Exciton dynamics in solid-state green fluorescent protein

We study the decay characteristics of Frenkel excitons in solid-state enhanced green fluorescent protein (eGFP) dried from solution. We further monitor the changes of the radiative exciton decay over time by crossing the phase transition from the solved to the solid state. Complex interactions betwe...

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Veröffentlicht in:Applied physics letters 2017-01, Vol.110 (4)
Hauptverfasser: Dietrich, Christof P., Siegert, Marie, Betzold, Simon, Ohmer, Jürgen, Fischer, Utz, Höfling, Sven
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container_issue 4
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container_title Applied physics letters
container_volume 110
creator Dietrich, Christof P.
Siegert, Marie
Betzold, Simon
Ohmer, Jürgen
Fischer, Utz
Höfling, Sven
description We study the decay characteristics of Frenkel excitons in solid-state enhanced green fluorescent protein (eGFP) dried from solution. We further monitor the changes of the radiative exciton decay over time by crossing the phase transition from the solved to the solid state. Complex interactions between protonated and deprotonated states in solid-state eGFP can be identified from temperature-dependent and time-resolved fluorescence experiments that further allow the determination of activation energies for each identified process.
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subjects Applied physics
Decay
Excitons
Fluorescence
Phase transitions
Proteins
Solid state
Temperature dependence
Time dependence
title Exciton dynamics in solid-state green fluorescent protein
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