Structural mechanisms of the high glass-forming ability in CuZrTiPd metallic glass
The issue, high glass-forming abilities (GFAs) in solute-absent multicomponent metallic glasses (MGs), has been investigated by systematic experimental measurements coupled with theoretical calculations in the Cu 34 Zr 14 Ti 36 Pd 16 quaternary alloy. It is found that the synergetic contribution of...
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Veröffentlicht in: | Journal of materials science 2019-11, Vol.54 (22), p.14209-14217 |
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creator | Li, Ming-Fei Liao, Bing Wang, Yin-Gang Yang, Liang |
description | The issue, high glass-forming abilities (GFAs) in solute-absent multicomponent metallic glasses (MGs), has been investigated by systematic experimental measurements coupled with theoretical calculations in the Cu
34
Zr
14
Ti
36
Pd
16
quaternary alloy. It is found that the synergetic contribution of some atomic- and cluster-level structural features leads to the high GFA in this quaternary composition. At the atomic scale, Pd and Ti addition decreases the size gaps between Cu and Zr atoms, and increases the atomic packing efficiency; at the cluster scale, there are more icosahedral or icosahedral-like local structures, and the cluster regularity is enhanced because of the optimization of both topological and chemical distributions in clusters. The present work provides an in-depth understanding of GFAs in multicomponent alloys, and will shed light on the development of more MGs with high GFAs. |
doi_str_mv | 10.1007/s10853-019-03890-1 |
format | Article |
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34
Zr
14
Ti
36
Pd
16
quaternary alloy. It is found that the synergetic contribution of some atomic- and cluster-level structural features leads to the high GFA in this quaternary composition. At the atomic scale, Pd and Ti addition decreases the size gaps between Cu and Zr atoms, and increases the atomic packing efficiency; at the cluster scale, there are more icosahedral or icosahedral-like local structures, and the cluster regularity is enhanced because of the optimization of both topological and chemical distributions in clusters. The present work provides an in-depth understanding of GFAs in multicomponent alloys, and will shed light on the development of more MGs with high GFAs.</description><identifier>ISSN: 0022-2461</identifier><identifier>EISSN: 1573-4803</identifier><identifier>DOI: 10.1007/s10853-019-03890-1</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Alloy development ; Amorphous materials ; Atoms ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Classical Mechanics ; Clusters ; Crystallography and Scattering Methods ; Glass ; Glass formation ; Icosahedral phase ; Materials Science ; Metallic glasses ; Metals & Corrosion ; Optimization ; Organic chemistry ; Palladium ; Polymer Sciences ; Quaternary alloys ; Solid Mechanics ; Titanium ; Zirconium</subject><ispartof>Journal of materials science, 2019-11, Vol.54 (22), p.14209-14217</ispartof><rights>Springer Science+Business Media, LLC, part of Springer Nature 2019</rights><rights>COPYRIGHT 2019 Springer</rights><rights>Journal of Materials Science is a copyright of Springer, (2019). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c392t-932cd2f7150dce3eb7d19829a13882baf9bc974c9d3518b528c697547076ca6d3</citedby><cites>FETCH-LOGICAL-c392t-932cd2f7150dce3eb7d19829a13882baf9bc974c9d3518b528c697547076ca6d3</cites><orcidid>0000-0001-9900-4244</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10853-019-03890-1$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10853-019-03890-1$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27903,27904,41467,42536,51298</link.rule.ids></links><search><creatorcontrib>Li, Ming-Fei</creatorcontrib><creatorcontrib>Liao, Bing</creatorcontrib><creatorcontrib>Wang, Yin-Gang</creatorcontrib><creatorcontrib>Yang, Liang</creatorcontrib><title>Structural mechanisms of the high glass-forming ability in CuZrTiPd metallic glass</title><title>Journal of materials science</title><addtitle>J Mater Sci</addtitle><description>The issue, high glass-forming abilities (GFAs) in solute-absent multicomponent metallic glasses (MGs), has been investigated by systematic experimental measurements coupled with theoretical calculations in the Cu
34
Zr
14
Ti
36
Pd
16
quaternary alloy. It is found that the synergetic contribution of some atomic- and cluster-level structural features leads to the high GFA in this quaternary composition. At the atomic scale, Pd and Ti addition decreases the size gaps between Cu and Zr atoms, and increases the atomic packing efficiency; at the cluster scale, there are more icosahedral or icosahedral-like local structures, and the cluster regularity is enhanced because of the optimization of both topological and chemical distributions in clusters. The present work provides an in-depth understanding of GFAs in multicomponent alloys, and will shed light on the development of more MGs with high GFAs.</description><subject>Alloy development</subject><subject>Amorphous materials</subject><subject>Atoms</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Classical Mechanics</subject><subject>Clusters</subject><subject>Crystallography and Scattering Methods</subject><subject>Glass</subject><subject>Glass formation</subject><subject>Icosahedral phase</subject><subject>Materials Science</subject><subject>Metallic glasses</subject><subject>Metals & Corrosion</subject><subject>Optimization</subject><subject>Organic chemistry</subject><subject>Palladium</subject><subject>Polymer Sciences</subject><subject>Quaternary alloys</subject><subject>Solid Mechanics</subject><subject>Titanium</subject><subject>Zirconium</subject><issn>0022-2461</issn><issn>1573-4803</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kU1r3DAQhkVJoZtt_0BPhpxy0HYkWZZ0DEubBhYasptLLkKWZa-CPxJJhuTfV6kLYS9hDgPD88wMvAh9J7AhAOJHJCA5w0AUBiYVYPIJrQgXDJcS2BlaAVCKaVmRL-g8xkcA4IKSFbrbpzDbNAfTF4OzRzP6OMRiaot0dMXRd8ei602MuJ3C4MeuMLXvfXot_Fhs54dw8LdNFpPpe28X9Cv63Jo-um__-xrd__p52P7Guz_XN9urHbZM0YQVo7ahrSAcGuuYq0VDlKTKECYlrU2raqtEaVXDOJE1p9JWSvBSgKisqRq2RhfL3qcwPc8uJv04zWHMJzWllSy5AioytVmozvRO-7GdUjA2V-MGb6fRtT7Pr3hezTglb8LliZCZ5F5SZ-YY9c3-7pSlC2vDFGNwrX4KfjDhVRPQb8HoJRidg9H_gtEkS2yRYobHzoX3vz-w_gKPGo7p</recordid><startdate>20191101</startdate><enddate>20191101</enddate><creator>Li, Ming-Fei</creator><creator>Liao, Bing</creator><creator>Wang, Yin-Gang</creator><creator>Yang, Liang</creator><general>Springer US</general><general>Springer</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>ISR</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>L6V</scope><scope>M7S</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PTHSS</scope><orcidid>https://orcid.org/0000-0001-9900-4244</orcidid></search><sort><creationdate>20191101</creationdate><title>Structural mechanisms of the high glass-forming ability in CuZrTiPd metallic glass</title><author>Li, Ming-Fei ; Liao, Bing ; Wang, Yin-Gang ; Yang, Liang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c392t-932cd2f7150dce3eb7d19829a13882baf9bc974c9d3518b528c697547076ca6d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Alloy development</topic><topic>Amorphous materials</topic><topic>Atoms</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Classical Mechanics</topic><topic>Clusters</topic><topic>Crystallography and Scattering Methods</topic><topic>Glass</topic><topic>Glass formation</topic><topic>Icosahedral phase</topic><topic>Materials Science</topic><topic>Metallic glasses</topic><topic>Metals & Corrosion</topic><topic>Optimization</topic><topic>Organic chemistry</topic><topic>Palladium</topic><topic>Polymer Sciences</topic><topic>Quaternary alloys</topic><topic>Solid Mechanics</topic><topic>Titanium</topic><topic>Zirconium</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Ming-Fei</creatorcontrib><creatorcontrib>Liao, Bing</creatorcontrib><creatorcontrib>Wang, Yin-Gang</creatorcontrib><creatorcontrib>Yang, Liang</creatorcontrib><collection>CrossRef</collection><collection>Gale In Context: Science</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>ProQuest Engineering Collection</collection><collection>Engineering Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Engineering Collection</collection><jtitle>Journal of materials science</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Ming-Fei</au><au>Liao, Bing</au><au>Wang, Yin-Gang</au><au>Yang, Liang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Structural mechanisms of the high glass-forming ability in CuZrTiPd metallic glass</atitle><jtitle>Journal of materials science</jtitle><stitle>J Mater Sci</stitle><date>2019-11-01</date><risdate>2019</risdate><volume>54</volume><issue>22</issue><spage>14209</spage><epage>14217</epage><pages>14209-14217</pages><issn>0022-2461</issn><eissn>1573-4803</eissn><abstract>The issue, high glass-forming abilities (GFAs) in solute-absent multicomponent metallic glasses (MGs), has been investigated by systematic experimental measurements coupled with theoretical calculations in the Cu
34
Zr
14
Ti
36
Pd
16
quaternary alloy. It is found that the synergetic contribution of some atomic- and cluster-level structural features leads to the high GFA in this quaternary composition. At the atomic scale, Pd and Ti addition decreases the size gaps between Cu and Zr atoms, and increases the atomic packing efficiency; at the cluster scale, there are more icosahedral or icosahedral-like local structures, and the cluster regularity is enhanced because of the optimization of both topological and chemical distributions in clusters. The present work provides an in-depth understanding of GFAs in multicomponent alloys, and will shed light on the development of more MGs with high GFAs.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10853-019-03890-1</doi><tpages>9</tpages><orcidid>https://orcid.org/0000-0001-9900-4244</orcidid></addata></record> |
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subjects | Alloy development Amorphous materials Atoms Characterization and Evaluation of Materials Chemistry and Materials Science Classical Mechanics Clusters Crystallography and Scattering Methods Glass Glass formation Icosahedral phase Materials Science Metallic glasses Metals & Corrosion Optimization Organic chemistry Palladium Polymer Sciences Quaternary alloys Solid Mechanics Titanium Zirconium |
title | Structural mechanisms of the high glass-forming ability in CuZrTiPd metallic glass |
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