Bias field effect on the temperature anomalies of dielectric permittivity in PbMg1/3Nb2/3O3- PbTiO3 single crystals

In contrast to ordinary ferroelectrics where the temperature, Tm, of the permittivity maximum monotonically increases with bias field, E, in (1-x)PbMg1/3Nb2/3O3-(x)PbTiO3 (0

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Veröffentlicht in:arXiv.org 2005-06
Hauptverfasser: Raevski, I P, Prosandeev, S A, Emelyanov, A S, Raevskaya, S I, Colla, Eugene V, Viehland, D, Kleemann, W, Vakhrushev, S B, J-L Dellis, M El Marssi, Jastrabik, L
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container_title arXiv.org
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creator Raevski, I P
Prosandeev, S A
Emelyanov, A S
Raevskaya, S I
Colla, Eugene V
Viehland, D
Kleemann, W
Vakhrushev, S B
J-L Dellis
M El Marssi
Jastrabik, L
description In contrast to ordinary ferroelectrics where the temperature, Tm, of the permittivity maximum monotonically increases with bias field, E, in (1-x)PbMg1/3Nb2/3O3-(x)PbTiO3 (0
doi_str_mv 10.48550/arxiv.0504789
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Et decreases with x and almost disappears at about x=0.4. We explain this field dependence by the quenched random fields and coupling between the orientable dipoles with average polarization. For crystals with 0.06&lt;x&lt;0.13, the T-E phase diagrams are constructed, which include the relaxor, ferroelectric, glass and mixed ferroelectric-glass phases. The boundary between the ferroelectric and relaxor phases corresponds to a first-order phase transition and is characterized by thermal hysteresis with a large curvature of the line obtained in the field cooling mode, and by the presence of the end-point above which there is no difference between the ferroelectric and relaxor phases. The glass phase has a nearly field-independent boundary in the vicinity of the Vogel-Fulcher temperature TVF. 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Et decreases with x and almost disappears at about x=0.4. We explain this field dependence by the quenched random fields and coupling between the orientable dipoles with average polarization. For crystals with 0.06&lt;x&lt;0.13, the T-E phase diagrams are constructed, which include the relaxor, ferroelectric, glass and mixed ferroelectric-glass phases. The boundary between the ferroelectric and relaxor phases corresponds to a first-order phase transition and is characterized by thermal hysteresis with a large curvature of the line obtained in the field cooling mode, and by the presence of the end-point above which there is no difference between the ferroelectric and relaxor phases. The glass phase has a nearly field-independent boundary in the vicinity of the Vogel-Fulcher temperature TVF. The coupling between the glass order parameter and polarization changes the ferroelectric boundary at temperatures lower than TV</description><subject>Anomalies</subject><subject>Bias</subject><subject>Coupling</subject><subject>Crystal structure</subject><subject>Curvature</subject><subject>Dependence</subject><subject>Dipoles</subject><subject>Ferroelectric materials</subject><subject>Ferroelectricity</subject><subject>Glass</subject><subject>Lead titanates</subject><subject>Order parameters</subject><subject>Permittivity</subject><subject>Phase diagrams</subject><subject>Phase transitions</subject><subject>Phases</subject><subject>Polarization</subject><subject>Relaxors</subject><subject>Single crystals</subject><subject>Temperature</subject><issn>2331-8422</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2005</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNqNyj1vwjAUhWELqRKoZWW-EnOIP2Iwa6tWXVoY2JEJ13BRYoPtoPLv66E_oNOro_MwNhN80RiteW3jD90XXPNmZdYjNpFKico0Uo7ZNKUL51wuV1JrNWHplWwCR9gdAZ3DNkPwkM8IGfsrRpuHiGB96G1HmCA4OBZcXKQWCugpZ7pTfgB52B6-TqJW3wdZq42qyt7RRkEif-oQ2vhI2XbphT25Epz-9ZnNP953b5_VNYbbgCnvL2GIvlx7ydd8KaQwRv1P_QKE7k_s</recordid><startdate>20050610</startdate><enddate>20050610</enddate><creator>Raevski, I P</creator><creator>Prosandeev, S A</creator><creator>Emelyanov, A S</creator><creator>Raevskaya, S I</creator><creator>Colla, Eugene V</creator><creator>Viehland, D</creator><creator>Kleemann, W</creator><creator>Vakhrushev, S B</creator><creator>J-L Dellis</creator><creator>M El Marssi</creator><creator>Jastrabik, L</creator><general>Cornell University Library, arXiv.org</general><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>L6V</scope><scope>M7S</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope></search><sort><creationdate>20050610</creationdate><title>Bias field effect on the temperature anomalies of dielectric permittivity in PbMg1/3Nb2/3O3- PbTiO3 single crystals</title><author>Raevski, I P ; 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subjects Anomalies
Bias
Coupling
Crystal structure
Curvature
Dependence
Dipoles
Ferroelectric materials
Ferroelectricity
Glass
Lead titanates
Order parameters
Permittivity
Phase diagrams
Phase transitions
Phases
Polarization
Relaxors
Single crystals
Temperature
title Bias field effect on the temperature anomalies of dielectric permittivity in PbMg1/3Nb2/3O3- PbTiO3 single crystals
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