Comment on “Observation of Fourier transform limited lines in hexagonal boron nitride”
Recently, emission linewidths of single defect centers in layered hexagonal boron nitride down to 50 MHz were reported, close to the lifetime limit. The linewidths were extracted from time traces of laser scanning photoluminescence excitation experiments. At the same time, temporal blinking was affe...
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Veröffentlicht in: | Physical review. B 2019-07, Vol.100 (4), p.047401, Article 047401 |
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description | Recently, emission linewidths of single defect centers in layered hexagonal boron nitride down to 50 MHz were reported, close to the lifetime limit. The linewidths were extracted from time traces of laser scanning photoluminescence excitation experiments. At the same time, temporal blinking was affecting the measured time traces even in the absence of a frequency scanning the excitation laser. I argue here that the reported temporal blinking timescale is consistent with the observed transients, implying that the interpretation as spectral shapes and thus the extracted linewidths are invalid. |
doi_str_mv | 10.1103/PhysRevB.100.047401 |
format | Article |
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The linewidths were extracted from time traces of laser scanning photoluminescence excitation experiments. At the same time, temporal blinking was affecting the measured time traces even in the absence of a frequency scanning the excitation laser. I argue here that the reported temporal blinking timescale is consistent with the observed transients, implying that the interpretation as spectral shapes and thus the extracted linewidths are invalid.</description><identifier>ISSN: 2469-9950</identifier><identifier>EISSN: 2469-9969</identifier><identifier>DOI: 10.1103/PhysRevB.100.047401</identifier><language>eng</language><publisher>College Park: American Physical Society</publisher><subject>Blinking ; Boron nitride ; Excitation ; Fourier transforms ; Frequency scanning ; Photoluminescence</subject><ispartof>Physical review. 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B</title><description>Recently, emission linewidths of single defect centers in layered hexagonal boron nitride down to 50 MHz were reported, close to the lifetime limit. The linewidths were extracted from time traces of laser scanning photoluminescence excitation experiments. At the same time, temporal blinking was affecting the measured time traces even in the absence of a frequency scanning the excitation laser. I argue here that the reported temporal blinking timescale is consistent with the observed transients, implying that the interpretation as spectral shapes and thus the extracted linewidths are invalid.</description><subject>Blinking</subject><subject>Boron nitride</subject><subject>Excitation</subject><subject>Fourier transforms</subject><subject>Frequency scanning</subject><subject>Photoluminescence</subject><issn>2469-9950</issn><issn>2469-9969</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNo9kM1KAzEUhYMoWGqfwE3A9dSbZP6y1GKtUKiIbtyEdObGpnQmNZkWu-uD6Mv1SYxUXZ17LudeDh8hlwyGjIG4flzswhNub4cMYAhpkQI7IT2e5jKRMpen_3MG52QQwhIAWA6yANkjryPXNNh21LX0sP-czQP6re5stM7Qsdt4i552XrfBON_QlW1sh3XUFgO1LV3gh35zrV7RufPxqrWdtzUe9l8X5MzoVcDBr_bJy_jueTRJprP7h9HNNKl4UXQJAmPVXOe8kAK1gDyFKmdVXrKiykwdvS4lZICSYVZmyI0otTC14RkIFLXok6vj37V37xsMnVrG2rFRUJwXgpUy4xBT4piqvAvBo1Frbxvtd4qB-uGo_jjGBagjR_ENcDxpzg</recordid><startdate>20190723</startdate><enddate>20190723</enddate><creator>Langbein, W.</creator><general>American Physical Society</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>H8D</scope><scope>JG9</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0001-9786-1023</orcidid></search><sort><creationdate>20190723</creationdate><title>Comment on “Observation of Fourier transform limited lines in hexagonal boron nitride”</title><author>Langbein, W.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c277t-e011cba62793ea30640c61c6817c5fd064a89050e91e585e2f38a3fdf2503e3d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Blinking</topic><topic>Boron nitride</topic><topic>Excitation</topic><topic>Fourier transforms</topic><topic>Frequency scanning</topic><topic>Photoluminescence</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Langbein, W.</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Physical review. B</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Langbein, W.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Comment on “Observation of Fourier transform limited lines in hexagonal boron nitride”</atitle><jtitle>Physical review. B</jtitle><date>2019-07-23</date><risdate>2019</risdate><volume>100</volume><issue>4</issue><spage>047401</spage><pages>047401-</pages><artnum>047401</artnum><issn>2469-9950</issn><eissn>2469-9969</eissn><abstract>Recently, emission linewidths of single defect centers in layered hexagonal boron nitride down to 50 MHz were reported, close to the lifetime limit. The linewidths were extracted from time traces of laser scanning photoluminescence excitation experiments. At the same time, temporal blinking was affecting the measured time traces even in the absence of a frequency scanning the excitation laser. I argue here that the reported temporal blinking timescale is consistent with the observed transients, implying that the interpretation as spectral shapes and thus the extracted linewidths are invalid.</abstract><cop>College Park</cop><pub>American Physical Society</pub><doi>10.1103/PhysRevB.100.047401</doi><orcidid>https://orcid.org/0000-0001-9786-1023</orcidid></addata></record> |
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subjects | Blinking Boron nitride Excitation Fourier transforms Frequency scanning Photoluminescence |
title | Comment on “Observation of Fourier transform limited lines in hexagonal boron nitride” |
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