Novel poly(3,4-ethylenedioxythiophene)/reduced graphene oxide incorporated with manganese oxide/iron oxide for supercapacitor device
A new composite namely PEDOT/RGO/MnO 2 /Fe 2 O 3 was successfully developed from mixed metal oxides (MnO 2 and Fe 2 O 3 ) incorporated with poly(3,4-ethylenedioxythiophene) (PEDOT) and reduced graphene oxide (RGO). The surface morphology of the prepared composite revealed that MnO 2 and Fe 2 O 3 par...
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| Veröffentlicht in: | Journal of materials science. Materials in electronics 2019-01, Vol.30 (2), p.1458-1467 |
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| creator | Azman, Nur Hawa Nabilah Sulaiman, Yusran Mamat @ Mat Nazir, Md Shuhazlly Lim, Hong Ngee |
| description | A new composite namely PEDOT/RGO/MnO
2
/Fe
2
O
3
was successfully developed from mixed metal oxides (MnO
2
and Fe
2
O
3
) incorporated with poly(3,4-ethylenedioxythiophene) (PEDOT) and reduced graphene oxide (RGO). The surface morphology of the prepared composite revealed that MnO
2
and Fe
2
O
3
particles were successfully coated on the wrinkles and curly like-sheets of PEDOT/RGO in order to prevent aggregation of RGO layers and the composite was able to retain 80% of its initial specific capacitance in 1 M KCl. The PEDOT/RGO/MnO
2
/Fe
2
O
3
composite with Mn:Fe molar ratio of 2:3 displayed the highest specific capacitance of 287 F/g indicating that Mn:Fe molar ratio gives significant effect on the supercapacitive performance of the composite. The specific capacitance of PEDOT/RGO/MnO
2
/Fe
2
O
3
was higher than the composites with monometallic oxide i.e. PEDOT/RGO/MnO
2
and PEDOT/RGO/Fe
2
O
3
. The PEDOT/RGO/MnO
2
/Fe
2
O
3
composite also revealed the lowest charge transfer resistance that leads to the superior supercapacitive performance. The specific energy and specific power of PEDOT/RGO/MnO
2
/Fe
2
O
3
composite were 11 Wh/kg and 1900 W/kg at 4 A/g, respectively. The results showed that the PEDOT/RGO/MnO
2
/Fe
2
O
3
composite is a promising electrode material for high-performance supercapacitor. |
| doi_str_mv | 10.1007/s10854-018-0415-0 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2137639469</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2137639469</sourcerecordid><originalsourceid>FETCH-LOGICAL-c396t-6e2e52a811e69d85d1b4526ad6538ee259aec729d0205daf559a80364e92a16f3</originalsourceid><addsrcrecordid>eNp1kMtOwzAQRS0EEqXwAewisQEJUz9iJ1miipdUwQYkdpaJJ42rNg52Upo9H45LK7FiNboz585oLkLnlNxQQrJJoCQXKSY0xySlApMDNKIi4zjN2fshGpFCZDgVjB2jkxAWhBCZ8nyEvp_dGpZJ65bDJb9OMXT1sIQGjHWboauta-uoriYeTF-CSeZe_3YSt7EGEtuUzrfO6y7OvmxXJyvdzHUDYU9MrHfNHq6cT0Lfgi91q0vbRWlgbUs4RUeVXgY429cxeru_e50-4tnLw9P0doZLXsgOS2AgmM4pBVmYXBj6ET-S2kjBcwAmCg1lxgpDGBFGVyI2csJlCgXTVFZ8jC52e1vvPnsInVq43jfxpGKUZ5IXqSwiRXdU6V0IHirVervSflCUqG3Yahe2imGrbdiKRA_beUJkmzn4v83_m34ARM2EeQ</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2137639469</pqid></control><display><type>article</type><title>Novel poly(3,4-ethylenedioxythiophene)/reduced graphene oxide incorporated with manganese oxide/iron oxide for supercapacitor device</title><source>Springer Nature - Complete Springer Journals</source><creator>Azman, Nur Hawa Nabilah ; Sulaiman, Yusran ; Mamat @ Mat Nazir, Md Shuhazlly ; Lim, Hong Ngee</creator><creatorcontrib>Azman, Nur Hawa Nabilah ; Sulaiman, Yusran ; Mamat @ Mat Nazir, Md Shuhazlly ; Lim, Hong Ngee</creatorcontrib><description>A new composite namely PEDOT/RGO/MnO
2
/Fe
2
O
3
was successfully developed from mixed metal oxides (MnO
2
and Fe
2
O
3
) incorporated with poly(3,4-ethylenedioxythiophene) (PEDOT) and reduced graphene oxide (RGO). The surface morphology of the prepared composite revealed that MnO
2
and Fe
2
O
3
particles were successfully coated on the wrinkles and curly like-sheets of PEDOT/RGO in order to prevent aggregation of RGO layers and the composite was able to retain 80% of its initial specific capacitance in 1 M KCl. The PEDOT/RGO/MnO
2
/Fe
2
O
3
composite with Mn:Fe molar ratio of 2:3 displayed the highest specific capacitance of 287 F/g indicating that Mn:Fe molar ratio gives significant effect on the supercapacitive performance of the composite. The specific capacitance of PEDOT/RGO/MnO
2
/Fe
2
O
3
was higher than the composites with monometallic oxide i.e. PEDOT/RGO/MnO
2
and PEDOT/RGO/Fe
2
O
3
. The PEDOT/RGO/MnO
2
/Fe
2
O
3
composite also revealed the lowest charge transfer resistance that leads to the superior supercapacitive performance. The specific energy and specific power of PEDOT/RGO/MnO
2
/Fe
2
O
3
composite were 11 Wh/kg and 1900 W/kg at 4 A/g, respectively. The results showed that the PEDOT/RGO/MnO
2
/Fe
2
O
3
composite is a promising electrode material for high-performance supercapacitor.</description><identifier>ISSN: 0957-4522</identifier><identifier>EISSN: 1573-482X</identifier><identifier>DOI: 10.1007/s10854-018-0415-0</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Capacitance ; Carbon ; Characterization and Evaluation of Materials ; Charge transfer ; Chemistry and Materials Science ; Electrode materials ; Electrodes ; Energy ; Graphene ; Iron oxides ; Laboratories ; Manganese dioxide ; Materials Science ; Medical equipment ; Metal oxides ; Morphology ; Optical and Electronic Materials ; Particulate composites ; Polymers ; Supercapacitors ; Zinc oxides</subject><ispartof>Journal of materials science. Materials in electronics, 2019-01, Vol.30 (2), p.1458-1467</ispartof><rights>Springer Science+Business Media, LLC, part of Springer Nature 2018</rights><rights>Journal of Materials Science: Materials in Electronics is a copyright of Springer, (2018). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c396t-6e2e52a811e69d85d1b4526ad6538ee259aec729d0205daf559a80364e92a16f3</citedby><cites>FETCH-LOGICAL-c396t-6e2e52a811e69d85d1b4526ad6538ee259aec729d0205daf559a80364e92a16f3</cites><orcidid>0000-0002-1841-2447</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10854-018-0415-0$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10854-018-0415-0$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27903,27904,41467,42536,51297</link.rule.ids></links><search><creatorcontrib>Azman, Nur Hawa Nabilah</creatorcontrib><creatorcontrib>Sulaiman, Yusran</creatorcontrib><creatorcontrib>Mamat @ Mat Nazir, Md Shuhazlly</creatorcontrib><creatorcontrib>Lim, Hong Ngee</creatorcontrib><title>Novel poly(3,4-ethylenedioxythiophene)/reduced graphene oxide incorporated with manganese oxide/iron oxide for supercapacitor device</title><title>Journal of materials science. Materials in electronics</title><addtitle>J Mater Sci: Mater Electron</addtitle><description>A new composite namely PEDOT/RGO/MnO
2
/Fe
2
O
3
was successfully developed from mixed metal oxides (MnO
2
and Fe
2
O
3
) incorporated with poly(3,4-ethylenedioxythiophene) (PEDOT) and reduced graphene oxide (RGO). The surface morphology of the prepared composite revealed that MnO
2
and Fe
2
O
3
particles were successfully coated on the wrinkles and curly like-sheets of PEDOT/RGO in order to prevent aggregation of RGO layers and the composite was able to retain 80% of its initial specific capacitance in 1 M KCl. The PEDOT/RGO/MnO
2
/Fe
2
O
3
composite with Mn:Fe molar ratio of 2:3 displayed the highest specific capacitance of 287 F/g indicating that Mn:Fe molar ratio gives significant effect on the supercapacitive performance of the composite. The specific capacitance of PEDOT/RGO/MnO
2
/Fe
2
O
3
was higher than the composites with monometallic oxide i.e. PEDOT/RGO/MnO
2
and PEDOT/RGO/Fe
2
O
3
. The PEDOT/RGO/MnO
2
/Fe
2
O
3
composite also revealed the lowest charge transfer resistance that leads to the superior supercapacitive performance. The specific energy and specific power of PEDOT/RGO/MnO
2
/Fe
2
O
3
composite were 11 Wh/kg and 1900 W/kg at 4 A/g, respectively. The results showed that the PEDOT/RGO/MnO
2
/Fe
2
O
3
composite is a promising electrode material for high-performance supercapacitor.</description><subject>Capacitance</subject><subject>Carbon</subject><subject>Characterization and Evaluation of Materials</subject><subject>Charge transfer</subject><subject>Chemistry and Materials Science</subject><subject>Electrode materials</subject><subject>Electrodes</subject><subject>Energy</subject><subject>Graphene</subject><subject>Iron oxides</subject><subject>Laboratories</subject><subject>Manganese dioxide</subject><subject>Materials Science</subject><subject>Medical equipment</subject><subject>Metal oxides</subject><subject>Morphology</subject><subject>Optical and Electronic Materials</subject><subject>Particulate composites</subject><subject>Polymers</subject><subject>Supercapacitors</subject><subject>Zinc oxides</subject><issn>0957-4522</issn><issn>1573-482X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp1kMtOwzAQRS0EEqXwAewisQEJUz9iJ1miipdUwQYkdpaJJ42rNg52Upo9H45LK7FiNboz585oLkLnlNxQQrJJoCQXKSY0xySlApMDNKIi4zjN2fshGpFCZDgVjB2jkxAWhBCZ8nyEvp_dGpZJ65bDJb9OMXT1sIQGjHWboauta-uoriYeTF-CSeZe_3YSt7EGEtuUzrfO6y7OvmxXJyvdzHUDYU9MrHfNHq6cT0Lfgi91q0vbRWlgbUs4RUeVXgY429cxeru_e50-4tnLw9P0doZLXsgOS2AgmM4pBVmYXBj6ET-S2kjBcwAmCg1lxgpDGBFGVyI2csJlCgXTVFZ8jC52e1vvPnsInVq43jfxpGKUZ5IXqSwiRXdU6V0IHirVervSflCUqG3Yahe2imGrbdiKRA_beUJkmzn4v83_m34ARM2EeQ</recordid><startdate>20190101</startdate><enddate>20190101</enddate><creator>Azman, Nur Hawa Nabilah</creator><creator>Sulaiman, Yusran</creator><creator>Mamat @ Mat Nazir, Md Shuhazlly</creator><creator>Lim, Hong Ngee</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>F28</scope><scope>FR3</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>L7M</scope><scope>P5Z</scope><scope>P62</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>S0W</scope><orcidid>https://orcid.org/0000-0002-1841-2447</orcidid></search><sort><creationdate>20190101</creationdate><title>Novel poly(3,4-ethylenedioxythiophene)/reduced graphene oxide incorporated with manganese oxide/iron oxide for supercapacitor device</title><author>Azman, Nur Hawa Nabilah ; Sulaiman, Yusran ; Mamat @ Mat Nazir, Md Shuhazlly ; Lim, Hong Ngee</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c396t-6e2e52a811e69d85d1b4526ad6538ee259aec729d0205daf559a80364e92a16f3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Capacitance</topic><topic>Carbon</topic><topic>Characterization and Evaluation of Materials</topic><topic>Charge transfer</topic><topic>Chemistry and Materials Science</topic><topic>Electrode materials</topic><topic>Electrodes</topic><topic>Energy</topic><topic>Graphene</topic><topic>Iron oxides</topic><topic>Laboratories</topic><topic>Manganese dioxide</topic><topic>Materials Science</topic><topic>Medical equipment</topic><topic>Metal oxides</topic><topic>Morphology</topic><topic>Optical and Electronic Materials</topic><topic>Particulate composites</topic><topic>Polymers</topic><topic>Supercapacitors</topic><topic>Zinc oxides</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Azman, Nur Hawa Nabilah</creatorcontrib><creatorcontrib>Sulaiman, Yusran</creatorcontrib><creatorcontrib>Mamat @ Mat Nazir, Md Shuhazlly</creatorcontrib><creatorcontrib>Lim, Hong Ngee</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>Materials Science Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>DELNET Engineering & Technology Collection</collection><jtitle>Journal of materials science. Materials in electronics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Azman, Nur Hawa Nabilah</au><au>Sulaiman, Yusran</au><au>Mamat @ Mat Nazir, Md Shuhazlly</au><au>Lim, Hong Ngee</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Novel poly(3,4-ethylenedioxythiophene)/reduced graphene oxide incorporated with manganese oxide/iron oxide for supercapacitor device</atitle><jtitle>Journal of materials science. Materials in electronics</jtitle><stitle>J Mater Sci: Mater Electron</stitle><date>2019-01-01</date><risdate>2019</risdate><volume>30</volume><issue>2</issue><spage>1458</spage><epage>1467</epage><pages>1458-1467</pages><issn>0957-4522</issn><eissn>1573-482X</eissn><abstract>A new composite namely PEDOT/RGO/MnO
2
/Fe
2
O
3
was successfully developed from mixed metal oxides (MnO
2
and Fe
2
O
3
) incorporated with poly(3,4-ethylenedioxythiophene) (PEDOT) and reduced graphene oxide (RGO). The surface morphology of the prepared composite revealed that MnO
2
and Fe
2
O
3
particles were successfully coated on the wrinkles and curly like-sheets of PEDOT/RGO in order to prevent aggregation of RGO layers and the composite was able to retain 80% of its initial specific capacitance in 1 M KCl. The PEDOT/RGO/MnO
2
/Fe
2
O
3
composite with Mn:Fe molar ratio of 2:3 displayed the highest specific capacitance of 287 F/g indicating that Mn:Fe molar ratio gives significant effect on the supercapacitive performance of the composite. The specific capacitance of PEDOT/RGO/MnO
2
/Fe
2
O
3
was higher than the composites with monometallic oxide i.e. PEDOT/RGO/MnO
2
and PEDOT/RGO/Fe
2
O
3
. The PEDOT/RGO/MnO
2
/Fe
2
O
3
composite also revealed the lowest charge transfer resistance that leads to the superior supercapacitive performance. The specific energy and specific power of PEDOT/RGO/MnO
2
/Fe
2
O
3
composite were 11 Wh/kg and 1900 W/kg at 4 A/g, respectively. The results showed that the PEDOT/RGO/MnO
2
/Fe
2
O
3
composite is a promising electrode material for high-performance supercapacitor.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10854-018-0415-0</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0002-1841-2447</orcidid><oa>free_for_read</oa></addata></record> |
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| ispartof | Journal of materials science. Materials in electronics, 2019-01, Vol.30 (2), p.1458-1467 |
| issn | 0957-4522 1573-482X |
| language | eng |
| recordid | cdi_proquest_journals_2137639469 |
| source | Springer Nature - Complete Springer Journals |
| subjects | Capacitance Carbon Characterization and Evaluation of Materials Charge transfer Chemistry and Materials Science Electrode materials Electrodes Energy Graphene Iron oxides Laboratories Manganese dioxide Materials Science Medical equipment Metal oxides Morphology Optical and Electronic Materials Particulate composites Polymers Supercapacitors Zinc oxides |
| title | Novel poly(3,4-ethylenedioxythiophene)/reduced graphene oxide incorporated with manganese oxide/iron oxide for supercapacitor device |
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