Comparative investigations of gamma and neutron radiation shielding parameters for different borate and tellurite glass systems using WinXCom program and MCNPX code
In the present article, for different chemical compositions of B2O3‒Bi2O3, B2O3‒Sb2O3, B2O3‒WO3‒La2O3, B2O3‒MoO3‒ZnO, and TeO2‒MO (M = Mg, Ba, and Zn) glasses, by applying WinXCom program we calculated the mass attenuation coefficient (μ/ρ) values, and from these values, the effective atomic number...
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description | In the present article, for different chemical compositions of B2O3‒Bi2O3, B2O3‒Sb2O3, B2O3‒WO3‒La2O3, B2O3‒MoO3‒ZnO, and TeO2‒MO (M = Mg, Ba, and Zn) glasses, by applying WinXCom program we calculated the mass attenuation coefficient (μ/ρ) values, and from these values, the effective atomic number (Zeff), electron density (Ne), mean free path (MFP), half-value layer (HVL), and exposure buildup factor (EBF) values using Geometric progression (G‒P) fitting method, including macroscopic effective removal cross-section (ΣR) values for fast neutrons are evaluated for their potential applications as γ-ray and neutron radiation shielding materials. Moreover, the μ/ρ values of all the studied different glass compositions were computed using MCNPX simulation code and compared with WinXCom results. BBi65 glass has the highest μ/ρ, and Zeff values in the B2O3‒Bi2O3 glasses and lower values of MFP, HVL, and EBF. The maximum values of μ/ρ and Zeff are recorded for BSb70 in the B2O3‒ Sb2O3 glasses. It is found that the Zeff for B2O3‒Bi2O3 glasses is higher than those for B2O3‒ Sb2O3 glasses, which reveal that the B2O3‒Bi2O3 glasses have better shielding properties than the B2O3‒Sb2O3 glasses. The μ/ρ values of B2O3‒WO3‒La2O3 glasses are higher than those B2O3‒MoO3‒ZnO glasses, which indicate that B2O3‒WO3‒La2O3 glasses show preferable radiation shielding effectiveness comparing with B2O3‒MoO3‒ZnO glasses. The variation of different shielding parameters for the selected glasses was discussed according to the three photon interactions with matter (Photoelectric effect, Compton scattering, and pair production). The calculated μ/ρ and Zeff for the selected glasses have been compared with different glasses. HVL values are compared with ordinary, hematite-serpentine, ilmenite, steel-scrap and ilmenite-limonite concretes. It is found that ΣR values for B2O3‒Bi2O3, B2O3‒Sb2O3, B2O3‒WO3‒La2O3, B2O3‒MoO3‒ZnO, and TeO2‒MO (M = Mg, Ba, and Zn) glasses lie within the range 0.1312–0.2823 cm−1, 0.0876–0.0957 cm−1, 0.1180–0.1085 cm−1, 0.1066–0.1002 cm−1, and 0.1040–0.1075 cm−1, respectively.
[Display omitted]
•The μ/ρ increases with an increase in Bi2O3 content in the B2O3-Bi2O3 glasses.•The Zeff increases with increasing Sb2O3 modifier in the B2O3‒Sb2O3 glasses.•The μ/ρ attains maximum values at 0.015 MeV where photoelectric effect dominates.•B2O3-WO3-La2O3 glasses show better shielding effectiveness than B2O3-MoO3-ZnO glasses.•B2O3-Bi2O3 glasses show better fast neutron shielding ef |
doi_str_mv | 10.1016/j.matchemphys.2018.04.106 |
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[Display omitted]
•The μ/ρ increases with an increase in Bi2O3 content in the B2O3-Bi2O3 glasses.•The Zeff increases with increasing Sb2O3 modifier in the B2O3‒Sb2O3 glasses.•The μ/ρ attains maximum values at 0.015 MeV where photoelectric effect dominates.•B2O3-WO3-La2O3 glasses show better shielding effectiveness than B2O3-MoO3-ZnO glasses.•B2O3-Bi2O3 glasses show better fast neutron shielding effectiveness than all other glasses.</description><identifier>ISSN: 0254-0584</identifier><identifier>EISSN: 1879-3312</identifier><identifier>DOI: 10.1016/j.matchemphys.2018.04.106</identifier><language>eng</language><publisher>Lausanne: Elsevier B.V</publisher><subject>Atomic properties ; Attenuation coefficients ; Bismuth oxides ; Bismuth trioxide ; Boron oxides ; Chemical composition ; Computer simulation ; Elastic scattering ; Electron density ; Electrons ; Fast neutrons ; Gamma rays ; Glass ; Half-value layer ; Hematite ; Ilmenite ; Lanthanum oxides ; Limonite ; Magnesium ; Mass attenuation coefficient ; Mathematical analysis ; MCNPX code ; Mean free path ; Molybdenum oxides ; Neutrons ; Organic chemistry ; Pair production ; Parameters ; Photoelectric effect ; Photoelectricity ; Radiation ; Radiation shielding ; Serpentine ; WinXCom</subject><ispartof>Materials chemistry and physics, 2018-08, Vol.215, p.183-202</ispartof><rights>2018 Elsevier B.V.</rights><rights>Copyright Elsevier BV Aug 15, 2018</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c349t-529f6c4379bfefca0c08bf3ace421750ed60c63073b4383cd190beca9667c203</citedby><cites>FETCH-LOGICAL-c349t-529f6c4379bfefca0c08bf3ace421750ed60c63073b4383cd190beca9667c203</cites><orcidid>0000-0002-1458-9368</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.matchemphys.2018.04.106$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3548,27922,27923,45993</link.rule.ids></links><search><creatorcontrib>Sayyed, M.I.</creatorcontrib><creatorcontrib>Dong, M.G.</creatorcontrib><creatorcontrib>Tekin, H.O.</creatorcontrib><creatorcontrib>Lakshminarayana, G.</creatorcontrib><creatorcontrib>Mahdi, M.A.</creatorcontrib><title>Comparative investigations of gamma and neutron radiation shielding parameters for different borate and tellurite glass systems using WinXCom program and MCNPX code</title><title>Materials chemistry and physics</title><description>In the present article, for different chemical compositions of B2O3‒Bi2O3, B2O3‒Sb2O3, B2O3‒WO3‒La2O3, B2O3‒MoO3‒ZnO, and TeO2‒MO (M = Mg, Ba, and Zn) glasses, by applying WinXCom program we calculated the mass attenuation coefficient (μ/ρ) values, and from these values, the effective atomic number (Zeff), electron density (Ne), mean free path (MFP), half-value layer (HVL), and exposure buildup factor (EBF) values using Geometric progression (G‒P) fitting method, including macroscopic effective removal cross-section (ΣR) values for fast neutrons are evaluated for their potential applications as γ-ray and neutron radiation shielding materials. Moreover, the μ/ρ values of all the studied different glass compositions were computed using MCNPX simulation code and compared with WinXCom results. BBi65 glass has the highest μ/ρ, and Zeff values in the B2O3‒Bi2O3 glasses and lower values of MFP, HVL, and EBF. The maximum values of μ/ρ and Zeff are recorded for BSb70 in the B2O3‒ Sb2O3 glasses. It is found that the Zeff for B2O3‒Bi2O3 glasses is higher than those for B2O3‒ Sb2O3 glasses, which reveal that the B2O3‒Bi2O3 glasses have better shielding properties than the B2O3‒Sb2O3 glasses. The μ/ρ values of B2O3‒WO3‒La2O3 glasses are higher than those B2O3‒MoO3‒ZnO glasses, which indicate that B2O3‒WO3‒La2O3 glasses show preferable radiation shielding effectiveness comparing with B2O3‒MoO3‒ZnO glasses. The variation of different shielding parameters for the selected glasses was discussed according to the three photon interactions with matter (Photoelectric effect, Compton scattering, and pair production). The calculated μ/ρ and Zeff for the selected glasses have been compared with different glasses. HVL values are compared with ordinary, hematite-serpentine, ilmenite, steel-scrap and ilmenite-limonite concretes. It is found that ΣR values for B2O3‒Bi2O3, B2O3‒Sb2O3, B2O3‒WO3‒La2O3, B2O3‒MoO3‒ZnO, and TeO2‒MO (M = Mg, Ba, and Zn) glasses lie within the range 0.1312–0.2823 cm−1, 0.0876–0.0957 cm−1, 0.1180–0.1085 cm−1, 0.1066–0.1002 cm−1, and 0.1040–0.1075 cm−1, respectively.
[Display omitted]
•The μ/ρ increases with an increase in Bi2O3 content in the B2O3-Bi2O3 glasses.•The Zeff increases with increasing Sb2O3 modifier in the B2O3‒Sb2O3 glasses.•The μ/ρ attains maximum values at 0.015 MeV where photoelectric effect dominates.•B2O3-WO3-La2O3 glasses show better shielding effectiveness than B2O3-MoO3-ZnO glasses.•B2O3-Bi2O3 glasses show better fast neutron shielding effectiveness than all other glasses.</description><subject>Atomic properties</subject><subject>Attenuation coefficients</subject><subject>Bismuth oxides</subject><subject>Bismuth trioxide</subject><subject>Boron oxides</subject><subject>Chemical composition</subject><subject>Computer simulation</subject><subject>Elastic scattering</subject><subject>Electron density</subject><subject>Electrons</subject><subject>Fast neutrons</subject><subject>Gamma rays</subject><subject>Glass</subject><subject>Half-value layer</subject><subject>Hematite</subject><subject>Ilmenite</subject><subject>Lanthanum oxides</subject><subject>Limonite</subject><subject>Magnesium</subject><subject>Mass attenuation coefficient</subject><subject>Mathematical analysis</subject><subject>MCNPX code</subject><subject>Mean free path</subject><subject>Molybdenum oxides</subject><subject>Neutrons</subject><subject>Organic chemistry</subject><subject>Pair production</subject><subject>Parameters</subject><subject>Photoelectric effect</subject><subject>Photoelectricity</subject><subject>Radiation</subject><subject>Radiation shielding</subject><subject>Serpentine</subject><subject>WinXCom</subject><issn>0254-0584</issn><issn>1879-3312</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNqNkU1u2zAQhYmiBeokvQOLruUORVk_y0JImwJpm0WAZEdQ5FCmIZEOSRnwfXrQ0HYXWXZFDN68jzPzCPnMYM2A1V9361kmtcV5vz3GdQmsXUOVpfodWbG26QrOWfmerKDcVAVs2uojuYpxB8AaxviK_O39vJdBJntAat0BY7JjrryL1Bs6ynmWVDpNHS4peEeD1Pas07i1OGnrRnoCzJgwRGp8oNoagwFdooPPZDz7E07TEmyuxknGSOMxJpwjXeKJ8GTdc56E7oMfM-vs-NX_fnimymu8IR-MnCJ--vdek8fvt4_9XXH_58fP_tt9oXjVpWJTdqZWFW-6waBREhS0g-FSYVWyZgOoa1A1h4YPFW-50qyDAZXs6rpRJfBr8uWCzVO8LPkSYueX4PKPooS2yVzO2tzVXbpU8DEGNGIf7CzDUTAQp0zETrzJRJwyEVBlqc7e_uLFvMXBYhBRWXQKtQ2oktDe_gflFThDoBA</recordid><startdate>20180815</startdate><enddate>20180815</enddate><creator>Sayyed, M.I.</creator><creator>Dong, M.G.</creator><creator>Tekin, H.O.</creator><creator>Lakshminarayana, G.</creator><creator>Mahdi, M.A.</creator><general>Elsevier B.V</general><general>Elsevier BV</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0002-1458-9368</orcidid></search><sort><creationdate>20180815</creationdate><title>Comparative investigations of gamma and neutron radiation shielding parameters for different borate and tellurite glass systems using WinXCom program and MCNPX code</title><author>Sayyed, M.I. ; Dong, M.G. ; Tekin, H.O. ; Lakshminarayana, G. ; Mahdi, M.A.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c349t-529f6c4379bfefca0c08bf3ace421750ed60c63073b4383cd190beca9667c203</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Atomic properties</topic><topic>Attenuation coefficients</topic><topic>Bismuth oxides</topic><topic>Bismuth trioxide</topic><topic>Boron oxides</topic><topic>Chemical composition</topic><topic>Computer simulation</topic><topic>Elastic scattering</topic><topic>Electron density</topic><topic>Electrons</topic><topic>Fast neutrons</topic><topic>Gamma rays</topic><topic>Glass</topic><topic>Half-value layer</topic><topic>Hematite</topic><topic>Ilmenite</topic><topic>Lanthanum oxides</topic><topic>Limonite</topic><topic>Magnesium</topic><topic>Mass attenuation coefficient</topic><topic>Mathematical analysis</topic><topic>MCNPX code</topic><topic>Mean free path</topic><topic>Molybdenum oxides</topic><topic>Neutrons</topic><topic>Organic chemistry</topic><topic>Pair production</topic><topic>Parameters</topic><topic>Photoelectric effect</topic><topic>Photoelectricity</topic><topic>Radiation</topic><topic>Radiation shielding</topic><topic>Serpentine</topic><topic>WinXCom</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Sayyed, M.I.</creatorcontrib><creatorcontrib>Dong, M.G.</creatorcontrib><creatorcontrib>Tekin, H.O.</creatorcontrib><creatorcontrib>Lakshminarayana, G.</creatorcontrib><creatorcontrib>Mahdi, M.A.</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Materials chemistry and physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Sayyed, M.I.</au><au>Dong, M.G.</au><au>Tekin, H.O.</au><au>Lakshminarayana, G.</au><au>Mahdi, M.A.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Comparative investigations of gamma and neutron radiation shielding parameters for different borate and tellurite glass systems using WinXCom program and MCNPX code</atitle><jtitle>Materials chemistry and physics</jtitle><date>2018-08-15</date><risdate>2018</risdate><volume>215</volume><spage>183</spage><epage>202</epage><pages>183-202</pages><issn>0254-0584</issn><eissn>1879-3312</eissn><abstract>In the present article, for different chemical compositions of B2O3‒Bi2O3, B2O3‒Sb2O3, B2O3‒WO3‒La2O3, B2O3‒MoO3‒ZnO, and TeO2‒MO (M = Mg, Ba, and Zn) glasses, by applying WinXCom program we calculated the mass attenuation coefficient (μ/ρ) values, and from these values, the effective atomic number (Zeff), electron density (Ne), mean free path (MFP), half-value layer (HVL), and exposure buildup factor (EBF) values using Geometric progression (G‒P) fitting method, including macroscopic effective removal cross-section (ΣR) values for fast neutrons are evaluated for their potential applications as γ-ray and neutron radiation shielding materials. Moreover, the μ/ρ values of all the studied different glass compositions were computed using MCNPX simulation code and compared with WinXCom results. BBi65 glass has the highest μ/ρ, and Zeff values in the B2O3‒Bi2O3 glasses and lower values of MFP, HVL, and EBF. The maximum values of μ/ρ and Zeff are recorded for BSb70 in the B2O3‒ Sb2O3 glasses. It is found that the Zeff for B2O3‒Bi2O3 glasses is higher than those for B2O3‒ Sb2O3 glasses, which reveal that the B2O3‒Bi2O3 glasses have better shielding properties than the B2O3‒Sb2O3 glasses. The μ/ρ values of B2O3‒WO3‒La2O3 glasses are higher than those B2O3‒MoO3‒ZnO glasses, which indicate that B2O3‒WO3‒La2O3 glasses show preferable radiation shielding effectiveness comparing with B2O3‒MoO3‒ZnO glasses. The variation of different shielding parameters for the selected glasses was discussed according to the three photon interactions with matter (Photoelectric effect, Compton scattering, and pair production). The calculated μ/ρ and Zeff for the selected glasses have been compared with different glasses. HVL values are compared with ordinary, hematite-serpentine, ilmenite, steel-scrap and ilmenite-limonite concretes. It is found that ΣR values for B2O3‒Bi2O3, B2O3‒Sb2O3, B2O3‒WO3‒La2O3, B2O3‒MoO3‒ZnO, and TeO2‒MO (M = Mg, Ba, and Zn) glasses lie within the range 0.1312–0.2823 cm−1, 0.0876–0.0957 cm−1, 0.1180–0.1085 cm−1, 0.1066–0.1002 cm−1, and 0.1040–0.1075 cm−1, respectively.
[Display omitted]
•The μ/ρ increases with an increase in Bi2O3 content in the B2O3-Bi2O3 glasses.•The Zeff increases with increasing Sb2O3 modifier in the B2O3‒Sb2O3 glasses.•The μ/ρ attains maximum values at 0.015 MeV where photoelectric effect dominates.•B2O3-WO3-La2O3 glasses show better shielding effectiveness than B2O3-MoO3-ZnO glasses.•B2O3-Bi2O3 glasses show better fast neutron shielding effectiveness than all other glasses.</abstract><cop>Lausanne</cop><pub>Elsevier B.V</pub><doi>10.1016/j.matchemphys.2018.04.106</doi><tpages>20</tpages><orcidid>https://orcid.org/0000-0002-1458-9368</orcidid></addata></record> |
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subjects | Atomic properties Attenuation coefficients Bismuth oxides Bismuth trioxide Boron oxides Chemical composition Computer simulation Elastic scattering Electron density Electrons Fast neutrons Gamma rays Glass Half-value layer Hematite Ilmenite Lanthanum oxides Limonite Magnesium Mass attenuation coefficient Mathematical analysis MCNPX code Mean free path Molybdenum oxides Neutrons Organic chemistry Pair production Parameters Photoelectric effect Photoelectricity Radiation Radiation shielding Serpentine WinXCom |
title | Comparative investigations of gamma and neutron radiation shielding parameters for different borate and tellurite glass systems using WinXCom program and MCNPX code |
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