Radioluminescent nuclear battery containing CsPbBr3 quantum dots: Application of a novel wave‐shifting agent

Summary Radioluminescent nuclear battery has been widely studied for its miniaturization and long life. In this study, all‐inorganic perovskite quantum dots (CsPbBr3 QDs) were selected as a novel wave‐shifting agent combined with liquid scintillator PPO (2,5‐diphenyloxazole). The QDs were used to re...

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Veröffentlicht in:International journal of energy research 2019-07, Vol.43 (9), p.4520-4533
Hauptverfasser: Chen, Wang, Tang, Xiaobin, Liu, Yunpeng, Xu, Zhiheng, Zicheng, Yuan, Zhang, Zhengrong, Liu, Kai
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Sprache:eng
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Zusammenfassung:Summary Radioluminescent nuclear battery has been widely studied for its miniaturization and long life. In this study, all‐inorganic perovskite quantum dots (CsPbBr3 QDs) were selected as a novel wave‐shifting agent combined with liquid scintillator PPO (2,5‐diphenyloxazole). The QDs were used to regulate the emission spectrum to match different GaAs devices. The maximum output power of the RL nuclear battery was greatly enhanced by 1.91 to 2.53 times. Perovskite QDs with adjustable emission spectra were used as wave‐shifting agents and exhibited more excellent properties and application prospects than traditional wave‐shifting agents. The Monte Carlo method was used to simulate the energy deposition of fluorescent materials under various radioactive source models. Results verified the advantages of using liquid radioactive sources and liquid fluorescent materials. The application and reference value of perovskite QDs in nuclear detection and nuclear medical imaging were also discussed. A novel radioluminescent nuclear battery with CsPbBr3 quantum dots as wave‐shifting agent has been developed, and its luminescence mechanism was studied. The significant improvement in the optical and electrical properties of the radioluminescent nuclear battery is mainly due to QDs regulating the RL spectra. Perovskite QDs also have excellent application prospects for the radioluminescent nuclear battery, nuclear detection, and nuclear medical imaging. This paper presents the results and laws of scientific, which is inside the scope of the International Journal of Energy Research.
ISSN:0363-907X
1099-114X
DOI:10.1002/er.4580