Infrared evidence for the existence of nitrate species on Cu-ZSM5 during isothermal rate oscillations in the decomposition of N2O

Isothermal oscillations in the rate of decomposition of N2O were studied on an over-exchanged Cu-ZSM-5 catalyst by mass spectroscopy and in situ transient FTIR. Oscillations in the production of O2 and N2 were observed to occur in a temperature range of 410–490°C at a total pressure of 1.0 Torr pure...

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Veröffentlicht in:	Catalysis letters 2001-01, Vol.77 (1-3), p.15-19
Hauptverfasser:	FANSON, Paul T, STRADT, Martin W, DELGASS, W. Nicholas, LAUTERBACH, Jochen
Format:	Artikel
Sprache:	eng
Schlagworte:	Catalysis Catalytic reactions Chemistry Copper Correlation analysis Decomposition Exact sciences and technology Fourier transforms General and physical chemistry Infrared spectroscopy Nitrates Nitrous oxide Oscillations Surface stability Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
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