High surface area ordered mesoporous carbons from waste polyester: effective adsorbent for organic pollutants from aqueous solution
With using ordered mesoporous silica as a hard template, high surface area porous carbon materials were prepared when a chemical degradation of waste polyester beverage packaging was employed as a precursor, and it was characterized by X-ray diffraction, Brunauer–Emmett–Teller, scanning electron mic...
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| Veröffentlicht in: | Journal of sol-gel science and technology 2017-08, Vol.83 (2), p.413-421 |
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| creator | Yang, Jie Jin, Ying Xue Yu, Xin Ping Yue, Qun Feng |
| description | With using ordered mesoporous silica as a hard template, high surface area porous carbon materials were prepared when a chemical degradation of waste polyester beverage packaging was employed as a precursor, and it was characterized by X-ray diffraction, Brunauer–Emmett–Teller, scanning electron microscopy, and transmission electron microscopy. Polyester derived porous carbons were used as adsorbents to remove three typical organic pollutants, phenol, methylene blue, and 1-butyl-3-methylimidazolium chloride ([Bmim]Cl) from water. The effects of several parameters including contact time, adsorption temperature, and initial concentration were investigated via batch adsorption experiments. The adsorption kinetics fitted well with pseudo-second-order model and intraparticle diffusion mode. Furthermore, linear isotherm studies revealed better fitting of Langmuir model to adsorption data, and the estimated maximum monolayer adsorption capacity for phenol, methylene blue, and [Bmim]Cl was 675.7, 5298.6, and 341.3 mg/g, respectively.
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| doi_str_mv | 10.1007/s10971-017-4419-7 |
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Graphical Abstract</description><subject>Adsorbents</subject><subject>Adsorption</subject><subject>Aqueous solutions</subject><subject>Ceramics</subject><subject>Chemistry and Materials Science</subject><subject>Chlorides</subject><subject>Composites</subject><subject>environment and building applications</subject><subject>Glass</subject><subject>Inorganic Chemistry</subject><subject>Materials Science</subject><subject>Methylene blue</subject><subject>Microscopy</subject><subject>Nanotechnology</subject><subject>Natural Materials</subject><subject>Optical and Electronic Materials</subject><subject>Organic chemistry</subject><subject>Original Paper: Sol-gel and hybrid materials for energy</subject><subject>Packaging</subject><subject>Phenols</subject><subject>Pollutants</subject><subject>Polyesters</subject><subject>Porous materials</subject><subject>Scanning electron microscopy</subject><subject>Silicon dioxide</subject><subject>Surface area</subject><subject>Surface chemistry</subject><subject>Transmission electron microscopy</subject><subject>X-ray diffraction</subject><issn>0928-0707</issn><issn>1573-4846</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kU1LxDAQhoMouH78AG8Bz9VJmzSNN1n8AsGLnkOaTtYuu806aRXP_nGzrAcvesoQnveZgZexMwEXAkBfJgFGiwKELqQUptB7bCaUrgrZyHqfzcCUTQEa9CE7SmkJAEoKPWNf9_3ilaeJgvPIHaHjkTok7PgaU9xEilPi3lEbh8QDxTX_cGlEvomrT8wDXXEMAf3Yv-d8lyK1OIw8RMqihRt6v0VX0-iG8Ufg3ibcWlPM330cTthBcKuEpz_vMXu5vXme3xePT3cP8-vHwleNGAvjpXcegtedQVAtli5ULtRGgcCuNihd03oFZVvJuqtbqU3rhWpqia3ofFUds_Odd0Mxn5BGu4wTDXmlLUtllCqz6T9KGKGUMY2CTIkd5SmmRBjshvq1o08rwG4bsbtGbG7EbhuxOmfKXSZldlgg_TL_GfoGA2yRkg</recordid><startdate>20170801</startdate><enddate>20170801</enddate><creator>Yang, Jie</creator><creator>Jin, Ying Xue</creator><creator>Yu, Xin Ping</creator><creator>Yue, Qun Feng</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>L6V</scope><scope>M7S</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope></search><sort><creationdate>20170801</creationdate><title>High surface area ordered mesoporous carbons from waste polyester: effective adsorbent for organic pollutants from aqueous solution</title><author>Yang, Jie ; Jin, Ying Xue ; Yu, Xin Ping ; Yue, Qun Feng</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c381t-9c4cac0fc7d9e05be2af3af69501ed69e4a8bc502b346d6b479bc15864eb1dc33</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><topic>Adsorbents</topic><topic>Adsorption</topic><topic>Aqueous solutions</topic><topic>Ceramics</topic><topic>Chemistry and Materials Science</topic><topic>Chlorides</topic><topic>Composites</topic><topic>environment and building applications</topic><topic>Glass</topic><topic>Inorganic Chemistry</topic><topic>Materials Science</topic><topic>Methylene blue</topic><topic>Microscopy</topic><topic>Nanotechnology</topic><topic>Natural Materials</topic><topic>Optical and Electronic Materials</topic><topic>Organic chemistry</topic><topic>Original Paper: Sol-gel and hybrid materials for energy</topic><topic>Packaging</topic><topic>Phenols</topic><topic>Pollutants</topic><topic>Polyesters</topic><topic>Porous materials</topic><topic>Scanning electron microscopy</topic><topic>Silicon dioxide</topic><topic>Surface area</topic><topic>Surface chemistry</topic><topic>Transmission electron microscopy</topic><topic>X-ray diffraction</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yang, Jie</creatorcontrib><creatorcontrib>Jin, Ying Xue</creatorcontrib><creatorcontrib>Yu, Xin Ping</creatorcontrib><creatorcontrib>Yue, Qun Feng</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>ProQuest Engineering Collection</collection><collection>Engineering Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Engineering Collection</collection><jtitle>Journal of sol-gel science and technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yang, Jie</au><au>Jin, Ying Xue</au><au>Yu, Xin Ping</au><au>Yue, Qun Feng</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>High surface area ordered mesoporous carbons from waste polyester: effective adsorbent for organic pollutants from aqueous solution</atitle><jtitle>Journal of sol-gel science and technology</jtitle><stitle>J Sol-Gel Sci Technol</stitle><date>2017-08-01</date><risdate>2017</risdate><volume>83</volume><issue>2</issue><spage>413</spage><epage>421</epage><pages>413-421</pages><issn>0928-0707</issn><eissn>1573-4846</eissn><abstract>With using ordered mesoporous silica as a hard template, high surface area porous carbon materials were prepared when a chemical degradation of waste polyester beverage packaging was employed as a precursor, and it was characterized by X-ray diffraction, Brunauer–Emmett–Teller, scanning electron microscopy, and transmission electron microscopy. Polyester derived porous carbons were used as adsorbents to remove three typical organic pollutants, phenol, methylene blue, and 1-butyl-3-methylimidazolium chloride ([Bmim]Cl) from water. The effects of several parameters including contact time, adsorption temperature, and initial concentration were investigated via batch adsorption experiments. The adsorption kinetics fitted well with pseudo-second-order model and intraparticle diffusion mode. Furthermore, linear isotherm studies revealed better fitting of Langmuir model to adsorption data, and the estimated maximum monolayer adsorption capacity for phenol, methylene blue, and [Bmim]Cl was 675.7, 5298.6, and 341.3 mg/g, respectively.
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| subjects | Adsorbents Adsorption Aqueous solutions Ceramics Chemistry and Materials Science Chlorides Composites environment and building applications Glass Inorganic Chemistry Materials Science Methylene blue Microscopy Nanotechnology Natural Materials Optical and Electronic Materials Organic chemistry Original Paper: Sol-gel and hybrid materials for energy Packaging Phenols Pollutants Polyesters Porous materials Scanning electron microscopy Silicon dioxide Surface area Surface chemistry Transmission electron microscopy X-ray diffraction |
| title | High surface area ordered mesoporous carbons from waste polyester: effective adsorbent for organic pollutants from aqueous solution |
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