Fluoride volatility experiments on irradiated thoria fuel at Canadian Nuclear Laboratories
[Display omitted] •Uranium was removed from irradiated thoria fuel via the fluoride volatility technique.•Longer fluorination times resulting in greater uranium removal for tests up to 24 h.•Fission products with volatile fluorides were also removed, Zr, Mo, Ru, and Rh. Fluoride volatility experimen...
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| Veröffentlicht in: | Journal of fluorine chemistry 2018-10, Vol.214, p.8-12 |
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| container_title | Journal of fluorine chemistry |
| container_volume | 214 |
| creator | Barry, Aaron Bergeron, Andrew Stoddard, Tim Crigger, Brent Hamilton, Holly Maybee, Adam |
| description | [Display omitted]
•Uranium was removed from irradiated thoria fuel via the fluoride volatility technique.•Longer fluorination times resulting in greater uranium removal for tests up to 24 h.•Fission products with volatile fluorides were also removed, Zr, Mo, Ru, and Rh.
Fluoride volatility experiments were completed on irradiated thoria fuel in a hot cell facility at Canadian Nuclear Laboratories (CNL). Uranium was removed from irradiated thoria fuel in significant quantities, with longer fluorination times resulting in greater uranium removal for tests up to 24 h. Some fission products were also removed via fluorination; fission products with fluorides having low boiling points (Mo and Ru) were removed in greater quantities than fission products with fluorides having higher boiling points (Zr and Rh). |
| doi_str_mv | 10.1016/j.jfluchem.2018.07.011 |
| format | Article |
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•Uranium was removed from irradiated thoria fuel via the fluoride volatility technique.•Longer fluorination times resulting in greater uranium removal for tests up to 24 h.•Fission products with volatile fluorides were also removed, Zr, Mo, Ru, and Rh.
Fluoride volatility experiments were completed on irradiated thoria fuel in a hot cell facility at Canadian Nuclear Laboratories (CNL). Uranium was removed from irradiated thoria fuel in significant quantities, with longer fluorination times resulting in greater uranium removal for tests up to 24 h. Some fission products were also removed via fluorination; fission products with fluorides having low boiling points (Mo and Ru) were removed in greater quantities than fission products with fluorides having higher boiling points (Zr and Rh).</description><identifier>ISSN: 0022-1139</identifier><identifier>EISSN: 1873-3328</identifier><identifier>DOI: 10.1016/j.jfluchem.2018.07.011</identifier><language>eng</language><publisher>Lausanne: Elsevier B.V</publisher><subject>Boiling ; Boiling points ; Chemistry ; Fission products ; Fluoride volatility ; Fluorides ; Fluorination ; Fuel ; Irradiated ; Laboratories ; Laboratory tests ; Nuclear fission ; Nuclear fuels ; Reprocessing ; ThO2 ; Thoria ; Thorium dioxide ; Uranium ; Volatility ; Zirconium</subject><ispartof>Journal of fluorine chemistry, 2018-10, Vol.214, p.8-12</ispartof><rights>2018</rights><rights>Copyright Elsevier BV Oct 2018</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c388t-eb5f523f80d1379105f998a0d045b8f24ffd215e791a4d6d4ec0af96e24007ea3</citedby><cites>FETCH-LOGICAL-c388t-eb5f523f80d1379105f998a0d045b8f24ffd215e791a4d6d4ec0af96e24007ea3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.jfluchem.2018.07.011$$EHTML$$P50$$Gelsevier$$Hfree_for_read</linktohtml><link.rule.ids>314,777,781,3537,27905,27906,45976</link.rule.ids></links><search><creatorcontrib>Barry, Aaron</creatorcontrib><creatorcontrib>Bergeron, Andrew</creatorcontrib><creatorcontrib>Stoddard, Tim</creatorcontrib><creatorcontrib>Crigger, Brent</creatorcontrib><creatorcontrib>Hamilton, Holly</creatorcontrib><creatorcontrib>Maybee, Adam</creatorcontrib><title>Fluoride volatility experiments on irradiated thoria fuel at Canadian Nuclear Laboratories</title><title>Journal of fluorine chemistry</title><description>[Display omitted]
•Uranium was removed from irradiated thoria fuel via the fluoride volatility technique.•Longer fluorination times resulting in greater uranium removal for tests up to 24 h.•Fission products with volatile fluorides were also removed, Zr, Mo, Ru, and Rh.
Fluoride volatility experiments were completed on irradiated thoria fuel in a hot cell facility at Canadian Nuclear Laboratories (CNL). Uranium was removed from irradiated thoria fuel in significant quantities, with longer fluorination times resulting in greater uranium removal for tests up to 24 h. Some fission products were also removed via fluorination; fission products with fluorides having low boiling points (Mo and Ru) were removed in greater quantities than fission products with fluorides having higher boiling points (Zr and Rh).</description><subject>Boiling</subject><subject>Boiling points</subject><subject>Chemistry</subject><subject>Fission products</subject><subject>Fluoride volatility</subject><subject>Fluorides</subject><subject>Fluorination</subject><subject>Fuel</subject><subject>Irradiated</subject><subject>Laboratories</subject><subject>Laboratory tests</subject><subject>Nuclear fission</subject><subject>Nuclear fuels</subject><subject>Reprocessing</subject><subject>ThO2</subject><subject>Thoria</subject><subject>Thorium dioxide</subject><subject>Uranium</subject><subject>Volatility</subject><subject>Zirconium</subject><issn>0022-1139</issn><issn>1873-3328</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNqFkLtOwzAUhi0EEqXwCsgSc8KxnYuzgSoKSBUssLBYbnysOkqTYjsVvD2uCjPTGf7L0f8Rcs0gZ8Cq2y7vbD-1G9zmHJjMoc6BsRMyY7IWmRBcnpIZAOcZY6I5JxchdABQQy1n5GPZT6N3Bul-7HV0vYvfFL926N0WhxjoOFDnvTZORzQ0bpJZUzthT3WkCz0clIG-TG2P2tOVXo9ex2TCcEnOrO4DXv3eOXlfPrwtnrLV6-Pz4n6VtULKmOG6tCUXVoJhom4YlLZppAYDRbmWlhfWGs5KTJIuTGUKbEHbpkJepBGoxZzcHHt3fvycMETVjZMf0kvFmRBSMC55clVHV-vHEDxatUsTtf9WDNSBo-rUH0d14KigVoljCt4dg5g27B16FVqHQ4vGeWyjMqP7r-IHzE2AXQ</recordid><startdate>201810</startdate><enddate>201810</enddate><creator>Barry, Aaron</creator><creator>Bergeron, Andrew</creator><creator>Stoddard, Tim</creator><creator>Crigger, Brent</creator><creator>Hamilton, Holly</creator><creator>Maybee, Adam</creator><general>Elsevier B.V</general><general>Elsevier BV</general><scope>6I.</scope><scope>AAFTH</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QF</scope><scope>7QO</scope><scope>7QP</scope><scope>7QQ</scope><scope>7SC</scope><scope>7SE</scope><scope>7SP</scope><scope>7SR</scope><scope>7TA</scope><scope>7TB</scope><scope>7U5</scope><scope>7U7</scope><scope>8BQ</scope><scope>8FD</scope><scope>C1K</scope><scope>F28</scope><scope>FR3</scope><scope>H8D</scope><scope>H8G</scope><scope>JG9</scope><scope>JQ2</scope><scope>KR7</scope><scope>L7M</scope><scope>L~C</scope><scope>L~D</scope><scope>P64</scope></search><sort><creationdate>201810</creationdate><title>Fluoride volatility experiments on irradiated thoria fuel at Canadian Nuclear Laboratories</title><author>Barry, Aaron ; 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•Uranium was removed from irradiated thoria fuel via the fluoride volatility technique.•Longer fluorination times resulting in greater uranium removal for tests up to 24 h.•Fission products with volatile fluorides were also removed, Zr, Mo, Ru, and Rh.
Fluoride volatility experiments were completed on irradiated thoria fuel in a hot cell facility at Canadian Nuclear Laboratories (CNL). Uranium was removed from irradiated thoria fuel in significant quantities, with longer fluorination times resulting in greater uranium removal for tests up to 24 h. Some fission products were also removed via fluorination; fission products with fluorides having low boiling points (Mo and Ru) were removed in greater quantities than fission products with fluorides having higher boiling points (Zr and Rh).</abstract><cop>Lausanne</cop><pub>Elsevier B.V</pub><doi>10.1016/j.jfluchem.2018.07.011</doi><tpages>5</tpages><oa>free_for_read</oa></addata></record> |
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| identifier | ISSN: 0022-1139 |
| ispartof | Journal of fluorine chemistry, 2018-10, Vol.214, p.8-12 |
| issn | 0022-1139 1873-3328 |
| language | eng |
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| source | Elsevier ScienceDirect Journals |
| subjects | Boiling Boiling points Chemistry Fission products Fluoride volatility Fluorides Fluorination Fuel Irradiated Laboratories Laboratory tests Nuclear fission Nuclear fuels Reprocessing ThO2 Thoria Thorium dioxide Uranium Volatility Zirconium |
| title | Fluoride volatility experiments on irradiated thoria fuel at Canadian Nuclear Laboratories |
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