Adhesive, self-healing and antibacterial properties of Cu-coordinated soft gel based on histamine-conjugated polyaspartamide
Metal-ligand coordination bonding is a non-covalent interaction that has been extensively studied as an effective way to improve the mechanical properties of hydrogels or to generate novel supramolecular self-healing gels. In this study, biodegradable polyaspartamide derivatives conjugated with hist...
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| Veröffentlicht in: | Journal of polymer research 2019, Vol.26 (1), p.1-13, Article 12 |
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| creator | Moon, Jong Ryoul Jeon, Young Sil Kim, Young Jun Kim, Ji-Heung |
| description | Metal-ligand coordination bonding is a non-covalent interaction that has been extensively studied as an effective way to improve the mechanical properties of hydrogels or to generate novel supramolecular self-healing gels. In this study, biodegradable polyaspartamide derivatives conjugated with histamine were synthesized and used to prepare the metal-coordinated supramolecular gel with several different metal-ions such as Cu(II), Ni(II), and Zn(II) in an aqueous solution. The resulting gels showed high adhesive properties on glass and plastics substrates, and the adhesive strength could be modulated by using different metal-ion species as well as the concentration and medium pH. In particular, the Cu(II)-coordinated gel exhibited a reversible self-healing behavior and good antibacterial activity. These wholly bio-based supramolecular polymer gels have potential for various biomedical applications with their multifunctional properties comprising adhesive, self-healing and antimicrobial properties in wet gel state. |
| doi_str_mv | 10.1007/s10965-018-1671-7 |
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In this study, biodegradable polyaspartamide derivatives conjugated with histamine were synthesized and used to prepare the metal-coordinated supramolecular gel with several different metal-ions such as Cu(II), Ni(II), and Zn(II) in an aqueous solution. The resulting gels showed high adhesive properties on glass and plastics substrates, and the adhesive strength could be modulated by using different metal-ion species as well as the concentration and medium pH. In particular, the Cu(II)-coordinated gel exhibited a reversible self-healing behavior and good antibacterial activity. These wholly bio-based supramolecular polymer gels have potential for various biomedical applications with their multifunctional properties comprising adhesive, self-healing and antimicrobial properties in wet gel state.</description><identifier>ISSN: 1022-9760</identifier><identifier>EISSN: 1572-8935</identifier><identifier>DOI: 10.1007/s10965-018-1671-7</identifier><language>eng</language><publisher>Dordrecht: Springer Netherlands</publisher><subject>Adhesive strength ; Adhesives ; Aqueous solutions ; Biodegradability ; Biomedical materials ; Characterization and Evaluation of Materials ; Chemistry ; Chemistry and Materials Science ; Coordination compounds ; Copper ; Glass substrates ; Histamine ; Hydrogels ; Industrial Chemistry/Chemical Engineering ; Ligands ; Mechanical properties ; Nickel ; Original Paper ; Polymer gels ; Polymer Sciences ; Polymers ; Self healing materials ; Supramolecular compounds ; Zinc</subject><ispartof>Journal of polymer research, 2019, Vol.26 (1), p.1-13, Article 12</ispartof><rights>The Polymer Society, Taipei 2018</rights><rights>Journal of Polymer Research is a copyright of Springer, (2018). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c316t-2f4bd9f76be539227f0961abcf4eef1477a0437b01647906d6a289d2ff49a7c33</citedby><cites>FETCH-LOGICAL-c316t-2f4bd9f76be539227f0961abcf4eef1477a0437b01647906d6a289d2ff49a7c33</cites><orcidid>0000-0002-7767-6952</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10965-018-1671-7$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10965-018-1671-7$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Moon, Jong Ryoul</creatorcontrib><creatorcontrib>Jeon, Young Sil</creatorcontrib><creatorcontrib>Kim, Young Jun</creatorcontrib><creatorcontrib>Kim, Ji-Heung</creatorcontrib><title>Adhesive, self-healing and antibacterial properties of Cu-coordinated soft gel based on histamine-conjugated polyaspartamide</title><title>Journal of polymer research</title><addtitle>J Polym Res</addtitle><description>Metal-ligand coordination bonding is a non-covalent interaction that has been extensively studied as an effective way to improve the mechanical properties of hydrogels or to generate novel supramolecular self-healing gels. In this study, biodegradable polyaspartamide derivatives conjugated with histamine were synthesized and used to prepare the metal-coordinated supramolecular gel with several different metal-ions such as Cu(II), Ni(II), and Zn(II) in an aqueous solution. The resulting gels showed high adhesive properties on glass and plastics substrates, and the adhesive strength could be modulated by using different metal-ion species as well as the concentration and medium pH. In particular, the Cu(II)-coordinated gel exhibited a reversible self-healing behavior and good antibacterial activity. These wholly bio-based supramolecular polymer gels have potential for various biomedical applications with their multifunctional properties comprising adhesive, self-healing and antimicrobial properties in wet gel state.</description><subject>Adhesive strength</subject><subject>Adhesives</subject><subject>Aqueous solutions</subject><subject>Biodegradability</subject><subject>Biomedical materials</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Coordination compounds</subject><subject>Copper</subject><subject>Glass substrates</subject><subject>Histamine</subject><subject>Hydrogels</subject><subject>Industrial Chemistry/Chemical Engineering</subject><subject>Ligands</subject><subject>Mechanical properties</subject><subject>Nickel</subject><subject>Original Paper</subject><subject>Polymer gels</subject><subject>Polymer Sciences</subject><subject>Polymers</subject><subject>Self healing materials</subject><subject>Supramolecular compounds</subject><subject>Zinc</subject><issn>1022-9760</issn><issn>1572-8935</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp1kE1LxDAQhosouK7-AG8Br0bz0SbtcVn8ggUveg5pO-lm6TY1SYUFf7ypK3jyMMwM87wzzJtl15TcUULkfaCkEgUmtMRUSIrlSbaghWS4rHhxmmrCGK6kIOfZRQg7QopCinKRfa3aLQT7CbcoQG_wFnRvhw7poU0Rba2bCN7qHo3ejeCjhYCcQesJN8751g46QouCMxF10KNah9S6AW1tiHpvB0jcsJu6H2x0_UGHUft51MJldmZ0H-DqNy-z98eHt_Uz3rw-vaxXG9xwKiJmJq_bykhRQ8ErxqRJv1JdNyYHMDSXUpOcy5pQkcuKiFZoVlYtMyavtGw4X2Y3x73ph48JQlQ7N_khnVSMFpwRTrhMFD1SjXcheDBq9Hav_UFRomaT1dFklUxWs8lq1rCjJiR26MD_bf5f9A0HgoFL</recordid><startdate>2019</startdate><enddate>2019</enddate><creator>Moon, Jong Ryoul</creator><creator>Jeon, Young Sil</creator><creator>Kim, Young Jun</creator><creator>Kim, Ji-Heung</creator><general>Springer Netherlands</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><orcidid>https://orcid.org/0000-0002-7767-6952</orcidid></search><sort><creationdate>2019</creationdate><title>Adhesive, self-healing and antibacterial properties of Cu-coordinated soft gel based on histamine-conjugated polyaspartamide</title><author>Moon, Jong Ryoul ; Jeon, Young Sil ; Kim, Young Jun ; Kim, Ji-Heung</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c316t-2f4bd9f76be539227f0961abcf4eef1477a0437b01647906d6a289d2ff49a7c33</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Adhesive strength</topic><topic>Adhesives</topic><topic>Aqueous solutions</topic><topic>Biodegradability</topic><topic>Biomedical materials</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Coordination compounds</topic><topic>Copper</topic><topic>Glass substrates</topic><topic>Histamine</topic><topic>Hydrogels</topic><topic>Industrial Chemistry/Chemical Engineering</topic><topic>Ligands</topic><topic>Mechanical properties</topic><topic>Nickel</topic><topic>Original Paper</topic><topic>Polymer gels</topic><topic>Polymer Sciences</topic><topic>Polymers</topic><topic>Self healing materials</topic><topic>Supramolecular compounds</topic><topic>Zinc</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Moon, Jong Ryoul</creatorcontrib><creatorcontrib>Jeon, Young Sil</creatorcontrib><creatorcontrib>Kim, Young Jun</creatorcontrib><creatorcontrib>Kim, Ji-Heung</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>Materials Science Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><jtitle>Journal of polymer research</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Moon, Jong Ryoul</au><au>Jeon, Young Sil</au><au>Kim, Young Jun</au><au>Kim, Ji-Heung</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Adhesive, self-healing and antibacterial properties of Cu-coordinated soft gel based on histamine-conjugated polyaspartamide</atitle><jtitle>Journal of polymer research</jtitle><stitle>J Polym Res</stitle><date>2019</date><risdate>2019</risdate><volume>26</volume><issue>1</issue><spage>1</spage><epage>13</epage><pages>1-13</pages><artnum>12</artnum><issn>1022-9760</issn><eissn>1572-8935</eissn><abstract>Metal-ligand coordination bonding is a non-covalent interaction that has been extensively studied as an effective way to improve the mechanical properties of hydrogels or to generate novel supramolecular self-healing gels. 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| subjects | Adhesive strength Adhesives Aqueous solutions Biodegradability Biomedical materials Characterization and Evaluation of Materials Chemistry Chemistry and Materials Science Coordination compounds Copper Glass substrates Histamine Hydrogels Industrial Chemistry/Chemical Engineering Ligands Mechanical properties Nickel Original Paper Polymer gels Polymer Sciences Polymers Self healing materials Supramolecular compounds Zinc |
| title | Adhesive, self-healing and antibacterial properties of Cu-coordinated soft gel based on histamine-conjugated polyaspartamide |
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