Highly efficient removal of Cr(VI) and Cu(II) by biochar derived from Artemisia argyi stem
In this work, a novel biochar was prepared from the Artemisia argyi stem at 300 °C (AS300), 450 °C (AS450), and 600 °C (AS600). The structural properties of these biochars were characterized with various tools. The sorption kinetic processes of Cr(VI) and Cu(II) onto these biochars were better descr...
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| Veröffentlicht in: | Environmental science and pollution research international 2019-05, Vol.26 (13), p.13221-13234 |
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| creator | Song, Jianyang He, Qiulai Hu, Xiaoling Zhang, Wei Wang, Chunyan Chen, Rongfan Wang, Hongyu Mosa, Ahmed |
| description | In this work, a novel biochar was prepared from the
Artemisia argyi
stem at 300 °C (AS300), 450 °C (AS450), and 600 °C (AS600). The structural properties of these biochars were characterized with various tools. The sorption kinetic processes of Cr(VI) and Cu(II) onto these biochars were better described by the pseudo-second order. The sorption isotherm processes of Cr(VI) onto these biochars were better described by the Freundlich model while the adsorption processes of Cu(II) were consistent with the Langmuir model. Batch sorption experiments showed that AS600 had the maximum adsorption capacity to Cr(VI) and Cu(II) with 161.92 and 155.96 mg/g, respectively. AS600 was selected for the follow-up batch and dynamic adsorption experiments. Results showed that AS600 had larger adsorption capacity for Cr(VI) at lower pH while the larger adsorption capacity for Cu(II) was found at higher pH. The effect of ionic strength on the adsorption of Cu(II) by AS600 was greater than that on the adsorption of Cr(VI). Dynamic adsorption experiments showed that Cu(II) had a higher affinity for the adsorption sites on the AS600 compared with Cr(VI). The adsorption mechanisms mainly involved electrostatic attraction, ion exchange, pore filling, and chemical bonding effect.
Graphical abstract |
| doi_str_mv | 10.1007/s11356-019-04863-2 |
| format | Article |
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Artemisia argyi
stem at 300 °C (AS300), 450 °C (AS450), and 600 °C (AS600). The structural properties of these biochars were characterized with various tools. The sorption kinetic processes of Cr(VI) and Cu(II) onto these biochars were better described by the pseudo-second order. The sorption isotherm processes of Cr(VI) onto these biochars were better described by the Freundlich model while the adsorption processes of Cu(II) were consistent with the Langmuir model. Batch sorption experiments showed that AS600 had the maximum adsorption capacity to Cr(VI) and Cu(II) with 161.92 and 155.96 mg/g, respectively. AS600 was selected for the follow-up batch and dynamic adsorption experiments. Results showed that AS600 had larger adsorption capacity for Cr(VI) at lower pH while the larger adsorption capacity for Cu(II) was found at higher pH. The effect of ionic strength on the adsorption of Cu(II) by AS600 was greater than that on the adsorption of Cr(VI). Dynamic adsorption experiments showed that Cu(II) had a higher affinity for the adsorption sites on the AS600 compared with Cr(VI). The adsorption mechanisms mainly involved electrostatic attraction, ion exchange, pore filling, and chemical bonding effect.
Graphical abstract</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-019-04863-2</identifier><identifier>PMID: 30903476</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorption ; Aquatic Pollution ; Artemisia - chemistry ; Artemisia argyi ; Atmospheric Protection/Air Quality Control/Air Pollution ; Charcoal ; Charcoal - chemistry ; Chemical bonds ; Chromium ; Chromium - chemistry ; Copper ; Copper - chemistry ; Earth and Environmental Science ; Ecotoxicology ; Electrostatic properties ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Experiments ; Ion exchange ; Ionic strength ; Organic chemistry ; pH effects ; Research Article ; Sorption ; Waste Water Technology ; Water Management ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2019-05, Vol.26 (13), p.13221-13234</ispartof><rights>Springer-Verlag GmbH Germany, part of Springer Nature 2019</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, (2019). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c412t-ffed100c6d456a23dfa18fd46d9366e3508ede3dec54e082bf3608b51cc1f62d3</citedby><cites>FETCH-LOGICAL-c412t-ffed100c6d456a23dfa18fd46d9366e3508ede3dec54e082bf3608b51cc1f62d3</cites><orcidid>0000-0001-5475-579X</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-019-04863-2$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-019-04863-2$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/30903476$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Song, Jianyang</creatorcontrib><creatorcontrib>He, Qiulai</creatorcontrib><creatorcontrib>Hu, Xiaoling</creatorcontrib><creatorcontrib>Zhang, Wei</creatorcontrib><creatorcontrib>Wang, Chunyan</creatorcontrib><creatorcontrib>Chen, Rongfan</creatorcontrib><creatorcontrib>Wang, Hongyu</creatorcontrib><creatorcontrib>Mosa, Ahmed</creatorcontrib><title>Highly efficient removal of Cr(VI) and Cu(II) by biochar derived from Artemisia argyi stem</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>In this work, a novel biochar was prepared from the
Artemisia argyi
stem at 300 °C (AS300), 450 °C (AS450), and 600 °C (AS600). The structural properties of these biochars were characterized with various tools. The sorption kinetic processes of Cr(VI) and Cu(II) onto these biochars were better described by the pseudo-second order. The sorption isotherm processes of Cr(VI) onto these biochars were better described by the Freundlich model while the adsorption processes of Cu(II) were consistent with the Langmuir model. Batch sorption experiments showed that AS600 had the maximum adsorption capacity to Cr(VI) and Cu(II) with 161.92 and 155.96 mg/g, respectively. AS600 was selected for the follow-up batch and dynamic adsorption experiments. Results showed that AS600 had larger adsorption capacity for Cr(VI) at lower pH while the larger adsorption capacity for Cu(II) was found at higher pH. The effect of ionic strength on the adsorption of Cu(II) by AS600 was greater than that on the adsorption of Cr(VI). Dynamic adsorption experiments showed that Cu(II) had a higher affinity for the adsorption sites on the AS600 compared with Cr(VI). The adsorption mechanisms mainly involved electrostatic attraction, ion exchange, pore filling, and chemical bonding effect.
Graphical abstract</description><subject>Adsorption</subject><subject>Aquatic Pollution</subject><subject>Artemisia - chemistry</subject><subject>Artemisia argyi</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Charcoal</subject><subject>Charcoal - chemistry</subject><subject>Chemical bonds</subject><subject>Chromium</subject><subject>Chromium - chemistry</subject><subject>Copper</subject><subject>Copper - chemistry</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Electrostatic properties</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Experiments</subject><subject>Ion exchange</subject><subject>Ionic strength</subject><subject>Organic chemistry</subject><subject>pH effects</subject><subject>Research Article</subject><subject>Sorption</subject><subject>Waste Water 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efficient removal of Cr(VI) and Cu(II) by biochar derived from Artemisia argyi stem</title><author>Song, Jianyang ; He, Qiulai ; Hu, Xiaoling ; Zhang, Wei ; Wang, Chunyan ; Chen, Rongfan ; Wang, Hongyu ; Mosa, Ahmed</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c412t-ffed100c6d456a23dfa18fd46d9366e3508ede3dec54e082bf3608b51cc1f62d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Adsorption</topic><topic>Aquatic Pollution</topic><topic>Artemisia - chemistry</topic><topic>Artemisia argyi</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Charcoal</topic><topic>Charcoal - chemistry</topic><topic>Chemical bonds</topic><topic>Chromium</topic><topic>Chromium - chemistry</topic><topic>Copper</topic><topic>Copper - chemistry</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Electrostatic properties</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental science</topic><topic>Experiments</topic><topic>Ion exchange</topic><topic>Ionic strength</topic><topic>Organic chemistry</topic><topic>pH effects</topic><topic>Research Article</topic><topic>Sorption</topic><topic>Waste Water Technology</topic><topic>Water Management</topic><topic>Water Pollution Control</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Song, Jianyang</creatorcontrib><creatorcontrib>He, Qiulai</creatorcontrib><creatorcontrib>Hu, Xiaoling</creatorcontrib><creatorcontrib>Zhang, Wei</creatorcontrib><creatorcontrib>Wang, Chunyan</creatorcontrib><creatorcontrib>Chen, Rongfan</creatorcontrib><creatorcontrib>Wang, Hongyu</creatorcontrib><creatorcontrib>Mosa, Ahmed</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE 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Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2019-05-01</date><risdate>2019</risdate><volume>26</volume><issue>13</issue><spage>13221</spage><epage>13234</epage><pages>13221-13234</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>In this work, a novel biochar was prepared from the
Artemisia argyi
stem at 300 °C (AS300), 450 °C (AS450), and 600 °C (AS600). The structural properties of these biochars were characterized with various tools. The sorption kinetic processes of Cr(VI) and Cu(II) onto these biochars were better described by the pseudo-second order. The sorption isotherm processes of Cr(VI) onto these biochars were better described by the Freundlich model while the adsorption processes of Cu(II) were consistent with the Langmuir model. Batch sorption experiments showed that AS600 had the maximum adsorption capacity to Cr(VI) and Cu(II) with 161.92 and 155.96 mg/g, respectively. AS600 was selected for the follow-up batch and dynamic adsorption experiments. Results showed that AS600 had larger adsorption capacity for Cr(VI) at lower pH while the larger adsorption capacity for Cu(II) was found at higher pH. The effect of ionic strength on the adsorption of Cu(II) by AS600 was greater than that on the adsorption of Cr(VI). Dynamic adsorption experiments showed that Cu(II) had a higher affinity for the adsorption sites on the AS600 compared with Cr(VI). The adsorption mechanisms mainly involved electrostatic attraction, ion exchange, pore filling, and chemical bonding effect.
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| subjects | Adsorption Aquatic Pollution Artemisia - chemistry Artemisia argyi Atmospheric Protection/Air Quality Control/Air Pollution Charcoal Charcoal - chemistry Chemical bonds Chromium Chromium - chemistry Copper Copper - chemistry Earth and Environmental Science Ecotoxicology Electrostatic properties Environment Environmental Chemistry Environmental Health Environmental science Experiments Ion exchange Ionic strength Organic chemistry pH effects Research Article Sorption Waste Water Technology Water Management Water Pollution Control |
| title | Highly efficient removal of Cr(VI) and Cu(II) by biochar derived from Artemisia argyi stem |
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