Exploring of multicolor emissive carbon dots with novel double emission mechanism

Multicolor emissive carbon dots with novel double emission mechanism and the corresponding applications. [Display omitted] Multicolor emissive carbon dots (CDs) was successfully synthesized via a facile one-pot solvothermal method with the assistance of ethanol, which is nominated as E-CDs. In the r...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Sensors and actuators. B, Chemical Chemical, 2018-12, Vol.277, p.373-380
Hauptverfasser: Gao, Dong, Liu, Xiaolu, Jiang, Dongli, Zhao, Huan, Zhu, Yuda, Chen, Xiaoqin, Luo, Hongrong, Fan, Hongsong, Zhang, Xingdong
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 380
container_issue
container_start_page 373
container_title Sensors and actuators. B, Chemical
container_volume 277
creator Gao, Dong
Liu, Xiaolu
Jiang, Dongli
Zhao, Huan
Zhu, Yuda
Chen, Xiaoqin
Luo, Hongrong
Fan, Hongsong
Zhang, Xingdong
description Multicolor emissive carbon dots with novel double emission mechanism and the corresponding applications. [Display omitted] Multicolor emissive carbon dots (CDs) was successfully synthesized via a facile one-pot solvothermal method with the assistance of ethanol, which is nominated as E-CDs. In the reaction system, the addition of ethanol plays a key role in synthesizing CDs with higher proportion of amorphous structures, resulting in multicolor emission of the E-CDs after dissolved in various solvents. Moreover, this solvent dependent multicolor emission of the E-CDs is found to be ascribed to a novel double emission mechanism. The excitation dependent blue emissions stem from intrinsic surface/defect states of the E-CDs while the excitation independent long wavelength emissions originate from solvent molecules connected on the surface of the E-CDs via hydrogen bond. Noticeably, the hydrogen bond between the E-CDs and surrounding environment endows the prepared E-CDs with a unique pH-sensitive feature, which can be used to construct fluorescent pH sensor. Besides, based on this multicolor emission, the E-CDs show potential in bio-labeling, multicolor patterning and solid luminous materials.
doi_str_mv 10.1016/j.snb.2018.09.031
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2159258919</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><els_id>S0925400518316447</els_id><sourcerecordid>2159258919</sourcerecordid><originalsourceid>FETCH-LOGICAL-c325t-7eaa6f2333dc9d255a5e3592296798ee1fd32927cdb6f613de5c183eadb2523b3</originalsourceid><addsrcrecordid>eNp9kE9LxDAQxYMouK5-AG8Fz62TZNM2eJLFf7Aggp5DmkzdLG2zJu2q394su2dPw8y892b4EXJNoaBAy9tNEYemYEDrAmQBnJ6QGa0rnnOoqlMyA8lEvgAQ5-Qixg0ALHgJM_L28LPtfHDDZ-bbrJ-60RmfBhn2Lka3w8zo0Pghs36M2bcb19ngd9ilfmo6PMrSvkez1oOL_SU5a3UX8epY5-Tj8eF9-ZyvXp9elver3HAmxrxCrcuWcc6tkZYJoQVyIRmTZSVrRNpaziSrjG3KtqTcojC05qhtwwTjDZ-Tm0PuNvivCeOoNn4KQzqpGE1BopZUJhU9qEzwMQZs1Ta4XodfRUHtyamNSuTUnpwCqRK55Lk7eDC9v3MYVDQOB4PWBTSjst794_4Dyrl3VA</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2159258919</pqid></control><display><type>article</type><title>Exploring of multicolor emissive carbon dots with novel double emission mechanism</title><source>Elsevier ScienceDirect Journals</source><creator>Gao, Dong ; Liu, Xiaolu ; Jiang, Dongli ; Zhao, Huan ; Zhu, Yuda ; Chen, Xiaoqin ; Luo, Hongrong ; Fan, Hongsong ; Zhang, Xingdong</creator><creatorcontrib>Gao, Dong ; Liu, Xiaolu ; Jiang, Dongli ; Zhao, Huan ; Zhu, Yuda ; Chen, Xiaoqin ; Luo, Hongrong ; Fan, Hongsong ; Zhang, Xingdong</creatorcontrib><description>Multicolor emissive carbon dots with novel double emission mechanism and the corresponding applications. [Display omitted] Multicolor emissive carbon dots (CDs) was successfully synthesized via a facile one-pot solvothermal method with the assistance of ethanol, which is nominated as E-CDs. In the reaction system, the addition of ethanol plays a key role in synthesizing CDs with higher proportion of amorphous structures, resulting in multicolor emission of the E-CDs after dissolved in various solvents. Moreover, this solvent dependent multicolor emission of the E-CDs is found to be ascribed to a novel double emission mechanism. The excitation dependent blue emissions stem from intrinsic surface/defect states of the E-CDs while the excitation independent long wavelength emissions originate from solvent molecules connected on the surface of the E-CDs via hydrogen bond. Noticeably, the hydrogen bond between the E-CDs and surrounding environment endows the prepared E-CDs with a unique pH-sensitive feature, which can be used to construct fluorescent pH sensor. Besides, based on this multicolor emission, the E-CDs show potential in bio-labeling, multicolor patterning and solid luminous materials.</description><identifier>ISSN: 0925-4005</identifier><identifier>EISSN: 1873-3077</identifier><identifier>DOI: 10.1016/j.snb.2018.09.031</identifier><language>eng</language><publisher>Lausanne: Elsevier B.V</publisher><subject>Carbon dots ; Cell labeling ; Chemical synthesis ; Emission ; Emissions ; Ethanol ; Ethanol-assisted synthesis ; Excitation ; Fluorescence ; Fluorescent pH sensor ; Hydrogen bonds ; multicolor emission ; Novel double emission mechanism ; Sensors ; Solvents</subject><ispartof>Sensors and actuators. B, Chemical, 2018-12, Vol.277, p.373-380</ispartof><rights>2018 Elsevier B.V.</rights><rights>Copyright Elsevier Science Ltd. Dec 20, 2018</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c325t-7eaa6f2333dc9d255a5e3592296798ee1fd32927cdb6f613de5c183eadb2523b3</citedby><cites>FETCH-LOGICAL-c325t-7eaa6f2333dc9d255a5e3592296798ee1fd32927cdb6f613de5c183eadb2523b3</cites><orcidid>0000-0003-3812-9208</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0925400518316447$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3537,27901,27902,65306</link.rule.ids></links><search><creatorcontrib>Gao, Dong</creatorcontrib><creatorcontrib>Liu, Xiaolu</creatorcontrib><creatorcontrib>Jiang, Dongli</creatorcontrib><creatorcontrib>Zhao, Huan</creatorcontrib><creatorcontrib>Zhu, Yuda</creatorcontrib><creatorcontrib>Chen, Xiaoqin</creatorcontrib><creatorcontrib>Luo, Hongrong</creatorcontrib><creatorcontrib>Fan, Hongsong</creatorcontrib><creatorcontrib>Zhang, Xingdong</creatorcontrib><title>Exploring of multicolor emissive carbon dots with novel double emission mechanism</title><title>Sensors and actuators. B, Chemical</title><description>Multicolor emissive carbon dots with novel double emission mechanism and the corresponding applications. [Display omitted] Multicolor emissive carbon dots (CDs) was successfully synthesized via a facile one-pot solvothermal method with the assistance of ethanol, which is nominated as E-CDs. In the reaction system, the addition of ethanol plays a key role in synthesizing CDs with higher proportion of amorphous structures, resulting in multicolor emission of the E-CDs after dissolved in various solvents. Moreover, this solvent dependent multicolor emission of the E-CDs is found to be ascribed to a novel double emission mechanism. The excitation dependent blue emissions stem from intrinsic surface/defect states of the E-CDs while the excitation independent long wavelength emissions originate from solvent molecules connected on the surface of the E-CDs via hydrogen bond. Noticeably, the hydrogen bond between the E-CDs and surrounding environment endows the prepared E-CDs with a unique pH-sensitive feature, which can be used to construct fluorescent pH sensor. Besides, based on this multicolor emission, the E-CDs show potential in bio-labeling, multicolor patterning and solid luminous materials.</description><subject>Carbon dots</subject><subject>Cell labeling</subject><subject>Chemical synthesis</subject><subject>Emission</subject><subject>Emissions</subject><subject>Ethanol</subject><subject>Ethanol-assisted synthesis</subject><subject>Excitation</subject><subject>Fluorescence</subject><subject>Fluorescent pH sensor</subject><subject>Hydrogen bonds</subject><subject>multicolor emission</subject><subject>Novel double emission mechanism</subject><subject>Sensors</subject><subject>Solvents</subject><issn>0925-4005</issn><issn>1873-3077</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNp9kE9LxDAQxYMouK5-AG8Fz62TZNM2eJLFf7Aggp5DmkzdLG2zJu2q394su2dPw8y892b4EXJNoaBAy9tNEYemYEDrAmQBnJ6QGa0rnnOoqlMyA8lEvgAQ5-Qixg0ALHgJM_L28LPtfHDDZ-bbrJ-60RmfBhn2Lka3w8zo0Pghs36M2bcb19ngd9ilfmo6PMrSvkez1oOL_SU5a3UX8epY5-Tj8eF9-ZyvXp9elver3HAmxrxCrcuWcc6tkZYJoQVyIRmTZSVrRNpaziSrjG3KtqTcojC05qhtwwTjDZ-Tm0PuNvivCeOoNn4KQzqpGE1BopZUJhU9qEzwMQZs1Ta4XodfRUHtyamNSuTUnpwCqRK55Lk7eDC9v3MYVDQOB4PWBTSjst794_4Dyrl3VA</recordid><startdate>20181220</startdate><enddate>20181220</enddate><creator>Gao, Dong</creator><creator>Liu, Xiaolu</creator><creator>Jiang, Dongli</creator><creator>Zhao, Huan</creator><creator>Zhu, Yuda</creator><creator>Chen, Xiaoqin</creator><creator>Luo, Hongrong</creator><creator>Fan, Hongsong</creator><creator>Zhang, Xingdong</creator><general>Elsevier B.V</general><general>Elsevier Science Ltd</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>7TB</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>FR3</scope><scope>JG9</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0003-3812-9208</orcidid></search><sort><creationdate>20181220</creationdate><title>Exploring of multicolor emissive carbon dots with novel double emission mechanism</title><author>Gao, Dong ; Liu, Xiaolu ; Jiang, Dongli ; Zhao, Huan ; Zhu, Yuda ; Chen, Xiaoqin ; Luo, Hongrong ; Fan, Hongsong ; Zhang, Xingdong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c325t-7eaa6f2333dc9d255a5e3592296798ee1fd32927cdb6f613de5c183eadb2523b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Carbon dots</topic><topic>Cell labeling</topic><topic>Chemical synthesis</topic><topic>Emission</topic><topic>Emissions</topic><topic>Ethanol</topic><topic>Ethanol-assisted synthesis</topic><topic>Excitation</topic><topic>Fluorescence</topic><topic>Fluorescent pH sensor</topic><topic>Hydrogen bonds</topic><topic>multicolor emission</topic><topic>Novel double emission mechanism</topic><topic>Sensors</topic><topic>Solvents</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Gao, Dong</creatorcontrib><creatorcontrib>Liu, Xiaolu</creatorcontrib><creatorcontrib>Jiang, Dongli</creatorcontrib><creatorcontrib>Zhao, Huan</creatorcontrib><creatorcontrib>Zhu, Yuda</creatorcontrib><creatorcontrib>Chen, Xiaoqin</creatorcontrib><creatorcontrib>Luo, Hongrong</creatorcontrib><creatorcontrib>Fan, Hongsong</creatorcontrib><creatorcontrib>Zhang, Xingdong</creatorcontrib><collection>CrossRef</collection><collection>Electronics &amp; Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Mechanical &amp; Transportation Engineering Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Sensors and actuators. B, Chemical</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Gao, Dong</au><au>Liu, Xiaolu</au><au>Jiang, Dongli</au><au>Zhao, Huan</au><au>Zhu, Yuda</au><au>Chen, Xiaoqin</au><au>Luo, Hongrong</au><au>Fan, Hongsong</au><au>Zhang, Xingdong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Exploring of multicolor emissive carbon dots with novel double emission mechanism</atitle><jtitle>Sensors and actuators. B, Chemical</jtitle><date>2018-12-20</date><risdate>2018</risdate><volume>277</volume><spage>373</spage><epage>380</epage><pages>373-380</pages><issn>0925-4005</issn><eissn>1873-3077</eissn><abstract>Multicolor emissive carbon dots with novel double emission mechanism and the corresponding applications. [Display omitted] Multicolor emissive carbon dots (CDs) was successfully synthesized via a facile one-pot solvothermal method with the assistance of ethanol, which is nominated as E-CDs. In the reaction system, the addition of ethanol plays a key role in synthesizing CDs with higher proportion of amorphous structures, resulting in multicolor emission of the E-CDs after dissolved in various solvents. Moreover, this solvent dependent multicolor emission of the E-CDs is found to be ascribed to a novel double emission mechanism. The excitation dependent blue emissions stem from intrinsic surface/defect states of the E-CDs while the excitation independent long wavelength emissions originate from solvent molecules connected on the surface of the E-CDs via hydrogen bond. Noticeably, the hydrogen bond between the E-CDs and surrounding environment endows the prepared E-CDs with a unique pH-sensitive feature, which can be used to construct fluorescent pH sensor. Besides, based on this multicolor emission, the E-CDs show potential in bio-labeling, multicolor patterning and solid luminous materials.</abstract><cop>Lausanne</cop><pub>Elsevier B.V</pub><doi>10.1016/j.snb.2018.09.031</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0003-3812-9208</orcidid></addata></record>
fulltext fulltext
identifier ISSN: 0925-4005
ispartof Sensors and actuators. B, Chemical, 2018-12, Vol.277, p.373-380
issn 0925-4005
1873-3077
language eng
recordid cdi_proquest_journals_2159258919
source Elsevier ScienceDirect Journals
subjects Carbon dots
Cell labeling
Chemical synthesis
Emission
Emissions
Ethanol
Ethanol-assisted synthesis
Excitation
Fluorescence
Fluorescent pH sensor
Hydrogen bonds
multicolor emission
Novel double emission mechanism
Sensors
Solvents
title Exploring of multicolor emissive carbon dots with novel double emission mechanism
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-11T02%3A57%3A54IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Exploring%20of%20multicolor%20emissive%20carbon%20dots%20with%20novel%20double%20emission%20mechanism&rft.jtitle=Sensors%20and%20actuators.%20B,%20Chemical&rft.au=Gao,%20Dong&rft.date=2018-12-20&rft.volume=277&rft.spage=373&rft.epage=380&rft.pages=373-380&rft.issn=0925-4005&rft.eissn=1873-3077&rft_id=info:doi/10.1016/j.snb.2018.09.031&rft_dat=%3Cproquest_cross%3E2159258919%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2159258919&rft_id=info:pmid/&rft_els_id=S0925400518316447&rfr_iscdi=true