Ultrafast pump-probe force microscopy with nanoscale resolution

We perform time-resolved pump-probe microscopy measurements by recording the local force between a sharp tip and the photo-excited sample as a readout mechanism for the material's nonlinear polarization. We show that the photo-induced force is sensitive to the same excited state dynamics as mea...

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Veröffentlicht in:Applied physics letters 2015-02, Vol.106 (8)
Hauptverfasser: Jahng, Junghoon, Brocious, Jordan, Fishman, Dmitry A., Yampolsky, Steven, Nowak, Derek, Huang, Fei, Apkarian, Vartkess A., Wickramasinghe, H. Kumar, Potma, Eric Olaf
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container_issue 8
container_start_page
container_title Applied physics letters
container_volume 106
creator Jahng, Junghoon
Brocious, Jordan
Fishman, Dmitry A.
Yampolsky, Steven
Nowak, Derek
Huang, Fei
Apkarian, Vartkess A.
Wickramasinghe, H. Kumar
Potma, Eric Olaf
description We perform time-resolved pump-probe microscopy measurements by recording the local force between a sharp tip and the photo-excited sample as a readout mechanism for the material's nonlinear polarization. We show that the photo-induced force is sensitive to the same excited state dynamics as measured in an optical pump-probe experiment. Ultrafast pump-probe force microscopy constitutes a non-optical detection technique with nanoscale resolution that pushes pump-probe sensitivities close to the realm of single molecule studies.
doi_str_mv 10.1063/1.4913853
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subjects Applied physics
Microscopy
Recording
title Ultrafast pump-probe force microscopy with nanoscale resolution
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