Nonlinear photoresponse of type-II Weyl semimetals

The experimental manifestation of topological effects in bulk materials is attracting enormous research interest. However, direct experimental evidence of the effective k -space monopole of the Weyl nodes has so far been lacking. Here, signatures of the singular topology of the type-II Weyl semimeta...

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Veröffentlicht in:Nature materials 2019-05, Vol.18 (5), p.476-481
Hauptverfasser: Ma, Junchao, Gu, Qiangqiang, Liu, Yinan, Lai, Jiawei, Yu, Peng, Zhuo, Xiao, Liu, Zheng, Chen, Jian-Hao, Feng, Ji, Sun, Dong
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container_issue 5
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container_title Nature materials
container_volume 18
creator Ma, Junchao
Gu, Qiangqiang
Liu, Yinan
Lai, Jiawei
Yu, Peng
Zhuo, Xiao
Liu, Zheng
Chen, Jian-Hao
Feng, Ji
Sun, Dong
description The experimental manifestation of topological effects in bulk materials is attracting enormous research interest. However, direct experimental evidence of the effective k -space monopole of the Weyl nodes has so far been lacking. Here, signatures of the singular topology of the type-II Weyl semimetal TaIrTe 4 are revealed in the photoresponses, which are related to divergence of the Berry curvature. TaIrTe 4 exhibits a large photoresponsivity of 130.2 mA W −1 —with 4 μm excitation in an unbiased field-effect transistor at room temperature—arising from the third-order nonlinear optical response, approaching the performance of commercial low-temperature detectors. In addition, the circularly polarized galvanic response is enhanced at 4 μm, possibly due to the same Berry curvature singularity enhancement. Considering the optical selection rule of chiral Weyl cones, this may open the door for studying and controlling the chiral polarization of Weyl fermions with an electric field in addition to the optical helicities. A large photoresponse is observed in the type-II Weyl semimetal TaIrTe 4 , and attributed to the diverging Berry curvature of the Weyl nodes.
doi_str_mv 10.1038/s41563-019-0296-5
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However, direct experimental evidence of the effective k -space monopole of the Weyl nodes has so far been lacking. Here, signatures of the singular topology of the type-II Weyl semimetal TaIrTe 4 are revealed in the photoresponses, which are related to divergence of the Berry curvature. TaIrTe 4 exhibits a large photoresponsivity of 130.2 mA W −1 —with 4 μm excitation in an unbiased field-effect transistor at room temperature—arising from the third-order nonlinear optical response, approaching the performance of commercial low-temperature detectors. In addition, the circularly polarized galvanic response is enhanced at 4 μm, possibly due to the same Berry curvature singularity enhancement. Considering the optical selection rule of chiral Weyl cones, this may open the door for studying and controlling the chiral polarization of Weyl fermions with an electric field in addition to the optical helicities. 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subjects 639/301/1019/385
639/301/119/2792
Biomaterials
Chemistry and Materials Science
Circular polarization
Condensed Matter Physics
Cones
Curvature
Divergence
Electric fields
Energy
Fermions
Field effect transistors
Low temperature
Materials Science
Metalloids
Nanotechnology
Nonlinear response
Optical and Electronic Materials
Semiconductor devices
Symmetry
Topology
title Nonlinear photoresponse of type-II Weyl semimetals
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