Magnetic properties of rare-earth sulfide YbAgS^sub 2
We have succeeded in synthesizing single-phase polycrystalline samples of YbAgS2 belonging to the tetragonal system with space group I41 md . YbAgS2 shows an antiferromagnetic transition at TN = 6.6 K . The effective magnetic moment is in good agreement with the theoretical value for Yb3+ free ion....
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Veröffentlicht in: | Physica. B, Condensed matter Condensed matter, 2018-05, Vol.536, p.314 |
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creator | Iizuka, Ryosuke Numakura, Ryosuke Michimura, Shinji Katano, Susumu Kosaka, Masashi |
description | We have succeeded in synthesizing single-phase polycrystalline samples of YbAgS2 belonging to the tetragonal system with space group I41 md . YbAgS2 shows an antiferromagnetic transition at TN = 6.6 K . The effective magnetic moment is in good agreement with the theoretical value for Yb3+ free ion. A broad anomaly is observed just above TN in the temperature dependence of magnetic susceptibility. The entropy released at TN is only about half of Rln2 expected for a Kramers doublet ground state. We consider that these phenomena are due to the existence of short-range magnetic correlations rather than the partial screening of the Yb moments by conduction electrons via the Kondo effect. |
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YbAgS2 shows an antiferromagnetic transition at TN = 6.6 K . The effective magnetic moment is in good agreement with the theoretical value for Yb3+ free ion. A broad anomaly is observed just above TN in the temperature dependence of magnetic susceptibility. The entropy released at TN is only about half of Rln2 expected for a Kramers doublet ground state. We consider that these phenomena are due to the existence of short-range magnetic correlations rather than the partial screening of the Yb moments by conduction electrons via the Kondo effect.</description><identifier>ISSN: 0921-4526</identifier><identifier>EISSN: 1873-2135</identifier><language>eng</language><publisher>Amsterdam: Elsevier BV</publisher><subject>Antiferromagnetism ; Conduction electrons ; Entropy ; Intermetallic compounds ; Kondo effect ; Magnetic moments ; Magnetic permeability ; Magnetic properties ; Magnetism ; Rare earth elements ; Temperature ; Temperature dependence ; Trace elements</subject><ispartof>Physica. 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The effective magnetic moment is in good agreement with the theoretical value for Yb3+ free ion. A broad anomaly is observed just above TN in the temperature dependence of magnetic susceptibility. The entropy released at TN is only about half of Rln2 expected for a Kramers doublet ground state. We consider that these phenomena are due to the existence of short-range magnetic correlations rather than the partial screening of the Yb moments by conduction electrons via the Kondo effect.</description><subject>Antiferromagnetism</subject><subject>Conduction electrons</subject><subject>Entropy</subject><subject>Intermetallic compounds</subject><subject>Kondo effect</subject><subject>Magnetic moments</subject><subject>Magnetic permeability</subject><subject>Magnetic properties</subject><subject>Magnetism</subject><subject>Rare earth elements</subject><subject>Temperature</subject><subject>Temperature dependence</subject><subject>Trace elements</subject><issn>0921-4526</issn><issn>1873-2135</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNpjYuA0tDA31jUyNDZlYeA0sDQy1DUxNTLjYOAqLs4yAAJDc0NOBlPfxPS81JLMZIWCovyC1KKSzNRihfw0haLEolTd1MSikgyF4tKctMyUVIXIJMf04Lji0iQFIx4G1rTEnOJUXijNzaDs5hri7KELNKSwNLW4JD4rv7QoDygVb2RgbmZkYGhpbG5MnCoARAs1qQ</recordid><startdate>20180501</startdate><enddate>20180501</enddate><creator>Iizuka, Ryosuke</creator><creator>Numakura, Ryosuke</creator><creator>Michimura, Shinji</creator><creator>Katano, Susumu</creator><creator>Kosaka, Masashi</creator><general>Elsevier BV</general><scope>7U5</scope><scope>8FD</scope><scope>L7M</scope></search><sort><creationdate>20180501</creationdate><title>Magnetic properties of rare-earth sulfide YbAgS^sub 2</title><author>Iizuka, Ryosuke ; Numakura, Ryosuke ; Michimura, Shinji ; Katano, Susumu ; Kosaka, Masashi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-proquest_journals_20762019373</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Antiferromagnetism</topic><topic>Conduction electrons</topic><topic>Entropy</topic><topic>Intermetallic compounds</topic><topic>Kondo effect</topic><topic>Magnetic moments</topic><topic>Magnetic permeability</topic><topic>Magnetic properties</topic><topic>Magnetism</topic><topic>Rare earth elements</topic><topic>Temperature</topic><topic>Temperature dependence</topic><topic>Trace elements</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Iizuka, Ryosuke</creatorcontrib><creatorcontrib>Numakura, Ryosuke</creatorcontrib><creatorcontrib>Michimura, Shinji</creatorcontrib><creatorcontrib>Katano, Susumu</creatorcontrib><creatorcontrib>Kosaka, Masashi</creatorcontrib><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Physica. B, Condensed matter</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Iizuka, Ryosuke</au><au>Numakura, Ryosuke</au><au>Michimura, Shinji</au><au>Katano, Susumu</au><au>Kosaka, Masashi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Magnetic properties of rare-earth sulfide YbAgS^sub 2</atitle><jtitle>Physica. B, Condensed matter</jtitle><date>2018-05-01</date><risdate>2018</risdate><volume>536</volume><spage>314</spage><pages>314-</pages><issn>0921-4526</issn><eissn>1873-2135</eissn><abstract>We have succeeded in synthesizing single-phase polycrystalline samples of YbAgS2 belonging to the tetragonal system with space group I41 md . YbAgS2 shows an antiferromagnetic transition at TN = 6.6 K . The effective magnetic moment is in good agreement with the theoretical value for Yb3+ free ion. A broad anomaly is observed just above TN in the temperature dependence of magnetic susceptibility. The entropy released at TN is only about half of Rln2 expected for a Kramers doublet ground state. We consider that these phenomena are due to the existence of short-range magnetic correlations rather than the partial screening of the Yb moments by conduction electrons via the Kondo effect.</abstract><cop>Amsterdam</cop><pub>Elsevier BV</pub></addata></record> |
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subjects | Antiferromagnetism Conduction electrons Entropy Intermetallic compounds Kondo effect Magnetic moments Magnetic permeability Magnetic properties Magnetism Rare earth elements Temperature Temperature dependence Trace elements |
title | Magnetic properties of rare-earth sulfide YbAgS^sub 2 |
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