Probing ultrafast dynamics during and after passing through conical intersections
Time-resolved photoelectron spectroscopy using vacuum-UV probe pulses enables observing ultrafast dynamics during and after passing through conical intersections (CIs). The ring-puckering CI plays a prominent role following the ππ* photoexcitation of furan. More than 90% of the excited molecules saf...
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| Veröffentlicht in: | Physical chemistry chemical physics : PCCP 2019-07, Vol.21 (26), p.1392-1395 |
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| container_issue | 26 |
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| container_title | Physical chemistry chemical physics : PCCP |
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| creator | Adachi, Shunsuke Schatteburg, Tom Humeniuk, Alexander Mitri, Roland Suzuki, Toshinori |
| description | Time-resolved photoelectron spectroscopy using vacuum-UV probe pulses enables observing ultrafast dynamics during and after passing through conical intersections (CIs). The ring-puckering CI plays a prominent role following the ππ* photoexcitation of furan. More than 90% of the excited molecules safely return to the original ground state, while the remaining 10% transforms into isomers after passing through the puckering CI.
Time-resolved photoelectron spectroscopy using vacuum-UV probe pulses enables observing ultrafast dynamics during and after passing through conical intersections. |
| doi_str_mv | 10.1039/c8cp04426k |
| format | Article |
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| ispartof | Physical chemistry chemical physics : PCCP, 2019-07, Vol.21 (26), p.1392-1395 |
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| language | eng |
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| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Intersections Isomers Photoelectrons Photoexcitation Potential energy Spectra Spectrum analysis |
| title | Probing ultrafast dynamics during and after passing through conical intersections |
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