Metal–nonmetal nanoarchitectures: quaternary PtPdNiP mesoporous nanospheres for enhanced oxygen reduction electrocatalysis
The controllable synthesis of mesoporous Pt-based catalysts with designed compositions is highly desired for the oxygen reduction reaction (ORR). In this work, we look beyond the traditional Pt-based all-metal alloys and fabricate quaternary PtPdNiP mesoporous nanospheres (PtPdNiP MNs) using a facil...
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Veröffentlicht in: | Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2019, Vol.7 (8), p.3910-3916 |
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container_title | Journal of materials chemistry. A, Materials for energy and sustainability |
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creator | Li, Chunjie Xu, You Deng, Kai Yin, Shuli Wang, Ziqiang Xue, Hairong Li, Xiaonian Wang, Liang Wang, Hongjing |
description | The controllable synthesis of mesoporous Pt-based catalysts with designed compositions is highly desired for the oxygen reduction reaction (ORR). In this work, we look beyond the traditional Pt-based all-metal alloys and fabricate quaternary PtPdNiP mesoporous nanospheres (PtPdNiP MNs) using a facile two-step strategy. Benefitting from their mesoporous nanoarchitectures and composition effect, the as-fabricated PtPdNiP MNs exhibit superior catalytic activity and durability for the ORR. The proposed synthetic strategy is highly feasible for the fabrication of metal–nonmetal nanoarchitectures with designed structures and controlled compositions. |
doi_str_mv | 10.1039/C8TA09620A |
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In this work, we look beyond the traditional Pt-based all-metal alloys and fabricate quaternary PtPdNiP mesoporous nanospheres (PtPdNiP MNs) using a facile two-step strategy. Benefitting from their mesoporous nanoarchitectures and composition effect, the as-fabricated PtPdNiP MNs exhibit superior catalytic activity and durability for the ORR. The proposed synthetic strategy is highly feasible for the fabrication of metal–nonmetal nanoarchitectures with designed structures and controlled compositions.</description><identifier>ISSN: 2050-7488</identifier><identifier>EISSN: 2050-7496</identifier><identifier>DOI: 10.1039/C8TA09620A</identifier><language>eng</language><publisher>Cambridge: Royal Society of Chemistry</publisher><subject>Catalysis ; Catalysts ; Catalytic activity ; Chemical reduction ; Chemical synthesis ; Composition effects ; Durability ; Fabrication ; Metals ; Nanospheres ; Oxygen ; Oxygen reduction reactions ; Platinum ; Stability</subject><ispartof>Journal of materials chemistry. 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A, Materials for energy and sustainability</title><description>The controllable synthesis of mesoporous Pt-based catalysts with designed compositions is highly desired for the oxygen reduction reaction (ORR). In this work, we look beyond the traditional Pt-based all-metal alloys and fabricate quaternary PtPdNiP mesoporous nanospheres (PtPdNiP MNs) using a facile two-step strategy. Benefitting from their mesoporous nanoarchitectures and composition effect, the as-fabricated PtPdNiP MNs exhibit superior catalytic activity and durability for the ORR. The proposed synthetic strategy is highly feasible for the fabrication of metal–nonmetal nanoarchitectures with designed structures and controlled compositions.</description><subject>Catalysis</subject><subject>Catalysts</subject><subject>Catalytic activity</subject><subject>Chemical reduction</subject><subject>Chemical synthesis</subject><subject>Composition effects</subject><subject>Durability</subject><subject>Fabrication</subject><subject>Metals</subject><subject>Nanospheres</subject><subject>Oxygen</subject><subject>Oxygen reduction reactions</subject><subject>Platinum</subject><subject>Stability</subject><issn>2050-7488</issn><issn>2050-7496</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNpFkM1KAzEUhYMoWLQbnyDgThhNJvOTuCvFP6jaRV0PmeSOnTJNpkkGLLjwHXxDn8TUit7NPYvvnss5CJ1RckkJE1dTvpgQUaRkcoBGKclJUmaiOPzTnB-jsfcrEocTUggxQu-PEGT39fFprFnvJDbSWOnUsg2gwuDAX-PNIAM4I90Wz8NcP7VzvAZve-vs4H8OfL-EiOLGOgxmKY0Cje3b9hUMdqAHFVprMHTR0lkl45-tb_0pOmpk52H8u0_Qy-3NYnqfzJ7vHqaTWaJYUYRESkmpllyRRtcAOS1ZWjPGSs102SgqWMGZpKTmdaZyrnVORVqWQmY5rcsM2Ak63_v2zm4G8KFa2SHm6XyVUs5YQfM8jdTFnlLOeu-gqXrXrmPoipJqV3D1XzD7BoqDccM</recordid><startdate>2019</startdate><enddate>2019</enddate><creator>Li, Chunjie</creator><creator>Xu, You</creator><creator>Deng, Kai</creator><creator>Yin, Shuli</creator><creator>Wang, Ziqiang</creator><creator>Xue, Hairong</creator><creator>Li, Xiaonian</creator><creator>Wang, Liang</creator><creator>Wang, Hongjing</creator><general>Royal Society of Chemistry</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>7ST</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>C1K</scope><scope>JG9</scope><scope>L7M</scope><scope>SOI</scope><orcidid>https://orcid.org/0000-0001-7375-8478</orcidid><orcidid>https://orcid.org/0000-0002-2979-9456</orcidid><orcidid>https://orcid.org/0000-0003-0641-3909</orcidid><orcidid>https://orcid.org/0000-0003-0735-201X</orcidid><orcidid>https://orcid.org/0000-0003-3856-4138</orcidid></search><sort><creationdate>2019</creationdate><title>Metal–nonmetal nanoarchitectures: quaternary PtPdNiP mesoporous nanospheres for enhanced oxygen reduction electrocatalysis</title><author>Li, Chunjie ; Xu, You ; Deng, Kai ; Yin, Shuli ; Wang, Ziqiang ; Xue, Hairong ; Li, Xiaonian ; Wang, Liang ; Wang, Hongjing</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c366t-aaa11da8c0fdbee51732b3337d3d7fc193683a10b8b4c58dd5192779a451b74e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Catalysis</topic><topic>Catalysts</topic><topic>Catalytic activity</topic><topic>Chemical reduction</topic><topic>Chemical synthesis</topic><topic>Composition effects</topic><topic>Durability</topic><topic>Fabrication</topic><topic>Metals</topic><topic>Nanospheres</topic><topic>Oxygen</topic><topic>Oxygen reduction reactions</topic><topic>Platinum</topic><topic>Stability</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Chunjie</creatorcontrib><creatorcontrib>Xu, You</creatorcontrib><creatorcontrib>Deng, Kai</creatorcontrib><creatorcontrib>Yin, Shuli</creatorcontrib><creatorcontrib>Wang, Ziqiang</creatorcontrib><creatorcontrib>Xue, Hairong</creatorcontrib><creatorcontrib>Li, Xiaonian</creatorcontrib><creatorcontrib>Wang, Liang</creatorcontrib><creatorcontrib>Wang, Hongjing</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Environment Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Environment Abstracts</collection><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Chunjie</au><au>Xu, You</au><au>Deng, Kai</au><au>Yin, Shuli</au><au>Wang, Ziqiang</au><au>Xue, Hairong</au><au>Li, Xiaonian</au><au>Wang, Liang</au><au>Wang, Hongjing</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Metal–nonmetal nanoarchitectures: quaternary PtPdNiP mesoporous nanospheres for enhanced oxygen reduction electrocatalysis</atitle><jtitle>Journal of materials chemistry. A, Materials for energy and sustainability</jtitle><date>2019</date><risdate>2019</risdate><volume>7</volume><issue>8</issue><spage>3910</spage><epage>3916</epage><pages>3910-3916</pages><issn>2050-7488</issn><eissn>2050-7496</eissn><abstract>The controllable synthesis of mesoporous Pt-based catalysts with designed compositions is highly desired for the oxygen reduction reaction (ORR). In this work, we look beyond the traditional Pt-based all-metal alloys and fabricate quaternary PtPdNiP mesoporous nanospheres (PtPdNiP MNs) using a facile two-step strategy. Benefitting from their mesoporous nanoarchitectures and composition effect, the as-fabricated PtPdNiP MNs exhibit superior catalytic activity and durability for the ORR. The proposed synthetic strategy is highly feasible for the fabrication of metal–nonmetal nanoarchitectures with designed structures and controlled compositions.</abstract><cop>Cambridge</cop><pub>Royal Society of Chemistry</pub><doi>10.1039/C8TA09620A</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0001-7375-8478</orcidid><orcidid>https://orcid.org/0000-0002-2979-9456</orcidid><orcidid>https://orcid.org/0000-0003-0641-3909</orcidid><orcidid>https://orcid.org/0000-0003-0735-201X</orcidid><orcidid>https://orcid.org/0000-0003-3856-4138</orcidid></addata></record> |
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source | Royal Society Of Chemistry Journals 2008- |
subjects | Catalysis Catalysts Catalytic activity Chemical reduction Chemical synthesis Composition effects Durability Fabrication Metals Nanospheres Oxygen Oxygen reduction reactions Platinum Stability |
title | Metal–nonmetal nanoarchitectures: quaternary PtPdNiP mesoporous nanospheres for enhanced oxygen reduction electrocatalysis |
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