Solution Processed Large-scale Multiferroic Complex Oxide Epitaxy with Magnetically Switched Polarization
Complex oxides with tunable structures have many fascinating properties, though high-quality complex oxide epitaxy with precisely controlled composition is still out of reach. Here we have successfully developed solution-based single crystalline epitaxy for multiferroic (1-x)BiTi(1-y)/2FeyMg(1-y)/2O...
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| creator | Liu, Cong An, Feng Gharavi, Paria S M Lu, Qinwen Chen, Chao Wang, Liming Zhan, Xiaozhi Xu, Zedong Zhang, Yuan Qu, Ke Yao, Junxiang Ou, Yun Zhong, Xiangli Zhang, Dongwen Nagarajan Valanoor Lang, Chen Zhu, Tao Chen, Deyang Zhai, Xiaofang Gao, Peng Jia, Tingting Xie, Shuhong Zhong, Gaokuo Li, Jiangyu |
| description | Complex oxides with tunable structures have many fascinating properties, though high-quality complex oxide epitaxy with precisely controlled composition is still out of reach. Here we have successfully developed solution-based single crystalline epitaxy for multiferroic (1-x)BiTi(1-y)/2FeyMg(1-y)/2O3-(x)CaTiO3 (BTFM-CTO) solid solution in large area, confirming its ferroelectricity at atomic-scale with a spontaneous polarization of 79~89uC/cm2. Careful compositional tuning leads to a bulk magnetization of ~0.07uB/Fe at room temperature, enabling magnetically induced polarization switching exhibiting a large magnetoelectric coefficient of 2.7-3.0X10-7s/m. This work demonstrates the great potential of solution processing in large-scale complex oxide epitaxy and establishes novel room-temperature magnetoelectric coupling in epitaxial BTFM-CTO film, making it possible to explore a much wider space of composition, phase, and structure that can be easily scaled up for industrial applications. |
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Here we have successfully developed solution-based single crystalline epitaxy for multiferroic (1-x)BiTi(1-y)/2FeyMg(1-y)/2O3-(x)CaTiO3 (BTFM-CTO) solid solution in large area, confirming its ferroelectricity at atomic-scale with a spontaneous polarization of 79~89uC/cm2. Careful compositional tuning leads to a bulk magnetization of ~0.07uB/Fe at room temperature, enabling magnetically induced polarization switching exhibiting a large magnetoelectric coefficient of 2.7-3.0X10-7s/m. 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An, Feng ; Gharavi, Paria S M ; Lu, Qinwen ; Chen, Chao ; Wang, Liming ; Zhan, Xiaozhi ; Xu, Zedong ; Zhang, Yuan ; Qu, Ke ; Yao, Junxiang ; Ou, Yun ; Zhong, Xiangli ; Zhang, Dongwen ; Nagarajan Valanoor ; Lang, Chen ; Zhu, Tao ; Chen, Deyang ; Zhai, Xiaofang ; Gao, Peng ; Jia, Tingting ; Xie, Shuhong ; Zhong, Gaokuo ; Li, Jiangyu</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-proquest_journals_22057582983</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Calcium titanate</topic><topic>Composition</topic><topic>Epitaxy</topic><topic>Ferroelectricity</topic><topic>Induced polarization</topic><topic>Industrial applications</topic><topic>Multiferroic materials</topic><topic>Solid solutions</topic><toplevel>online_resources</toplevel><creatorcontrib>Liu, Cong</creatorcontrib><creatorcontrib>An, Feng</creatorcontrib><creatorcontrib>Gharavi, Paria S M</creatorcontrib><creatorcontrib>Lu, Qinwen</creatorcontrib><creatorcontrib>Chen, Chao</creatorcontrib><creatorcontrib>Wang, Liming</creatorcontrib><creatorcontrib>Zhan, Xiaozhi</creatorcontrib><creatorcontrib>Xu, Zedong</creatorcontrib><creatorcontrib>Zhang, Yuan</creatorcontrib><creatorcontrib>Qu, Ke</creatorcontrib><creatorcontrib>Yao, Junxiang</creatorcontrib><creatorcontrib>Ou, Yun</creatorcontrib><creatorcontrib>Zhong, Xiangli</creatorcontrib><creatorcontrib>Zhang, Dongwen</creatorcontrib><creatorcontrib>Nagarajan Valanoor</creatorcontrib><creatorcontrib>Lang, Chen</creatorcontrib><creatorcontrib>Zhu, Tao</creatorcontrib><creatorcontrib>Chen, Deyang</creatorcontrib><creatorcontrib>Zhai, Xiaofang</creatorcontrib><creatorcontrib>Gao, Peng</creatorcontrib><creatorcontrib>Jia, Tingting</creatorcontrib><creatorcontrib>Xie, Shuhong</creatorcontrib><creatorcontrib>Zhong, Gaokuo</creatorcontrib><creatorcontrib>Li, Jiangyu</creatorcontrib><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Engineering Collection</collection><collection>Engineering Database</collection><collection>Access via ProQuest (Open Access)</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Engineering Collection</collection></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Liu, Cong</au><au>An, Feng</au><au>Gharavi, Paria S M</au><au>Lu, Qinwen</au><au>Chen, Chao</au><au>Wang, Liming</au><au>Zhan, Xiaozhi</au><au>Xu, Zedong</au><au>Zhang, Yuan</au><au>Qu, Ke</au><au>Yao, Junxiang</au><au>Ou, Yun</au><au>Zhong, Xiangli</au><au>Zhang, Dongwen</au><au>Nagarajan Valanoor</au><au>Lang, Chen</au><au>Zhu, Tao</au><au>Chen, Deyang</au><au>Zhai, Xiaofang</au><au>Gao, Peng</au><au>Jia, Tingting</au><au>Xie, Shuhong</au><au>Zhong, Gaokuo</au><au>Li, Jiangyu</au><format>book</format><genre>document</genre><ristype>GEN</ristype><atitle>Solution Processed Large-scale Multiferroic Complex Oxide Epitaxy with Magnetically Switched Polarization</atitle><jtitle>arXiv.org</jtitle><date>2019-04-06</date><risdate>2019</risdate><eissn>2331-8422</eissn><abstract>Complex oxides with tunable structures have many fascinating properties, though high-quality complex oxide epitaxy with precisely controlled composition is still out of reach. 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| subjects | Calcium titanate Composition Epitaxy Ferroelectricity Induced polarization Industrial applications Multiferroic materials Solid solutions |
| title | Solution Processed Large-scale Multiferroic Complex Oxide Epitaxy with Magnetically Switched Polarization |
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