Facile synthesis of nitrogen-containing porous carbon as electrode materials for superior-performance electrical double-layer capacitors
Nitrogen-containing porous carbons with numerous micropores were fabricated by pyrolysing polyvinylidene fluoride (PVDF) membrane following potassium hydroxide (KOH) activation at 600–900 °C for 2 h under N 2 atmosphere. The fabricated nitrogen-containing porous carbons have a large specific surface...
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Veröffentlicht in: | Journal of materials science 2018-02, Vol.53 (3), p.2137-2148 |
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container_title | Journal of materials science |
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creator | Chen, Jing Wei, Huanming Fu, Ning Chen, Haijun Lan, Guoxian Lin, Hualin Han, Sheng |
description | Nitrogen-containing porous carbons with numerous micropores were fabricated by pyrolysing polyvinylidene fluoride (PVDF) membrane following potassium hydroxide (KOH) activation at 600–900 °C for 2 h under N
2
atmosphere. The fabricated nitrogen-containing porous carbons have a large specific surface area of approximately 2289 m
2
g
−1
, a certain nitrogen content of 1.35 at.% and a favourable hierarchical porous structure possessing a great number of micropores and a part of mesopores. The carbon materials exhibit high specific capacitance of 338 F g
−1
at 0.5 A g
−1
in a 6 M KOH and outstanding cycling property of 91.6% maintenance at 2 A g
−1
after 10000 cycles. An all-solid-state symmetrical supercapacitor with these as-prepared materials as electrodes can deliver energy densities of 21.9 to 10.4 W h kg
−1
at power densities from 700.8 to 12910.3 W kg
−1
. To sum up, the as-obtained porous carbon is a type of potential electrode material for electrical double-layer capacitor. |
doi_str_mv | 10.1007/s10853-017-1664-7 |
format | Article |
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2
atmosphere. The fabricated nitrogen-containing porous carbons have a large specific surface area of approximately 2289 m
2
g
−1
, a certain nitrogen content of 1.35 at.% and a favourable hierarchical porous structure possessing a great number of micropores and a part of mesopores. The carbon materials exhibit high specific capacitance of 338 F g
−1
at 0.5 A g
−1
in a 6 M KOH and outstanding cycling property of 91.6% maintenance at 2 A g
−1
after 10000 cycles. An all-solid-state symmetrical supercapacitor with these as-prepared materials as electrodes can deliver energy densities of 21.9 to 10.4 W h kg
−1
at power densities from 700.8 to 12910.3 W kg
−1
. To sum up, the as-obtained porous carbon is a type of potential electrode material for electrical double-layer capacitor.</description><identifier>ISSN: 0022-2461</identifier><identifier>EISSN: 1573-4803</identifier><identifier>DOI: 10.1007/s10853-017-1664-7</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Capacitors ; Carbon ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Circuit components ; Classical Mechanics ; Crystallography and Scattering Methods ; Electrode materials ; Electrodes ; Electronic components industry ; Energy Materials ; Hydroxides ; Materials Science ; Nitrogen ; Polymer Sciences ; Polyvinylidene fluoride ; Polyvinylidene fluorides ; Porous materials ; Potassium hydroxides ; Solid Mechanics ; Structural hierarchy</subject><ispartof>Journal of materials science, 2018-02, Vol.53 (3), p.2137-2148</ispartof><rights>Springer Science+Business Media, LLC 2017</rights><rights>COPYRIGHT 2018 Springer</rights><rights>Journal of Materials Science is a copyright of Springer, (2017). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c426t-82ec3b3b3146f59836d554a8e39454b1061441466267ea469633c8e645a9978a3</citedby><cites>FETCH-LOGICAL-c426t-82ec3b3b3146f59836d554a8e39454b1061441466267ea469633c8e645a9978a3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10853-017-1664-7$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10853-017-1664-7$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27903,27904,41467,42536,51298</link.rule.ids></links><search><creatorcontrib>Chen, Jing</creatorcontrib><creatorcontrib>Wei, Huanming</creatorcontrib><creatorcontrib>Fu, Ning</creatorcontrib><creatorcontrib>Chen, Haijun</creatorcontrib><creatorcontrib>Lan, Guoxian</creatorcontrib><creatorcontrib>Lin, Hualin</creatorcontrib><creatorcontrib>Han, Sheng</creatorcontrib><title>Facile synthesis of nitrogen-containing porous carbon as electrode materials for superior-performance electrical double-layer capacitors</title><title>Journal of materials science</title><addtitle>J Mater Sci</addtitle><description>Nitrogen-containing porous carbons with numerous micropores were fabricated by pyrolysing polyvinylidene fluoride (PVDF) membrane following potassium hydroxide (KOH) activation at 600–900 °C for 2 h under N
2
atmosphere. The fabricated nitrogen-containing porous carbons have a large specific surface area of approximately 2289 m
2
g
−1
, a certain nitrogen content of 1.35 at.% and a favourable hierarchical porous structure possessing a great number of micropores and a part of mesopores. The carbon materials exhibit high specific capacitance of 338 F g
−1
at 0.5 A g
−1
in a 6 M KOH and outstanding cycling property of 91.6% maintenance at 2 A g
−1
after 10000 cycles. An all-solid-state symmetrical supercapacitor with these as-prepared materials as electrodes can deliver energy densities of 21.9 to 10.4 W h kg
−1
at power densities from 700.8 to 12910.3 W kg
−1
. To sum up, the as-obtained porous carbon is a type of potential electrode material for electrical double-layer capacitor.</description><subject>Capacitors</subject><subject>Carbon</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Circuit components</subject><subject>Classical Mechanics</subject><subject>Crystallography and Scattering Methods</subject><subject>Electrode materials</subject><subject>Electrodes</subject><subject>Electronic components industry</subject><subject>Energy Materials</subject><subject>Hydroxides</subject><subject>Materials Science</subject><subject>Nitrogen</subject><subject>Polymer Sciences</subject><subject>Polyvinylidene fluoride</subject><subject>Polyvinylidene fluorides</subject><subject>Porous materials</subject><subject>Potassium hydroxides</subject><subject>Solid Mechanics</subject><subject>Structural hierarchy</subject><issn>0022-2461</issn><issn>1573-4803</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp1kc-KFDEQxoMoOK4-gLeAJw9Z87-7j8vi6sLCwqrnkMlUt1l6kjZJg_MGPrY19ILsQepQFPl99YX6CHkv-KXgvPtUBe-NYlx0TFirWfeC7ITpFNM9Vy_JjnMpmdRWvCZvan3knJtOih35c-NDnIHWU2o_ocZK80hTbCVPkFjIqfmYYprokkteKw2-7HOivlKYISB2AHr0DUr0c6VjLrSuC065MGw4H30K8ATH4Gd6yOt-Bjb7ExRct6B_y6W-Ja9GXAHvnvoF-XHz-fv1V3Z3_-X2-uqOBS1tY72EoPZYQtvRDL2yB2O070EN2ui94FZojW9W2g68toNVKvRgtfHD0PVeXZAP296l5F8r1OYe81oSWjopzWCF0tYgdblRk5_BxTTmVnzAOsAx4lVgxKO5K4NmepCiQ8HHZ4Lz5eB3m_xaq7v99vCcFRsbSq61wOiWEo--nJzg7pym29J0mKY7p-nOGrlpKrJpgvLv2_8X_QU5l6LO</recordid><startdate>20180201</startdate><enddate>20180201</enddate><creator>Chen, Jing</creator><creator>Wei, Huanming</creator><creator>Fu, Ning</creator><creator>Chen, Haijun</creator><creator>Lan, Guoxian</creator><creator>Lin, Hualin</creator><creator>Han, Sheng</creator><general>Springer US</general><general>Springer</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>ISR</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>L6V</scope><scope>M7S</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope></search><sort><creationdate>20180201</creationdate><title>Facile synthesis of nitrogen-containing porous carbon as electrode materials for superior-performance electrical double-layer capacitors</title><author>Chen, Jing ; Wei, Huanming ; Fu, Ning ; Chen, Haijun ; Lan, Guoxian ; Lin, Hualin ; Han, Sheng</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c426t-82ec3b3b3146f59836d554a8e39454b1061441466267ea469633c8e645a9978a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Capacitors</topic><topic>Carbon</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Circuit components</topic><topic>Classical Mechanics</topic><topic>Crystallography and Scattering Methods</topic><topic>Electrode materials</topic><topic>Electrodes</topic><topic>Electronic components industry</topic><topic>Energy Materials</topic><topic>Hydroxides</topic><topic>Materials Science</topic><topic>Nitrogen</topic><topic>Polymer Sciences</topic><topic>Polyvinylidene fluoride</topic><topic>Polyvinylidene fluorides</topic><topic>Porous materials</topic><topic>Potassium hydroxides</topic><topic>Solid Mechanics</topic><topic>Structural hierarchy</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chen, Jing</creatorcontrib><creatorcontrib>Wei, Huanming</creatorcontrib><creatorcontrib>Fu, Ning</creatorcontrib><creatorcontrib>Chen, Haijun</creatorcontrib><creatorcontrib>Lan, Guoxian</creatorcontrib><creatorcontrib>Lin, Hualin</creatorcontrib><creatorcontrib>Han, Sheng</creatorcontrib><collection>CrossRef</collection><collection>Gale In Context: Science</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>ProQuest Engineering Collection</collection><collection>Engineering Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Engineering Collection</collection><jtitle>Journal of materials science</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chen, Jing</au><au>Wei, Huanming</au><au>Fu, Ning</au><au>Chen, Haijun</au><au>Lan, Guoxian</au><au>Lin, Hualin</au><au>Han, Sheng</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Facile synthesis of nitrogen-containing porous carbon as electrode materials for superior-performance electrical double-layer capacitors</atitle><jtitle>Journal of materials science</jtitle><stitle>J Mater Sci</stitle><date>2018-02-01</date><risdate>2018</risdate><volume>53</volume><issue>3</issue><spage>2137</spage><epage>2148</epage><pages>2137-2148</pages><issn>0022-2461</issn><eissn>1573-4803</eissn><abstract>Nitrogen-containing porous carbons with numerous micropores were fabricated by pyrolysing polyvinylidene fluoride (PVDF) membrane following potassium hydroxide (KOH) activation at 600–900 °C for 2 h under N
2
atmosphere. The fabricated nitrogen-containing porous carbons have a large specific surface area of approximately 2289 m
2
g
−1
, a certain nitrogen content of 1.35 at.% and a favourable hierarchical porous structure possessing a great number of micropores and a part of mesopores. The carbon materials exhibit high specific capacitance of 338 F g
−1
at 0.5 A g
−1
in a 6 M KOH and outstanding cycling property of 91.6% maintenance at 2 A g
−1
after 10000 cycles. An all-solid-state symmetrical supercapacitor with these as-prepared materials as electrodes can deliver energy densities of 21.9 to 10.4 W h kg
−1
at power densities from 700.8 to 12910.3 W kg
−1
. To sum up, the as-obtained porous carbon is a type of potential electrode material for electrical double-layer capacitor.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10853-017-1664-7</doi><tpages>12</tpages></addata></record> |
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subjects | Capacitors Carbon Characterization and Evaluation of Materials Chemistry and Materials Science Circuit components Classical Mechanics Crystallography and Scattering Methods Electrode materials Electrodes Electronic components industry Energy Materials Hydroxides Materials Science Nitrogen Polymer Sciences Polyvinylidene fluoride Polyvinylidene fluorides Porous materials Potassium hydroxides Solid Mechanics Structural hierarchy |
title | Facile synthesis of nitrogen-containing porous carbon as electrode materials for superior-performance electrical double-layer capacitors |
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