Removal of methylene blue from aqueous solution using sediment obtained from a canal in an industrial park
Drainage canal sediments in an industrial park are generally dredged to landfill in Taiwan. The objective of this study was to evaluate feasibility employing the sediment as an adsorbent for removal of dye. The sediment contained approximately 10% of organic matter and little heavy metals. Infrared...
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| Veröffentlicht in: | Water science and technology 2018-09, Vol.78 (3-4), p.556-570 |
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| creator | Chen, Lih-Fu Wang, Hsiou-Hsuan Lin, Kao-Yung Kuo, Jui-Yen Wang, Ming-Kuang Liu, Cheng-Chung |
| description | Drainage canal sediments in an industrial park are generally dredged to landfill in Taiwan. The objective of this study was to evaluate feasibility employing the sediment as an adsorbent for removal of dye. The sediment contained approximately 10% of organic matter and little heavy metals. Infrared (IR) analysis revealed that carboxyl was the most important functional group for methylene blue (MB) sorption. Canal sediment could remove the most MB from water at pH 8.0 and this removal increased with increasing temperature. The MB sorption was well described by the Langmuir, Dubinin-Radushkevich, and Temkin sorption isotherms at 10°C, but it showed good compliance with Freundlich isotherm at 25°C and 40°C. The MB adsorption was a spontaneous and endothermic reaction; its maximum calculated adsorption capacity (Q
) was 56.0 mg g
at 10°C by the Langmuir isotherm. The calculated values of enthalpy (ΔH°) and entropy (ΔS°) are 14.6 kJ mol
and 149.2 kJ mol
, respectively. Only pseudo-second-order adsorption kinetic model successfully described the kinetics of MB onto the sediment at different operation parameters. Activation energy of MB adsorption calculated from Arrhenius equation was 16.434 kJ mol
, indicating the binding between canal sediment and MB was a physical adsorption. |
| doi_str_mv | 10.2166/wst.2018.326 |
| format | Article |
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) was 56.0 mg g
at 10°C by the Langmuir isotherm. The calculated values of enthalpy (ΔH°) and entropy (ΔS°) are 14.6 kJ mol
and 149.2 kJ mol
, respectively. Only pseudo-second-order adsorption kinetic model successfully described the kinetics of MB onto the sediment at different operation parameters. Activation energy of MB adsorption calculated from Arrhenius equation was 16.434 kJ mol
, indicating the binding between canal sediment and MB was a physical adsorption.</description><identifier>ISSN: 0273-1223</identifier><identifier>EISSN: 1996-9732</identifier><identifier>DOI: 10.2166/wst.2018.326</identifier><identifier>PMID: 30207997</identifier><language>eng</language><publisher>England: IWA Publishing</publisher><subject>Activated carbon ; Adsorbents ; Adsorption ; Aqueous solutions ; Canals ; Drainage canals ; Dredging ; Dyes ; Endothermic reactions ; Enthalpy ; Entropy ; Feasibility studies ; Functional groups ; Hazardous materials ; Heavy metals ; Hydrogen-Ion Concentration ; Industrial parks ; Infrared analysis ; Isotherms ; Kinetics ; Landfills ; Membrane separation ; Metals ; Methylene Blue ; Organic matter ; Particle size ; Reaction kinetics ; Removal ; Sediment ; Sediments ; Soil testing ; Sorption ; Taiwan ; Temperature ; Thermodynamics ; Waste disposal sites ; Water Pollutants, Chemical ; Water Purification</subject><ispartof>Water science and technology, 2018-09, Vol.78 (3-4), p.556-570</ispartof><rights>Copyright IWA Publishing Sep 2018</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c423t-9d9a5b99f2450e785858fd8bc6733f220c2886a5c4ba638c5c87cab15efb42ab3</citedby><cites>FETCH-LOGICAL-c423t-9d9a5b99f2450e785858fd8bc6733f220c2886a5c4ba638c5c87cab15efb42ab3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/30207997$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Chen, Lih-Fu</creatorcontrib><creatorcontrib>Wang, Hsiou-Hsuan</creatorcontrib><creatorcontrib>Lin, Kao-Yung</creatorcontrib><creatorcontrib>Kuo, Jui-Yen</creatorcontrib><creatorcontrib>Wang, Ming-Kuang</creatorcontrib><creatorcontrib>Liu, Cheng-Chung</creatorcontrib><title>Removal of methylene blue from aqueous solution using sediment obtained from a canal in an industrial park</title><title>Water science and technology</title><addtitle>Water Sci Technol</addtitle><description>Drainage canal sediments in an industrial park are generally dredged to landfill in Taiwan. The objective of this study was to evaluate feasibility employing the sediment as an adsorbent for removal of dye. The sediment contained approximately 10% of organic matter and little heavy metals. Infrared (IR) analysis revealed that carboxyl was the most important functional group for methylene blue (MB) sorption. Canal sediment could remove the most MB from water at pH 8.0 and this removal increased with increasing temperature. The MB sorption was well described by the Langmuir, Dubinin-Radushkevich, and Temkin sorption isotherms at 10°C, but it showed good compliance with Freundlich isotherm at 25°C and 40°C. The MB adsorption was a spontaneous and endothermic reaction; its maximum calculated adsorption capacity (Q
) was 56.0 mg g
at 10°C by the Langmuir isotherm. The calculated values of enthalpy (ΔH°) and entropy (ΔS°) are 14.6 kJ mol
and 149.2 kJ mol
, respectively. Only pseudo-second-order adsorption kinetic model successfully described the kinetics of MB onto the sediment at different operation parameters. Activation energy of MB adsorption calculated from Arrhenius equation was 16.434 kJ mol
, indicating the binding between canal sediment and MB was a physical adsorption.</description><subject>Activated carbon</subject><subject>Adsorbents</subject><subject>Adsorption</subject><subject>Aqueous solutions</subject><subject>Canals</subject><subject>Drainage canals</subject><subject>Dredging</subject><subject>Dyes</subject><subject>Endothermic reactions</subject><subject>Enthalpy</subject><subject>Entropy</subject><subject>Feasibility studies</subject><subject>Functional groups</subject><subject>Hazardous materials</subject><subject>Heavy metals</subject><subject>Hydrogen-Ion Concentration</subject><subject>Industrial parks</subject><subject>Infrared analysis</subject><subject>Isotherms</subject><subject>Kinetics</subject><subject>Landfills</subject><subject>Membrane separation</subject><subject>Metals</subject><subject>Methylene Blue</subject><subject>Organic matter</subject><subject>Particle size</subject><subject>Reaction kinetics</subject><subject>Removal</subject><subject>Sediment</subject><subject>Sediments</subject><subject>Soil testing</subject><subject>Sorption</subject><subject>Taiwan</subject><subject>Temperature</subject><subject>Thermodynamics</subject><subject>Waste disposal sites</subject><subject>Water Pollutants, Chemical</subject><subject>Water Purification</subject><issn>0273-1223</issn><issn>1996-9732</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNo9kE1LxDAQhoMo7rp68ywBr3bNR5s0R1n8AkEQPYckTbRrm6xJquy_N-IqAzMwPLzMPACcYrQkmLHLr5SXBOF2SQnbA3MsBKsEp2QfzBHhtMKE0Bk4SmmNEOK0RodgRhFBXAg-B-snO4ZPNcDg4Gjz23aw3kI9TBa6GEaoPiYbpgRTGKbcBw-n1PtXmGzXj9ZnGHRWvbfdjoZG-RLWe6h86d2UcuzLYqPi-zE4cGpI9mQ3F-Dl5vp5dVc9PN7er64eKlMTmivRCdVoIRypG2R525RyXasN45Q6QpAhbctUY2qtGG1NY1pulMaNdbomStMFOP_N3cRQrk9ZrsMUy1lJEkwRYrw8X6iLX8rEkFK0Tm5iP6q4lRjJH7GyiJU_YmURW_CzXeikR9v9w38m6TfNgnUi</recordid><startdate>201809</startdate><enddate>201809</enddate><creator>Chen, Lih-Fu</creator><creator>Wang, Hsiou-Hsuan</creator><creator>Lin, Kao-Yung</creator><creator>Kuo, Jui-Yen</creator><creator>Wang, Ming-Kuang</creator><creator>Liu, Cheng-Chung</creator><general>IWA 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sediment obtained from a canal in an industrial park</title><author>Chen, Lih-Fu ; Wang, Hsiou-Hsuan ; Lin, Kao-Yung ; Kuo, Jui-Yen ; Wang, Ming-Kuang ; Liu, Cheng-Chung</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c423t-9d9a5b99f2450e785858fd8bc6733f220c2886a5c4ba638c5c87cab15efb42ab3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Activated carbon</topic><topic>Adsorbents</topic><topic>Adsorption</topic><topic>Aqueous solutions</topic><topic>Canals</topic><topic>Drainage canals</topic><topic>Dredging</topic><topic>Dyes</topic><topic>Endothermic reactions</topic><topic>Enthalpy</topic><topic>Entropy</topic><topic>Feasibility studies</topic><topic>Functional groups</topic><topic>Hazardous materials</topic><topic>Heavy metals</topic><topic>Hydrogen-Ion Concentration</topic><topic>Industrial parks</topic><topic>Infrared analysis</topic><topic>Isotherms</topic><topic>Kinetics</topic><topic>Landfills</topic><topic>Membrane separation</topic><topic>Metals</topic><topic>Methylene Blue</topic><topic>Organic matter</topic><topic>Particle size</topic><topic>Reaction kinetics</topic><topic>Removal</topic><topic>Sediment</topic><topic>Sediments</topic><topic>Soil testing</topic><topic>Sorption</topic><topic>Taiwan</topic><topic>Temperature</topic><topic>Thermodynamics</topic><topic>Waste disposal sites</topic><topic>Water Pollutants, Chemical</topic><topic>Water Purification</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chen, Lih-Fu</creatorcontrib><creatorcontrib>Wang, Hsiou-Hsuan</creatorcontrib><creatorcontrib>Lin, Kao-Yung</creatorcontrib><creatorcontrib>Kuo, Jui-Yen</creatorcontrib><creatorcontrib>Wang, Ming-Kuang</creatorcontrib><creatorcontrib>Liu, 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methylene blue from aqueous solution using sediment obtained from a canal in an industrial park</atitle><jtitle>Water science and technology</jtitle><addtitle>Water Sci Technol</addtitle><date>2018-09</date><risdate>2018</risdate><volume>78</volume><issue>3-4</issue><spage>556</spage><epage>570</epage><pages>556-570</pages><issn>0273-1223</issn><eissn>1996-9732</eissn><abstract>Drainage canal sediments in an industrial park are generally dredged to landfill in Taiwan. The objective of this study was to evaluate feasibility employing the sediment as an adsorbent for removal of dye. The sediment contained approximately 10% of organic matter and little heavy metals. Infrared (IR) analysis revealed that carboxyl was the most important functional group for methylene blue (MB) sorption. Canal sediment could remove the most MB from water at pH 8.0 and this removal increased with increasing temperature. The MB sorption was well described by the Langmuir, Dubinin-Radushkevich, and Temkin sorption isotherms at 10°C, but it showed good compliance with Freundlich isotherm at 25°C and 40°C. The MB adsorption was a spontaneous and endothermic reaction; its maximum calculated adsorption capacity (Q
) was 56.0 mg g
at 10°C by the Langmuir isotherm. The calculated values of enthalpy (ΔH°) and entropy (ΔS°) are 14.6 kJ mol
and 149.2 kJ mol
, respectively. Only pseudo-second-order adsorption kinetic model successfully described the kinetics of MB onto the sediment at different operation parameters. Activation energy of MB adsorption calculated from Arrhenius equation was 16.434 kJ mol
, indicating the binding between canal sediment and MB was a physical adsorption.</abstract><cop>England</cop><pub>IWA Publishing</pub><pmid>30207997</pmid><doi>10.2166/wst.2018.326</doi><tpages>15</tpages><oa>free_for_read</oa></addata></record> |
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| ispartof | Water science and technology, 2018-09, Vol.78 (3-4), p.556-570 |
| issn | 0273-1223 1996-9732 |
| language | eng |
| recordid | cdi_proquest_journals_2130067207 |
| source | MEDLINE; EZB-FREE-00999 freely available EZB journals |
| subjects | Activated carbon Adsorbents Adsorption Aqueous solutions Canals Drainage canals Dredging Dyes Endothermic reactions Enthalpy Entropy Feasibility studies Functional groups Hazardous materials Heavy metals Hydrogen-Ion Concentration Industrial parks Infrared analysis Isotherms Kinetics Landfills Membrane separation Metals Methylene Blue Organic matter Particle size Reaction kinetics Removal Sediment Sediments Soil testing Sorption Taiwan Temperature Thermodynamics Waste disposal sites Water Pollutants, Chemical Water Purification |
| title | Removal of methylene blue from aqueous solution using sediment obtained from a canal in an industrial park |
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