Negative muon capture ratios for nitrogen oxide molecules
Per-atom muon capture ratios are precisely determined from characteristic muonic X-ray measurements of three nitrogen oxide samples (NO, N 2 O, and NO 2 ) at pressures below 100 kPa. A higher density of covalent electrons at the N atoms relative to the O atoms is required if we explain the experimen...
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| Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2019-03, Vol.319 (3), p.767-773 |
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| container_title | Journal of radioanalytical and nuclear chemistry |
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| creator | Ninomiya, Kazuhiko Ito, Takashi U. Higemoto, Wataru Kawamura, Naritoshi Strasser, Patrick Nagatomo, Takashi Shimomura, Koichiro Miyake, Yasuhiro Kita, Makoto Shinohara, Atsushi Kubo, Kenya M. Miura, Taichi |
| description | Per-atom muon capture ratios are precisely determined from characteristic muonic X-ray measurements of three nitrogen oxide samples (NO, N
2
O, and NO
2
) at pressures below 100 kPa. A higher density of covalent electrons at the N atoms relative to the O atoms is required if we explain the experimental results using the proposed muon capture models. From molecular orbit calculations, we found that the electron distributions of only the highest occupied molecular orbitals (HOMO) are dominant at the N atoms, and the electrons in the HOMO significantly contribute to the muon capture phenomena in the nitrogen oxide molecules. |
| doi_str_mv | 10.1007/s10967-018-6366-3 |
| format | Article |
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2
O, and NO
2
) at pressures below 100 kPa. A higher density of covalent electrons at the N atoms relative to the O atoms is required if we explain the experimental results using the proposed muon capture models. From molecular orbit calculations, we found that the electron distributions of only the highest occupied molecular orbitals (HOMO) are dominant at the N atoms, and the electrons in the HOMO significantly contribute to the muon capture phenomena in the nitrogen oxide molecules.</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-018-6366-3</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Chemistry ; Chemistry and Materials Science ; Diagnostic Radiology ; Electrons ; Hadrons ; Heavy Ions ; Inorganic Chemistry ; Molecular orbitals ; Muons ; Nitrogen ; Nitrogen (Chemical element) ; Nitrogen dioxide ; Nitrogen oxides ; Nuclear Chemistry ; Nuclear energy ; Nuclear Physics ; Nuclear reactors ; Physical Chemistry</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2019-03, Vol.319 (3), p.767-773</ispartof><rights>Akadémiai Kiadó, Budapest, Hungary 2018</rights><rights>COPYRIGHT 2019 Springer</rights><rights>Copyright Springer Nature B.V. 2019</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c355t-3af870d89a6a751263d92cd2f478b532687c4c585f99897172dd9359688b76563</citedby><cites>FETCH-LOGICAL-c355t-3af870d89a6a751263d92cd2f478b532687c4c585f99897172dd9359688b76563</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10967-018-6366-3$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10967-018-6366-3$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Ninomiya, Kazuhiko</creatorcontrib><creatorcontrib>Ito, Takashi U.</creatorcontrib><creatorcontrib>Higemoto, Wataru</creatorcontrib><creatorcontrib>Kawamura, Naritoshi</creatorcontrib><creatorcontrib>Strasser, Patrick</creatorcontrib><creatorcontrib>Nagatomo, Takashi</creatorcontrib><creatorcontrib>Shimomura, Koichiro</creatorcontrib><creatorcontrib>Miyake, Yasuhiro</creatorcontrib><creatorcontrib>Kita, Makoto</creatorcontrib><creatorcontrib>Shinohara, Atsushi</creatorcontrib><creatorcontrib>Kubo, Kenya M.</creatorcontrib><creatorcontrib>Miura, Taichi</creatorcontrib><title>Negative muon capture ratios for nitrogen oxide molecules</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>Per-atom muon capture ratios are precisely determined from characteristic muonic X-ray measurements of three nitrogen oxide samples (NO, N
2
O, and NO
2
) at pressures below 100 kPa. A higher density of covalent electrons at the N atoms relative to the O atoms is required if we explain the experimental results using the proposed muon capture models. From molecular orbit calculations, we found that the electron distributions of only the highest occupied molecular orbitals (HOMO) are dominant at the N atoms, and the electrons in the HOMO significantly contribute to the muon capture phenomena in the nitrogen oxide molecules.</description><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Diagnostic Radiology</subject><subject>Electrons</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>Inorganic Chemistry</subject><subject>Molecular orbitals</subject><subject>Muons</subject><subject>Nitrogen</subject><subject>Nitrogen (Chemical element)</subject><subject>Nitrogen dioxide</subject><subject>Nitrogen oxides</subject><subject>Nuclear Chemistry</subject><subject>Nuclear energy</subject><subject>Nuclear Physics</subject><subject>Nuclear reactors</subject><subject>Physical Chemistry</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNp1kE1LAzEQhoMoWKs_wNuC59R8NMnkWIpaoehFzyHNJsuW7aYmu6L_3pQVPMkcBobnmRlehG4pWVBC1H2mREuFCQUsuZSYn6EZFQCYKSDnaEYYl1goTi_RVc57QogG4DOkX3xjh_bTV4cx9pWzx2FMvkplFnMVYqr6dkix8X0Vv9q6YLHzbux8vkYXwXbZ3_z2OXp_fHhbb_D29el5vdpix4UYMLcBFKlBW2mVoEzyWjNXs7BUsBOcSVBu6QSIoDVoRRWra82FlgA7JYXkc3Q37T2m-DH6PJh9HFNfThpGQSrGGGWFWkxUYztv2j7EIVlXqvaH1sXeh7bMV0JJJiksVRHoJLgUc04-mGNqDzZ9G0rMKVIzRWpKpOYUqeHFYZOTC9s3Pv298r_0A84idus</recordid><startdate>20190301</startdate><enddate>20190301</enddate><creator>Ninomiya, Kazuhiko</creator><creator>Ito, Takashi U.</creator><creator>Higemoto, Wataru</creator><creator>Kawamura, Naritoshi</creator><creator>Strasser, Patrick</creator><creator>Nagatomo, Takashi</creator><creator>Shimomura, Koichiro</creator><creator>Miyake, Yasuhiro</creator><creator>Kita, Makoto</creator><creator>Shinohara, Atsushi</creator><creator>Kubo, Kenya M.</creator><creator>Miura, Taichi</creator><general>Springer International Publishing</general><general>Springer</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20190301</creationdate><title>Negative muon capture ratios for nitrogen oxide molecules</title><author>Ninomiya, Kazuhiko ; 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2
O, and NO
2
) at pressures below 100 kPa. A higher density of covalent electrons at the N atoms relative to the O atoms is required if we explain the experimental results using the proposed muon capture models. From molecular orbit calculations, we found that the electron distributions of only the highest occupied molecular orbitals (HOMO) are dominant at the N atoms, and the electrons in the HOMO significantly contribute to the muon capture phenomena in the nitrogen oxide molecules.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s10967-018-6366-3</doi><tpages>7</tpages></addata></record> |
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| subjects | Chemistry Chemistry and Materials Science Diagnostic Radiology Electrons Hadrons Heavy Ions Inorganic Chemistry Molecular orbitals Muons Nitrogen Nitrogen (Chemical element) Nitrogen dioxide Nitrogen oxides Nuclear Chemistry Nuclear energy Nuclear Physics Nuclear reactors Physical Chemistry |
| title | Negative muon capture ratios for nitrogen oxide molecules |
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