Highly adsorptive chitosan/saponin-bentonite composite film for removal of methyl orange and Cr(VI)
Robust and simple composite films for the removal of methyl orange (MO) and Cr(VI) have been prepared by combining chitosan, saponin, and bentonite at a specific ratio. There are several composite films (chitosan-saponin-bentonite (CSB)) prepared; among them, the composite films CSB 2:3 and CSB 1:1...
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| Veröffentlicht in: | Environmental science and pollution research international 2019-02, Vol.26 (5), p.5020-5037 |
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| creator | Laysandra, Livy Ondang, Immanuel Joseph Ju, Yi-Hsu Ariandini, Benedikta Hervina Mariska, Agatha Soetaredjo, Felycia Edi Putro, Jindrayani Nyoo Santoso, Shella Permatasari Darsono, Farida Lanawati Ismadji, Suryadi |
| description | Robust and simple composite films for the removal of methyl orange (MO) and Cr(VI) have been prepared by combining chitosan, saponin, and bentonite at a specific ratio. There are several composite films (chitosan-saponin-bentonite (CSB)) prepared; among them, the composite films CSB
2:3
and CSB
1:1
have the highest removal efficiency toward MO and Cr(VI) where the maximum removal is 70.4% (pH 4.80) and 92.3% (pH 5.30), respectively. It was found that different types of adsorbate have different thermodynamic properties of the adsorption process; the adsorption of MO onto CSB
2:3
, chitosan, and acid-activated bentonite (AAB) proceeded endothermically, while the adsorption of Cr(VI) onto CSB
1:1
, chitosan, and AAB proceeded exothermically. The parameters of the adsorption were modeled by using isotherm and kinetic equations. The models of Langmuir, Freundlich, Redlich-Peterson, Sips, and Toth were used for fitting the adsorption isotherm data at a temperature of 30, 45, and 60 °C; all of the isotherm models could represent the data well. The result indicates that CSB
2:3
has the highest adsorption capacity toward MO with
q
m
of 360.90 mg g
−1
at 60 °C; meanwhile, CSB
1:1
has the highest adsorption capacity toward Cr(VI) with
q
m
641.99 mg g
−1
at 30 °C. The pseudo-second-order model could represent the adsorption kinetics data better than the pseudo-first-order equation. The adsorption mechanism was proposed, and the thermodynamic properties of the adsorption were also studied. |
| doi_str_mv | 10.1007/s11356-018-4035-2 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2162262487</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2162262487</sourcerecordid><originalsourceid>FETCH-LOGICAL-c411t-4839d769a6160925c0a361ae9abb0f6d16f42d43c17aa94abf32fdc8aa8f29cd3</originalsourceid><addsrcrecordid>eNp1kMtOwzAQRS0EgvL4ADYoEhtYGDy268RLVAGtVIkNsLUmiU1TNXGw00r9e1yVx4rVXGnu3Jk5hFwCuwPG8vsIIMaKMiioZGJM-QEZgQJJc6n1IRkxLSUFIeUJOY1xyRhnmufH5EQwxZjUMCLVtPlYrLYZ1tGHfmg2NqsWzeAjdvcRe981HS1tNyQxpJZvex93yjWrNnM-ZMG2foOrzLustcNim1TA7sNm2NXZJNy8z27PyZHDVbQX3_WMvD09vk6mdP7yPJs8zGklAQYqC6HrXGlUoNKd44qhUIBWY1kyp2pQTvJaigpyRC2xdIK7uioQC8d1VYszcr3P7YP_XNs4mKVfhy6tNBwU54rLIk8u2Luq4GMM1pk-NC2GrQFmdljNHqtJWM0Oq-Fp5uo7eV22tv6d-OGYDHxviKmVvg9_q_9P_QKi4oNE</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2162262487</pqid></control><display><type>article</type><title>Highly adsorptive chitosan/saponin-bentonite composite film for removal of methyl orange and Cr(VI)</title><source>MEDLINE</source><source>Springer Nature - Complete Springer Journals</source><creator>Laysandra, Livy ; Ondang, Immanuel Joseph ; Ju, Yi-Hsu ; Ariandini, Benedikta Hervina ; Mariska, Agatha ; Soetaredjo, Felycia Edi ; Putro, Jindrayani Nyoo ; Santoso, Shella Permatasari ; Darsono, Farida Lanawati ; Ismadji, Suryadi</creator><creatorcontrib>Laysandra, Livy ; Ondang, Immanuel Joseph ; Ju, Yi-Hsu ; Ariandini, Benedikta Hervina ; Mariska, Agatha ; Soetaredjo, Felycia Edi ; Putro, Jindrayani Nyoo ; Santoso, Shella Permatasari ; Darsono, Farida Lanawati ; Ismadji, Suryadi</creatorcontrib><description>Robust and simple composite films for the removal of methyl orange (MO) and Cr(VI) have been prepared by combining chitosan, saponin, and bentonite at a specific ratio. There are several composite films (chitosan-saponin-bentonite (CSB)) prepared; among them, the composite films CSB
2:3
and CSB
1:1
have the highest removal efficiency toward MO and Cr(VI) where the maximum removal is 70.4% (pH 4.80) and 92.3% (pH 5.30), respectively. It was found that different types of adsorbate have different thermodynamic properties of the adsorption process; the adsorption of MO onto CSB
2:3
, chitosan, and acid-activated bentonite (AAB) proceeded endothermically, while the adsorption of Cr(VI) onto CSB
1:1
, chitosan, and AAB proceeded exothermically. The parameters of the adsorption were modeled by using isotherm and kinetic equations. The models of Langmuir, Freundlich, Redlich-Peterson, Sips, and Toth were used for fitting the adsorption isotherm data at a temperature of 30, 45, and 60 °C; all of the isotherm models could represent the data well. The result indicates that CSB
2:3
has the highest adsorption capacity toward MO with
q
m
of 360.90 mg g
−1
at 60 °C; meanwhile, CSB
1:1
has the highest adsorption capacity toward Cr(VI) with
q
m
641.99 mg g
−1
at 30 °C. The pseudo-second-order model could represent the adsorption kinetics data better than the pseudo-first-order equation. The adsorption mechanism was proposed, and the thermodynamic properties of the adsorption were also studied.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-018-4035-2</identifier><identifier>PMID: 30600491</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorbates ; Adsorption ; Adsorptivity ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Azo Compounds - analysis ; Bentonite ; Bentonite - chemistry ; Chitosan ; Chitosan - chemistry ; Chromium ; Chromium - analysis ; Dyes ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Hydrogen-Ion Concentration ; Isotherms ; Kinetic equations ; Kinetics ; Linear equations ; pH effects ; Research Article ; Saponins - chemistry ; Surface Properties ; Temperature ; Thermodynamic properties ; Thermodynamics ; Waste Water Technology ; Water Management ; Water Pollutants, Chemical - analysis ; Water Pollution Control ; Water Purification - methods</subject><ispartof>Environmental science and pollution research international, 2019-02, Vol.26 (5), p.5020-5037</ispartof><rights>Springer-Verlag GmbH Germany, part of Springer Nature 2019</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, (2019). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c411t-4839d769a6160925c0a361ae9abb0f6d16f42d43c17aa94abf32fdc8aa8f29cd3</citedby><cites>FETCH-LOGICAL-c411t-4839d769a6160925c0a361ae9abb0f6d16f42d43c17aa94abf32fdc8aa8f29cd3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-018-4035-2$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-018-4035-2$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/30600491$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Laysandra, Livy</creatorcontrib><creatorcontrib>Ondang, Immanuel Joseph</creatorcontrib><creatorcontrib>Ju, Yi-Hsu</creatorcontrib><creatorcontrib>Ariandini, Benedikta Hervina</creatorcontrib><creatorcontrib>Mariska, Agatha</creatorcontrib><creatorcontrib>Soetaredjo, Felycia Edi</creatorcontrib><creatorcontrib>Putro, Jindrayani Nyoo</creatorcontrib><creatorcontrib>Santoso, Shella Permatasari</creatorcontrib><creatorcontrib>Darsono, Farida Lanawati</creatorcontrib><creatorcontrib>Ismadji, Suryadi</creatorcontrib><title>Highly adsorptive chitosan/saponin-bentonite composite film for removal of methyl orange and Cr(VI)</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Robust and simple composite films for the removal of methyl orange (MO) and Cr(VI) have been prepared by combining chitosan, saponin, and bentonite at a specific ratio. There are several composite films (chitosan-saponin-bentonite (CSB)) prepared; among them, the composite films CSB
2:3
and CSB
1:1
have the highest removal efficiency toward MO and Cr(VI) where the maximum removal is 70.4% (pH 4.80) and 92.3% (pH 5.30), respectively. It was found that different types of adsorbate have different thermodynamic properties of the adsorption process; the adsorption of MO onto CSB
2:3
, chitosan, and acid-activated bentonite (AAB) proceeded endothermically, while the adsorption of Cr(VI) onto CSB
1:1
, chitosan, and AAB proceeded exothermically. The parameters of the adsorption were modeled by using isotherm and kinetic equations. The models of Langmuir, Freundlich, Redlich-Peterson, Sips, and Toth were used for fitting the adsorption isotherm data at a temperature of 30, 45, and 60 °C; all of the isotherm models could represent the data well. The result indicates that CSB
2:3
has the highest adsorption capacity toward MO with
q
m
of 360.90 mg g
−1
at 60 °C; meanwhile, CSB
1:1
has the highest adsorption capacity toward Cr(VI) with
q
m
641.99 mg g
−1
at 30 °C. The pseudo-second-order model could represent the adsorption kinetics data better than the pseudo-first-order equation. The adsorption mechanism was proposed, and the thermodynamic properties of the adsorption were also studied.</description><subject>Adsorbates</subject><subject>Adsorption</subject><subject>Adsorptivity</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Azo Compounds - analysis</subject><subject>Bentonite</subject><subject>Bentonite - chemistry</subject><subject>Chitosan</subject><subject>Chitosan - chemistry</subject><subject>Chromium</subject><subject>Chromium - analysis</subject><subject>Dyes</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Hydrogen-Ion Concentration</subject><subject>Isotherms</subject><subject>Kinetic equations</subject><subject>Kinetics</subject><subject>Linear equations</subject><subject>pH effects</subject><subject>Research Article</subject><subject>Saponins - chemistry</subject><subject>Surface Properties</subject><subject>Temperature</subject><subject>Thermodynamic properties</subject><subject>Thermodynamics</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollutants, Chemical - analysis</subject><subject>Water Pollution Control</subject><subject>Water Purification - methods</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>BENPR</sourceid><recordid>eNp1kMtOwzAQRS0EgvL4ADYoEhtYGDy268RLVAGtVIkNsLUmiU1TNXGw00r9e1yVx4rVXGnu3Jk5hFwCuwPG8vsIIMaKMiioZGJM-QEZgQJJc6n1IRkxLSUFIeUJOY1xyRhnmufH5EQwxZjUMCLVtPlYrLYZ1tGHfmg2NqsWzeAjdvcRe981HS1tNyQxpJZvex93yjWrNnM-ZMG2foOrzLustcNim1TA7sNm2NXZJNy8z27PyZHDVbQX3_WMvD09vk6mdP7yPJs8zGklAQYqC6HrXGlUoNKd44qhUIBWY1kyp2pQTvJaigpyRC2xdIK7uioQC8d1VYszcr3P7YP_XNs4mKVfhy6tNBwU54rLIk8u2Luq4GMM1pk-NC2GrQFmdljNHqtJWM0Oq-Fp5uo7eV22tv6d-OGYDHxviKmVvg9_q_9P_QKi4oNE</recordid><startdate>20190201</startdate><enddate>20190201</enddate><creator>Laysandra, Livy</creator><creator>Ondang, Immanuel Joseph</creator><creator>Ju, Yi-Hsu</creator><creator>Ariandini, Benedikta Hervina</creator><creator>Mariska, Agatha</creator><creator>Soetaredjo, Felycia Edi</creator><creator>Putro, 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adsorptive chitosan/saponin-bentonite composite film for removal of methyl orange and Cr(VI)</title><author>Laysandra, Livy ; Ondang, Immanuel Joseph ; Ju, Yi-Hsu ; Ariandini, Benedikta Hervina ; Mariska, Agatha ; Soetaredjo, Felycia Edi ; Putro, Jindrayani Nyoo ; Santoso, Shella Permatasari ; Darsono, Farida Lanawati ; Ismadji, Suryadi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c411t-4839d769a6160925c0a361ae9abb0f6d16f42d43c17aa94abf32fdc8aa8f29cd3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Adsorbates</topic><topic>Adsorption</topic><topic>Adsorptivity</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Azo Compounds - analysis</topic><topic>Bentonite</topic><topic>Bentonite - chemistry</topic><topic>Chitosan</topic><topic>Chitosan - chemistry</topic><topic>Chromium</topic><topic>Chromium - analysis</topic><topic>Dyes</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental science</topic><topic>Hydrogen-Ion Concentration</topic><topic>Isotherms</topic><topic>Kinetic equations</topic><topic>Kinetics</topic><topic>Linear equations</topic><topic>pH effects</topic><topic>Research Article</topic><topic>Saponins - chemistry</topic><topic>Surface Properties</topic><topic>Temperature</topic><topic>Thermodynamic properties</topic><topic>Thermodynamics</topic><topic>Waste Water Technology</topic><topic>Water Management</topic><topic>Water Pollutants, Chemical - analysis</topic><topic>Water Pollution Control</topic><topic>Water Purification - methods</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Laysandra, Livy</creatorcontrib><creatorcontrib>Ondang, Immanuel 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international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Laysandra, Livy</au><au>Ondang, Immanuel Joseph</au><au>Ju, Yi-Hsu</au><au>Ariandini, Benedikta Hervina</au><au>Mariska, Agatha</au><au>Soetaredjo, Felycia Edi</au><au>Putro, Jindrayani Nyoo</au><au>Santoso, Shella Permatasari</au><au>Darsono, Farida Lanawati</au><au>Ismadji, Suryadi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Highly adsorptive chitosan/saponin-bentonite composite film for removal of methyl orange and Cr(VI)</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2019-02-01</date><risdate>2019</risdate><volume>26</volume><issue>5</issue><spage>5020</spage><epage>5037</epage><pages>5020-5037</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Robust and simple composite films for the removal of methyl orange (MO) and Cr(VI) have been prepared by combining chitosan, saponin, and bentonite at a specific ratio. There are several composite films (chitosan-saponin-bentonite (CSB)) prepared; among them, the composite films CSB
2:3
and CSB
1:1
have the highest removal efficiency toward MO and Cr(VI) where the maximum removal is 70.4% (pH 4.80) and 92.3% (pH 5.30), respectively. It was found that different types of adsorbate have different thermodynamic properties of the adsorption process; the adsorption of MO onto CSB
2:3
, chitosan, and acid-activated bentonite (AAB) proceeded endothermically, while the adsorption of Cr(VI) onto CSB
1:1
, chitosan, and AAB proceeded exothermically. The parameters of the adsorption were modeled by using isotherm and kinetic equations. The models of Langmuir, Freundlich, Redlich-Peterson, Sips, and Toth were used for fitting the adsorption isotherm data at a temperature of 30, 45, and 60 °C; all of the isotherm models could represent the data well. The result indicates that CSB
2:3
has the highest adsorption capacity toward MO with
q
m
of 360.90 mg g
−1
at 60 °C; meanwhile, CSB
1:1
has the highest adsorption capacity toward Cr(VI) with
q
m
641.99 mg g
−1
at 30 °C. The pseudo-second-order model could represent the adsorption kinetics data better than the pseudo-first-order equation. The adsorption mechanism was proposed, and the thermodynamic properties of the adsorption were also studied.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>30600491</pmid><doi>10.1007/s11356-018-4035-2</doi><tpages>18</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0944-1344 |
| ispartof | Environmental science and pollution research international, 2019-02, Vol.26 (5), p.5020-5037 |
| issn | 0944-1344 1614-7499 |
| language | eng |
| recordid | cdi_proquest_journals_2162262487 |
| source | MEDLINE; Springer Nature - Complete Springer Journals |
| subjects | Adsorbates Adsorption Adsorptivity Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Azo Compounds - analysis Bentonite Bentonite - chemistry Chitosan Chitosan - chemistry Chromium Chromium - analysis Dyes Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental science Hydrogen-Ion Concentration Isotherms Kinetic equations Kinetics Linear equations pH effects Research Article Saponins - chemistry Surface Properties Temperature Thermodynamic properties Thermodynamics Waste Water Technology Water Management Water Pollutants, Chemical - analysis Water Pollution Control Water Purification - methods |
| title | Highly adsorptive chitosan/saponin-bentonite composite film for removal of methyl orange and Cr(VI) |
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