Diprotic Ammonium Succinate Ionic Liquid in Thin Film Aqueous Lubrication and in Graphene Nanolubricant
An ammonium succinate protic ionic liquid (PIL) has been used as additive in water and as base lubricant for graphene dispersions in sapphire-stainless steel lubrication. The tribological performance of a water-based lubricant containing the PIL additive di[bis(2-hydroxyethyl)ammonium] succinate (DS...
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| Veröffentlicht in: | Tribology letters 2019-03, Vol.67 (1), p.1-10, Article 26 |
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| creator | Avilés, M. D. Carrión-Vilches, F. J. Sanes, J. Bermúdez, M. D. |
| description | An ammonium succinate protic ionic liquid (PIL) has been used as additive in water and as base lubricant for graphene dispersions in sapphire-stainless steel lubrication. The tribological performance of a water-based lubricant containing the PIL additive di[bis(2-hydroxyethyl)ammonium] succinate (DSu) in 1 wt% proportion (Water + DSu) has been studied. Both neat DSu and Water + DSu lubricants present a high friction coefficient during the running-in period. Elimination of the running-in high friction period has been achieved with a DSu layer generated on the steel surface by evaporation of water, before the sliding begins. This DSu surface layer reduces the wear rate in two orders of magnitude with respect to full-fluid Water + DSu and to neat DSu lubricants. The high friction running-in period can also be eliminated by the addition of 0.05 wt% few-layers graphene (G) to DSu. The new (DSu + 0.05G) nanolubricant also prevents wear and surface damage on stainless steel. Surface interactions are discussed from contact angles, SEM and TEM microscopies, XPS surface analysis, and Raman microscopy results. |
| doi_str_mv | 10.1007/s11249-019-1138-y |
| format | Article |
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D. ; Carrión-Vilches, F. J. ; Sanes, J. ; Bermúdez, M. D.</creator><creatorcontrib>Avilés, M. D. ; Carrión-Vilches, F. J. ; Sanes, J. ; Bermúdez, M. D.</creatorcontrib><description>An ammonium succinate protic ionic liquid (PIL) has been used as additive in water and as base lubricant for graphene dispersions in sapphire-stainless steel lubrication. The tribological performance of a water-based lubricant containing the PIL additive di[bis(2-hydroxyethyl)ammonium] succinate (DSu) in 1 wt% proportion (Water + DSu) has been studied. Both neat DSu and Water + DSu lubricants present a high friction coefficient during the running-in period. Elimination of the running-in high friction period has been achieved with a DSu layer generated on the steel surface by evaporation of water, before the sliding begins. This DSu surface layer reduces the wear rate in two orders of magnitude with respect to full-fluid Water + DSu and to neat DSu lubricants. The high friction running-in period can also be eliminated by the addition of 0.05 wt% few-layers graphene (G) to DSu. The new (DSu + 0.05G) nanolubricant also prevents wear and surface damage on stainless steel. Surface interactions are discussed from contact angles, SEM and TEM microscopies, XPS surface analysis, and Raman microscopy results.</description><identifier>ISSN: 1023-8883</identifier><identifier>EISSN: 1573-2711</identifier><identifier>DOI: 10.1007/s11249-019-1138-y</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Chemistry and Materials Science ; Coefficient of friction ; Contact angle ; Corrosion and Coatings ; Friction ; Graphene ; Ionic liquids ; Ions ; Linearization ; Lubricants ; Lubricants & lubrication ; Lubrication ; Materials Science ; Nanotechnology ; Original Paper ; Physical Chemistry ; Sapphire ; Stainless steel ; Stainless steels ; Surface analysis (chemical) ; Surface layers ; Surfaces and Interfaces ; Theoretical and Applied Mechanics ; Thin Films ; Tribology ; Wear rate ; X ray photoelectron spectroscopy</subject><ispartof>Tribology letters, 2019-03, Vol.67 (1), p.1-10, Article 26</ispartof><rights>Springer Science+Business Media, LLC, part of Springer Nature 2019</rights><rights>Tribology Letters is a copyright of Springer, (2019). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c316t-b233540b847fbaaa31a66553ce164ae2219889fe1f5b9a036a238afe02e285e13</citedby><cites>FETCH-LOGICAL-c316t-b233540b847fbaaa31a66553ce164ae2219889fe1f5b9a036a238afe02e285e13</cites><orcidid>0000-0002-5366-8165</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11249-019-1138-y$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11249-019-1138-y$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Avilés, M. D.</creatorcontrib><creatorcontrib>Carrión-Vilches, F. J.</creatorcontrib><creatorcontrib>Sanes, J.</creatorcontrib><creatorcontrib>Bermúdez, M. 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The high friction running-in period can also be eliminated by the addition of 0.05 wt% few-layers graphene (G) to DSu. The new (DSu + 0.05G) nanolubricant also prevents wear and surface damage on stainless steel. Surface interactions are discussed from contact angles, SEM and TEM microscopies, XPS surface analysis, and Raman microscopy results.</description><subject>Chemistry and Materials Science</subject><subject>Coefficient of friction</subject><subject>Contact angle</subject><subject>Corrosion and Coatings</subject><subject>Friction</subject><subject>Graphene</subject><subject>Ionic liquids</subject><subject>Ions</subject><subject>Linearization</subject><subject>Lubricants</subject><subject>Lubricants & lubrication</subject><subject>Lubrication</subject><subject>Materials Science</subject><subject>Nanotechnology</subject><subject>Original Paper</subject><subject>Physical Chemistry</subject><subject>Sapphire</subject><subject>Stainless steel</subject><subject>Stainless steels</subject><subject>Surface analysis (chemical)</subject><subject>Surface layers</subject><subject>Surfaces and Interfaces</subject><subject>Theoretical and Applied Mechanics</subject><subject>Thin Films</subject><subject>Tribology</subject><subject>Wear rate</subject><subject>X ray photoelectron spectroscopy</subject><issn>1023-8883</issn><issn>1573-2711</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp1UMFOwzAMjRBIjMEHcIvEORAnTZsep8HGpAoOjHOUhnTLtKZb0h7292QUiRMX27Lfe7YfQvdAH4HS4ikCsKwkFEoCwCU5XaAJiIITVgBcppoyTqSU_BrdxLijNLGkmKDNszuErncGz9q2825o8cdgjPO6t3iVGgZX7ji4L-w8Xm9TWLh9i2fHwXZDxNVQB2d07zqPtf8BLYM-bK23-E37bj_OfX-Lrhq9j_buN0_R5-JlPX8l1ftyNZ9VxHDIe1IzzkVGa5kVTa215qDzXAhuLOSZtoxBKWXZWGhEXWrKc8241I2lzDIpLPApehh101fpxtirXTcEn1YqxiRwmkkhEwpGlAldjME26hBcq8NJAVVnP9Xop0p-qrOf6pQ4bOTEhPUbG_6U_yd9A-wEeOA</recordid><startdate>20190301</startdate><enddate>20190301</enddate><creator>Avilés, M. 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D.</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>AUTh Library subscriptions: ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>ProQuest Engineering Collection</collection><collection>ProQuest Engineering Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Engineering collection</collection><jtitle>Tribology letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Avilés, M. D.</au><au>Carrión-Vilches, F. J.</au><au>Sanes, J.</au><au>Bermúdez, M. D.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Diprotic Ammonium Succinate Ionic Liquid in Thin Film Aqueous Lubrication and in Graphene Nanolubricant</atitle><jtitle>Tribology letters</jtitle><stitle>Tribol Lett</stitle><date>2019-03-01</date><risdate>2019</risdate><volume>67</volume><issue>1</issue><spage>1</spage><epage>10</epage><pages>1-10</pages><artnum>26</artnum><issn>1023-8883</issn><eissn>1573-2711</eissn><abstract>An ammonium succinate protic ionic liquid (PIL) has been used as additive in water and as base lubricant for graphene dispersions in sapphire-stainless steel lubrication. The tribological performance of a water-based lubricant containing the PIL additive di[bis(2-hydroxyethyl)ammonium] succinate (DSu) in 1 wt% proportion (Water + DSu) has been studied. Both neat DSu and Water + DSu lubricants present a high friction coefficient during the running-in period. Elimination of the running-in high friction period has been achieved with a DSu layer generated on the steel surface by evaporation of water, before the sliding begins. This DSu surface layer reduces the wear rate in two orders of magnitude with respect to full-fluid Water + DSu and to neat DSu lubricants. The high friction running-in period can also be eliminated by the addition of 0.05 wt% few-layers graphene (G) to DSu. The new (DSu + 0.05G) nanolubricant also prevents wear and surface damage on stainless steel. Surface interactions are discussed from contact angles, SEM and TEM microscopies, XPS surface analysis, and Raman microscopy results.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s11249-019-1138-y</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0002-5366-8165</orcidid></addata></record> |
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| subjects | Chemistry and Materials Science Coefficient of friction Contact angle Corrosion and Coatings Friction Graphene Ionic liquids Ions Linearization Lubricants Lubricants & lubrication Lubrication Materials Science Nanotechnology Original Paper Physical Chemistry Sapphire Stainless steel Stainless steels Surface analysis (chemical) Surface layers Surfaces and Interfaces Theoretical and Applied Mechanics Thin Films Tribology Wear rate X ray photoelectron spectroscopy |
| title | Diprotic Ammonium Succinate Ionic Liquid in Thin Film Aqueous Lubrication and in Graphene Nanolubricant |
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