Realization of an all-optically controlled dynamic superlattice for exciton-polaritons

Exciton-polaritons, formed by the strong coupling between excitons and cavity-confined photons, are the building blocks of polaritonic devices. In this work, we report experimental realization of an all-optically controlled dynamic superlattice for polaritons working in the ultraviolet wavelength ra...

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Veröffentlicht in:Nanoscale 2018-08, Vol.1 (29), p.1482-1489
Hauptverfasser: Zhang, Yingjun, Zhang, Xinhan, Tang, Bing, Tian, Chuan, Xu, Chunyan, Dong, Hongxing, Zhou, Weihang
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container_end_page 1489
container_issue 29
container_start_page 1482
container_title Nanoscale
container_volume 1
creator Zhang, Yingjun
Zhang, Xinhan
Tang, Bing
Tian, Chuan
Xu, Chunyan
Dong, Hongxing
Zhou, Weihang
description Exciton-polaritons, formed by the strong coupling between excitons and cavity-confined photons, are the building blocks of polaritonic devices. In this work, we report experimental realization of an all-optically controlled dynamic superlattice for polaritons working in the ultraviolet wavelength range at room temperature. The optical superlattice was realized on a one-dimensional (1D) ZnO microrod using an array of periodically arranged laser spots. Polaritonic mini-band features were clearly observed by both momentum- and real-space imaging spectroscopy. By controlling the periodicity of the laser spots, we demonstrated that the band structures of polaritons can be well controlled by external lasers. Theoretically, by extending the Kronig-Penney model to the polariton system, we calculated the polaritonic mini-bands and found it to be in good agreement with our experimental observations. By imaging the polariton flow in real space, the lifetime of polaritons and their relationship with their exitonic fractions were also extracted. The polaritonic superlattices demonstrated in this work are fully reconfigurable and optically controlled, and our results could thus stimulate the development of polaritonic all-optical devices. An optically-controlled and fully reconfigurable dynamic superlattice was realized on a one-dimensional ZnO microrod for exciton-polaritons.
doi_str_mv 10.1039/c8nr02190b
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In this work, we report experimental realization of an all-optically controlled dynamic superlattice for polaritons working in the ultraviolet wavelength range at room temperature. The optical superlattice was realized on a one-dimensional (1D) ZnO microrod using an array of periodically arranged laser spots. Polaritonic mini-band features were clearly observed by both momentum- and real-space imaging spectroscopy. By controlling the periodicity of the laser spots, we demonstrated that the band structures of polaritons can be well controlled by external lasers. Theoretically, by extending the Kronig-Penney model to the polariton system, we calculated the polaritonic mini-bands and found it to be in good agreement with our experimental observations. By imaging the polariton flow in real space, the lifetime of polaritons and their relationship with their exitonic fractions were also extracted. The polaritonic superlattices demonstrated in this work are fully reconfigurable and optically controlled, and our results could thus stimulate the development of polaritonic all-optical devices. 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source Royal Society Of Chemistry Journals
subjects Excitons
Laser arrays
Periodic variations
Photons
Polaritons
Superlattices
Zinc oxide
title Realization of an all-optically controlled dynamic superlattice for exciton-polaritons
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