KR7</scope><scope>L7M</scope><scope>SOI</scope><orcidid>https://orcid.org/0000-0001-6238-4992</orcidid></search><sort><creationdate>20190915</creationdate><title>In-situ synthesis of organic-inorganic hybrid thin film of PEDOT/V2O5 as hole transport layer for polymer solar cells</title><author>Ling, Hanbing ; Zhang, Rui ; Ye, Xiaoqin ; Wen, Zhiyue ; Xia, Jiangbin ; Lu, Xing</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c376t-f3aaad02875593765c3d97adc1016cefcf0c6a4efd21d53ded0536fd7d3de8ac3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Buffer layers</topic><topic>Control stability</topic><topic>Energy conversion efficiency</topic><topic>Hole transport layer</topic><topic>In-situ synthesis</topic><topic>Nanoparticles</topic><topic>PEDOT/V2O5</topic><topic>Photovoltaic cells</topic><topic>Polymer solar cell</topic><topic>Polymerization</topic><topic>Polymers</topic><topic>Solar cells</topic><topic>Solar energy</topic><topic>Surface defects</topic><topic>Synthesis</topic><topic>Thin films</topic><topic>Transport</topic><topic>Vanadium pentoxide</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ling, Hanbing</creatorcontrib><creatorcontrib>Zhang, Rui</creatorcontrib><creatorcontrib>Ye, Xiaoqin</creatorcontrib><creatorcontrib>Wen, Zhiyue</creatorcontrib><creatorcontrib>Xia, Jiangbin</creatorcontrib><creatorcontrib>Lu, Xing</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Environment Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Civil Engineering Abstracts</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Environment Abstracts</collection><jtitle>Solar energy</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ling, Hanbing</au><au>Zhang, Rui</au><au>Ye, Xiaoqin</au><au>Wen, Zhiyue</au><au>Xia, Jiangbin</au><au>Lu, Xing</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>In-situ synthesis of organic-inorganic hybrid thin film of PEDOT/V2O5 as hole transport layer for polymer solar cells</atitle><jtitle>Solar energy</jtitle><date>2019-09-15</date><risdate>2019</risdate><volume>190</volume><spage>63</spage><epage>68</epage><pages>63-68</pages><issn>0038-092X</issn><eissn>1471-1257</eissn><abstract>•Hybrid film of PEDOT/V2O5 was obtained via an in-situ synthesis method.•A higher PCE of 3.76% is achieved using PEDOT/V2O5, which increased by 8% than that of the regular PEDOT:PSS device.•Devices with PEDOT/V2O5 show better stability.
Here, an organic-inorganic hybrid thin film of PEDOT/V2O5 complex was successfully obtained via an in-situ synthesis method. In detail, PEDOT buffer layer was prepared by in-situ oxidative polymerization. Then, a layer of V2O5 nanoparticles was deposited on it. V2O5 nanoparticles can closely combine with PEDOT and modifying the surface defects of PEDOT. For the control polymer solar cells (PSCs) with a PEDOT:PSS hole transport layer (HTL), a power conversion efficiency (PCE) of 3.50% is obtained. Encouragingly, a higher PCE of 3.76% is achieved for the cell using the as-prepared PEDOT/V2O5 as the HTL, which increased by 8% than that of the control device. Furthermore, the devices with PEDOT/V2O5 show a better stability than the control devices using PEDOT:PSS as HTL. The results indicate that PEDOT/V2O5 is an excellent HTL for efficient and stable PSCs.</abstract><cop>New York</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.solener.2019.07.095</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0001-6238-4992</orcidid></addata></record> |
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| subjects | Buffer layers Control stability Energy conversion efficiency Hole transport layer In-situ synthesis Nanoparticles PEDOT/V2O5 Photovoltaic cells Polymer solar cell Polymerization Polymers Solar cells Solar energy Surface defects Synthesis Thin films Transport Vanadium pentoxide |
| title | In-situ synthesis of organic-inorganic hybrid thin film of PEDOT/V2O5 as hole transport layer for polymer solar cells |
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