Ambient electrohydrogenation of N2 for NH3 synthesis on non-metal boron phosphide nanoparticles: the critical role of P in boosting the catalytic activity

As a carbon-neutral alternative to the Haber–Bosch process, electrochemical N2 reduction enables environment-friendly NH3 synthesis under ambient conditions but needs active electrocatalysts for the N2 reduction reaction (NRR). In this communication, we report on the first experimental demonstration...

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Veröffentlicht in:	Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2019-01, Vol.7 (27), p.16117-16121
Hauptverfasser:	Zhu, Xiaojuan, Wu, Tongwei, Ji, Lei, Li, Chengbo, Wang, Ting, Wen, Shaohua, Gao, Shuyan, Shi, Xifeng, Luo, Yonglan, Peng, Qiling, Sun, Xuping
Format:	Artikel
Sprache:	eng
Schlagworte:	Ammonia Boron Boron phosphides Catalysis Catalysts Catalytic activity Chemical reduction Density functional theory Electrocatalysts Electrochemistry Metals Nanoparticles Selectivity Synthesis
Online-Zugang:	Volltext
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