Bismuth oxide-based nanocomposite for high-energy electron radiation shielding
A novel polymer-based nanocomposite was fabricated to investigate its shielding properties against high-energy electron radiation for potential applications in space industry. Bismuth oxide (Bi 2 O 3 ) nanoparticles and multi-walled carbon nanotubes (MWCNT) were added to poly (methyl methacrylate) (...
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Veröffentlicht in: | Journal of materials science 2019-02, Vol.54 (4), p.3023-3034 |
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creator | Chen, Siyuan Nambiar, Shruti Li, Zhenhao Osei, Ernest Darko, Johnson Zheng, Wanping Sun, Zhendong Liu, Ping Yeow, John T. W. |
description | A novel polymer-based nanocomposite was fabricated to investigate its shielding properties against high-energy electron radiation for potential applications in space industry. Bismuth oxide (Bi
2
O
3
) nanoparticles and multi-walled carbon nanotubes (MWCNT) were added to poly (methyl methacrylate) (PMMA) to fabricate the nanocomposite. Radiation shielding efficiency of different samples, pure PMMA, PMMA/MWCNT, and PMMA/MWCNT/Bi
2
O
3
, was characterized and compared with aluminum (Al). The electron-beam attenuation characteristics show that PMMA/MWCNT/Bi
2
O
3
nanocomposite was 37% lighter in comparison with Al at the same radiation shielding effectiveness in electron energy range of 9–20 MeV. Furthermore, mechanical and thermal properties indicate that PMMA/MWCNT/Bi
2
O
3
can achieve significantly improved tensile strength, initial decomposition temperature, and glass transition temperature over pure PMMA. The stabled thermal properties, chemical structures, and morphology of all materials before and after electron irradiation lead to excellent radiation resistance of PMMA and nanocomposite. In conclusion, the proposed nanocomposite is a promising material for high-energy, electron-beam shielding applications. |
doi_str_mv | 10.1007/s10853-018-3063-0 |
format | Article |
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2
O
3
) nanoparticles and multi-walled carbon nanotubes (MWCNT) were added to poly (methyl methacrylate) (PMMA) to fabricate the nanocomposite. Radiation shielding efficiency of different samples, pure PMMA, PMMA/MWCNT, and PMMA/MWCNT/Bi
2
O
3
, was characterized and compared with aluminum (Al). The electron-beam attenuation characteristics show that PMMA/MWCNT/Bi
2
O
3
nanocomposite was 37% lighter in comparison with Al at the same radiation shielding effectiveness in electron energy range of 9–20 MeV. Furthermore, mechanical and thermal properties indicate that PMMA/MWCNT/Bi
2
O
3
can achieve significantly improved tensile strength, initial decomposition temperature, and glass transition temperature over pure PMMA. The stabled thermal properties, chemical structures, and morphology of all materials before and after electron irradiation lead to excellent radiation resistance of PMMA and nanocomposite. In conclusion, the proposed nanocomposite is a promising material for high-energy, electron-beam shielding applications.</description><identifier>ISSN: 0022-2461</identifier><identifier>EISSN: 1573-4803</identifier><identifier>DOI: 10.1007/s10853-018-3063-0</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Aluminum ; Attenuation ; Bismuth oxides ; Bismuth trioxide ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Classical Mechanics ; Composites ; Crystallography and Scattering Methods ; Electron beams ; Electron energy ; Electron irradiation ; Electron radiation ; Glass transition temperature ; High energy electrons ; Materials Science ; Morphology ; Multi wall carbon nanotubes ; Nanocomposites ; Nanoparticles ; Organic chemistry ; Polymer Sciences ; Polymethyl methacrylate ; Radiation shielding ; Radiation tolerance ; Solid Mechanics ; Thermodynamic properties</subject><ispartof>Journal of materials science, 2019-02, Vol.54 (4), p.3023-3034</ispartof><rights>Springer Science+Business Media, LLC, part of Springer Nature 2018</rights><rights>COPYRIGHT 2019 Springer</rights><rights>Copyright Springer Science & Business Media 2019</rights><rights>Journal of Materials Science is a copyright of Springer, (2018). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c417t-b87a8483df6162d4b3b371a98819ee03d9b31f72a46f9a0b25c89275363b9d513</citedby><cites>FETCH-LOGICAL-c417t-b87a8483df6162d4b3b371a98819ee03d9b31f72a46f9a0b25c89275363b9d513</cites><orcidid>0000-0003-0622-6652 ; 0000-0002-0740-8055 ; 0000-0001-6260-377X ; 0000-0002-8499-9098 ; 0000-0002-3751-2697 ; 0000-0002-4114-3273 ; 0000-0002-5474-0819 ; 0000-0003-2289-5047 ; 0000-0002-9506-1679</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10853-018-3063-0$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10853-018-3063-0$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Chen, Siyuan</creatorcontrib><creatorcontrib>Nambiar, Shruti</creatorcontrib><creatorcontrib>Li, Zhenhao</creatorcontrib><creatorcontrib>Osei, Ernest</creatorcontrib><creatorcontrib>Darko, Johnson</creatorcontrib><creatorcontrib>Zheng, Wanping</creatorcontrib><creatorcontrib>Sun, Zhendong</creatorcontrib><creatorcontrib>Liu, Ping</creatorcontrib><creatorcontrib>Yeow, John T. W.</creatorcontrib><title>Bismuth oxide-based nanocomposite for high-energy electron radiation shielding</title><title>Journal of materials science</title><addtitle>J Mater Sci</addtitle><description>A novel polymer-based nanocomposite was fabricated to investigate its shielding properties against high-energy electron radiation for potential applications in space industry. Bismuth oxide (Bi
2
O
3
) nanoparticles and multi-walled carbon nanotubes (MWCNT) were added to poly (methyl methacrylate) (PMMA) to fabricate the nanocomposite. Radiation shielding efficiency of different samples, pure PMMA, PMMA/MWCNT, and PMMA/MWCNT/Bi
2
O
3
, was characterized and compared with aluminum (Al). The electron-beam attenuation characteristics show that PMMA/MWCNT/Bi
2
O
3
nanocomposite was 37% lighter in comparison with Al at the same radiation shielding effectiveness in electron energy range of 9–20 MeV. Furthermore, mechanical and thermal properties indicate that PMMA/MWCNT/Bi
2
O
3
can achieve significantly improved tensile strength, initial decomposition temperature, and glass transition temperature over pure PMMA. The stabled thermal properties, chemical structures, and morphology of all materials before and after electron irradiation lead to excellent radiation resistance of PMMA and nanocomposite. In conclusion, the proposed nanocomposite is a promising material for high-energy, electron-beam shielding applications.</description><subject>Aluminum</subject><subject>Attenuation</subject><subject>Bismuth oxides</subject><subject>Bismuth trioxide</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Classical Mechanics</subject><subject>Composites</subject><subject>Crystallography and Scattering Methods</subject><subject>Electron beams</subject><subject>Electron energy</subject><subject>Electron irradiation</subject><subject>Electron radiation</subject><subject>Glass transition temperature</subject><subject>High energy electrons</subject><subject>Materials Science</subject><subject>Morphology</subject><subject>Multi wall carbon nanotubes</subject><subject>Nanocomposites</subject><subject>Nanoparticles</subject><subject>Organic chemistry</subject><subject>Polymer Sciences</subject><subject>Polymethyl methacrylate</subject><subject>Radiation shielding</subject><subject>Radiation tolerance</subject><subject>Solid Mechanics</subject><subject>Thermodynamic properties</subject><issn>0022-2461</issn><issn>1573-4803</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kU1rJCEQhmXZhZ3N5gfsrWFPezAptbXtYxL2IxASyMdZ7La6xzCjE3Ug-fdr6EDIIcGDRfE8avkS8oPBEQPojjMDLQUFpqkAVYtPZMVkJ2irQXwmKwDOKW8V-0q-5XwPALLjbEUuT33e7su6iY_eIR1sRtcEG-IYt7uYfcFmiqlZ-3lNMWCanxrc4FhSDE2yztvia5XXHjfOh_k7-TLZTcbDl_2A3P35fXv2j15c_T0_O7mgY8u6QgfdWd1q4SbFFHftIAbRMdtrzXpEEK4fBJs6bls19RYGLkfd804KJYbeSSYOyM_l3F2KD3vMxdzHfQr1SsO57JWos8sPKSZ0_TIu2kodLdRsN2h8mGJJdqzL4daPMeDka_9EKqUAFPAq_HojVKbgY5ntPmdzfnP9lmULO6aYc8LJ7JLf2vRkGJjn5MySnKnJmefkDFSHL06ubJgxvT77fek_ukqYkg</recordid><startdate>20190201</startdate><enddate>20190201</enddate><creator>Chen, Siyuan</creator><creator>Nambiar, Shruti</creator><creator>Li, Zhenhao</creator><creator>Osei, Ernest</creator><creator>Darko, Johnson</creator><creator>Zheng, Wanping</creator><creator>Sun, Zhendong</creator><creator>Liu, Ping</creator><creator>Yeow, John T. W.</creator><general>Springer US</general><general>Springer</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>ISR</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>L6V</scope><scope>M7S</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope><orcidid>https://orcid.org/0000-0003-0622-6652</orcidid><orcidid>https://orcid.org/0000-0002-0740-8055</orcidid><orcidid>https://orcid.org/0000-0001-6260-377X</orcidid><orcidid>https://orcid.org/0000-0002-8499-9098</orcidid><orcidid>https://orcid.org/0000-0002-3751-2697</orcidid><orcidid>https://orcid.org/0000-0002-4114-3273</orcidid><orcidid>https://orcid.org/0000-0002-5474-0819</orcidid><orcidid>https://orcid.org/0000-0003-2289-5047</orcidid><orcidid>https://orcid.org/0000-0002-9506-1679</orcidid></search><sort><creationdate>20190201</creationdate><title>Bismuth oxide-based nanocomposite for high-energy electron radiation shielding</title><author>Chen, Siyuan ; Nambiar, Shruti ; Li, Zhenhao ; Osei, Ernest ; Darko, Johnson ; Zheng, Wanping ; Sun, Zhendong ; Liu, Ping ; Yeow, John T. W.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c417t-b87a8483df6162d4b3b371a98819ee03d9b31f72a46f9a0b25c89275363b9d513</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Aluminum</topic><topic>Attenuation</topic><topic>Bismuth oxides</topic><topic>Bismuth trioxide</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Classical Mechanics</topic><topic>Composites</topic><topic>Crystallography and Scattering Methods</topic><topic>Electron beams</topic><topic>Electron energy</topic><topic>Electron irradiation</topic><topic>Electron radiation</topic><topic>Glass transition temperature</topic><topic>High energy electrons</topic><topic>Materials Science</topic><topic>Morphology</topic><topic>Multi wall carbon nanotubes</topic><topic>Nanocomposites</topic><topic>Nanoparticles</topic><topic>Organic chemistry</topic><topic>Polymer Sciences</topic><topic>Polymethyl methacrylate</topic><topic>Radiation shielding</topic><topic>Radiation tolerance</topic><topic>Solid Mechanics</topic><topic>Thermodynamic properties</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chen, Siyuan</creatorcontrib><creatorcontrib>Nambiar, Shruti</creatorcontrib><creatorcontrib>Li, Zhenhao</creatorcontrib><creatorcontrib>Osei, Ernest</creatorcontrib><creatorcontrib>Darko, Johnson</creatorcontrib><creatorcontrib>Zheng, Wanping</creatorcontrib><creatorcontrib>Sun, Zhendong</creatorcontrib><creatorcontrib>Liu, Ping</creatorcontrib><creatorcontrib>Yeow, John T. 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W.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Bismuth oxide-based nanocomposite for high-energy electron radiation shielding</atitle><jtitle>Journal of materials science</jtitle><stitle>J Mater Sci</stitle><date>2019-02-01</date><risdate>2019</risdate><volume>54</volume><issue>4</issue><spage>3023</spage><epage>3034</epage><pages>3023-3034</pages><issn>0022-2461</issn><eissn>1573-4803</eissn><abstract>A novel polymer-based nanocomposite was fabricated to investigate its shielding properties against high-energy electron radiation for potential applications in space industry. Bismuth oxide (Bi
2
O
3
) nanoparticles and multi-walled carbon nanotubes (MWCNT) were added to poly (methyl methacrylate) (PMMA) to fabricate the nanocomposite. Radiation shielding efficiency of different samples, pure PMMA, PMMA/MWCNT, and PMMA/MWCNT/Bi
2
O
3
, was characterized and compared with aluminum (Al). The electron-beam attenuation characteristics show that PMMA/MWCNT/Bi
2
O
3
nanocomposite was 37% lighter in comparison with Al at the same radiation shielding effectiveness in electron energy range of 9–20 MeV. Furthermore, mechanical and thermal properties indicate that PMMA/MWCNT/Bi
2
O
3
can achieve significantly improved tensile strength, initial decomposition temperature, and glass transition temperature over pure PMMA. The stabled thermal properties, chemical structures, and morphology of all materials before and after electron irradiation lead to excellent radiation resistance of PMMA and nanocomposite. In conclusion, the proposed nanocomposite is a promising material for high-energy, electron-beam shielding applications.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10853-018-3063-0</doi><tpages>12</tpages><orcidid>https://orcid.org/0000-0003-0622-6652</orcidid><orcidid>https://orcid.org/0000-0002-0740-8055</orcidid><orcidid>https://orcid.org/0000-0001-6260-377X</orcidid><orcidid>https://orcid.org/0000-0002-8499-9098</orcidid><orcidid>https://orcid.org/0000-0002-3751-2697</orcidid><orcidid>https://orcid.org/0000-0002-4114-3273</orcidid><orcidid>https://orcid.org/0000-0002-5474-0819</orcidid><orcidid>https://orcid.org/0000-0003-2289-5047</orcidid><orcidid>https://orcid.org/0000-0002-9506-1679</orcidid></addata></record> |
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subjects | Aluminum Attenuation Bismuth oxides Bismuth trioxide Characterization and Evaluation of Materials Chemistry and Materials Science Classical Mechanics Composites Crystallography and Scattering Methods Electron beams Electron energy Electron irradiation Electron radiation Glass transition temperature High energy electrons Materials Science Morphology Multi wall carbon nanotubes Nanocomposites Nanoparticles Organic chemistry Polymer Sciences Polymethyl methacrylate Radiation shielding Radiation tolerance Solid Mechanics Thermodynamic properties |
title | Bismuth oxide-based nanocomposite for high-energy electron radiation shielding |
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