Effect of charge ordering on crossplane thermal conductivity in correlated perovskite oxide superlattices

Lattice thermal conductivity is a sensitive probe of distortions of the translational invariance of crystalline materials. Crossplane thermal conductivity, κ(T), was studied by the 3ω technique in superlattices, comprising orthorhombic charge/orbital ordered manganite Pr0.7Ca0.3MnO3 and cubic SrTiO3...

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Veröffentlicht in:Physical review. B 2018-11, Vol.98 (19), Article 195114
Hauptverfasser: Thiessen, P., Roddatis, V., Rieger, F., Belenchuk, A., Keunecke, M., Moshnyaga, V., Jooss, Ch
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container_issue 19
container_start_page
container_title Physical review. B
container_volume 98
creator Thiessen, P.
Roddatis, V.
Rieger, F.
Belenchuk, A.
Keunecke, M.
Moshnyaga, V.
Jooss, Ch
description Lattice thermal conductivity is a sensitive probe of distortions of the translational invariance of crystalline materials. Crossplane thermal conductivity, κ(T), was studied by the 3ω technique in superlattices, comprising orthorhombic charge/orbital ordered manganite Pr0.7Ca0.3MnO3 and cubic SrTiO3. The manganite/titanite superlattices show a peak in κ(T) just above the charge order transition temperature TCO∼240K with a pronounced thermal hysteresis. This ordering peak in κ(T) is successively suppressed with decreasing layer thickness. Our results demonstrate a minor effect of the interface density on κ, primarily visible below TCO. In contrast, much higher changes in κ(T) evolve close to TCO, due to interface-induced effects on charge and orbital ordering. Our results suggest that the ordering peak in κ(T) is a result of lattice softening above the phase transition which is modified by thickness-dependent misfit strain.
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subjects Heat conductivity
Heat transfer
Manganites
Perovskites
Phase transitions
Strontium titanates
Superlattices
Thermal conductivity
Thickness
Transition temperature
title Effect of charge ordering on crossplane thermal conductivity in correlated perovskite oxide superlattices
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