Preparation, adsorption and recognition properties of uranyl ion-imprinted marine facultative fungus mainly modified by phytic acid and tetraethyl silicate
Uranyl ion-imprinted polymers (U(VI)-IIPs) were successfully prepared by combining phytic acid as the functional monomer, uranyl ion (UO 2 2+ ) as the template, and tetraethyl silicate (TEOS) as the cross-linker with the marine facultative fungus Fusarium sp. #ZZF51 addicted to U (VI) mycelium throu...
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| Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2018-08, Vol.317 (2), p.701-714 |
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| container_title | Journal of radioanalytical and nuclear chemistry |
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| creator | Zhang, W. Tan, N. Hou, D. Lin, Y. W. Yan, X. M. Gao, Y. He, D. X. Jiang, M. Wang, J. |
| description | Uranyl ion-imprinted polymers (U(VI)-IIPs) were successfully prepared by combining phytic acid as the functional monomer, uranyl ion (UO
2
2+
) as the template, and tetraethyl silicate (TEOS) as the cross-linker with the marine facultative fungus
Fusarium
sp. #ZZF51 addicted to U (VI) mycelium through the ion-imprinted sol–gel method. Single-factor experiments were performed to optimize the preparation conditions and the prepared materials were better characterized with FTIR, SEM and BET meter. The optimum adsorption conditions were explored by single-factor experiments and BBD response surface method in detail. The adsorption–desorption recycling and adsorption selectivity experiments revealed that U(VI)-IIPs had a good stability and selectivity. The U (VI) adsorption process of U(VI)-IIPs was better described by the pseudo-second order kinetic equation and Langmuir isotherm model. |
| doi_str_mv | 10.1007/s10967-018-5937-7 |
| format | Article |
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2
2+
) as the template, and tetraethyl silicate (TEOS) as the cross-linker with the marine facultative fungus
Fusarium
sp. #ZZF51 addicted to U (VI) mycelium through the ion-imprinted sol–gel method. Single-factor experiments were performed to optimize the preparation conditions and the prepared materials were better characterized with FTIR, SEM and BET meter. The optimum adsorption conditions were explored by single-factor experiments and BBD response surface method in detail. The adsorption–desorption recycling and adsorption selectivity experiments revealed that U(VI)-IIPs had a good stability and selectivity. The U (VI) adsorption process of U(VI)-IIPs was better described by the pseudo-second order kinetic equation and Langmuir isotherm model.</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-018-5937-7</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Adsorption ; Analysis ; Chemistry ; Chemistry and Materials Science ; Crosslinking ; Diagnostic Radiology ; Experiments ; Fungi ; Hadrons ; Heavy Ions ; Imprinted polymers ; Inorganic Chemistry ; Kinetic equations ; Nuclear Chemistry ; Nuclear Physics ; Optimization ; Phosphates ; Physical Chemistry ; Phytic acid ; Response surface methodology ; Selectivity ; Silicates ; Sol-gel processes ; Sorption ; Tetraethyl orthosilicate ; Uranium</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2018-08, Vol.317 (2), p.701-714</ispartof><rights>Akadémiai Kiadó, Budapest, Hungary 2018</rights><rights>COPYRIGHT 2018 Springer</rights><rights>Copyright Springer Science & Business Media 2018</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c355t-c1ed2fef096af921d4d3f19db3ca9e2d2d4edc117442ec34483c6a08e109500d3</citedby><cites>FETCH-LOGICAL-c355t-c1ed2fef096af921d4d3f19db3ca9e2d2d4edc117442ec34483c6a08e109500d3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10967-018-5937-7$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10967-018-5937-7$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Zhang, W.</creatorcontrib><creatorcontrib>Tan, N.</creatorcontrib><creatorcontrib>Hou, D.</creatorcontrib><creatorcontrib>Lin, Y. W.</creatorcontrib><creatorcontrib>Yan, X. M.</creatorcontrib><creatorcontrib>Gao, Y.</creatorcontrib><creatorcontrib>He, D. X.</creatorcontrib><creatorcontrib>Jiang, M.</creatorcontrib><creatorcontrib>Wang, J.</creatorcontrib><title>Preparation, adsorption and recognition properties of uranyl ion-imprinted marine facultative fungus mainly modified by phytic acid and tetraethyl silicate</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>Uranyl ion-imprinted polymers (U(VI)-IIPs) were successfully prepared by combining phytic acid as the functional monomer, uranyl ion (UO
2
2+
) as the template, and tetraethyl silicate (TEOS) as the cross-linker with the marine facultative fungus
Fusarium
sp. #ZZF51 addicted to U (VI) mycelium through the ion-imprinted sol–gel method. Single-factor experiments were performed to optimize the preparation conditions and the prepared materials were better characterized with FTIR, SEM and BET meter. The optimum adsorption conditions were explored by single-factor experiments and BBD response surface method in detail. The adsorption–desorption recycling and adsorption selectivity experiments revealed that U(VI)-IIPs had a good stability and selectivity. The U (VI) adsorption process of U(VI)-IIPs was better described by the pseudo-second order kinetic equation and Langmuir isotherm model.</description><subject>Adsorption</subject><subject>Analysis</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Crosslinking</subject><subject>Diagnostic Radiology</subject><subject>Experiments</subject><subject>Fungi</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>Imprinted polymers</subject><subject>Inorganic Chemistry</subject><subject>Kinetic equations</subject><subject>Nuclear Chemistry</subject><subject>Nuclear Physics</subject><subject>Optimization</subject><subject>Phosphates</subject><subject>Physical Chemistry</subject><subject>Phytic acid</subject><subject>Response surface methodology</subject><subject>Selectivity</subject><subject>Silicates</subject><subject>Sol-gel processes</subject><subject>Sorption</subject><subject>Tetraethyl orthosilicate</subject><subject>Uranium</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNp1UU1v3CAQRVErZZv0B_SG1Gud8GEv-BhFbVopUnpozojAsCHyggu4kn9L_2xn40o9VRyYYea9Gd4j5ANnV5wxdV05G_eqY1x3wyhVp87Ijg9ad0Jp9obsmJD7blCSn5N3tb4wxkat5Y78_l5gtsW2mNMnan3NZT7F1CZPC7h8SPE1n0ueobQIleZAl2LTOlEsdPE4l5gaeHq0GAAN1i1TQ8ZfGC_psFSsxDSt9Jh9DBE7n1Y6P68tOmpd9K-zGrRioT0ja41TdLbBJXkb7FTh_d_7gjx--fzj9mt3_3D37fbmvnNyGFrnOHgRIKAANoyC-97LwEf_JJ0dQXjhe_COc9X3Apzsey3d3jINKNnAmJcX5OPGi3_8uUBt5iUvJeFII5hielBM9Nh1tXUd7AQmppBxYYfHwzG6nCBEfL8Z-r3q9aAZAvgGcCXXWiAYFAo1Wg1n5mSa2UwzaJo5mWYUYsSGqSdRD1D-rfJ_0B-T-J54</recordid><startdate>20180801</startdate><enddate>20180801</enddate><creator>Zhang, W.</creator><creator>Tan, N.</creator><creator>Hou, D.</creator><creator>Lin, Y. W.</creator><creator>Yan, X. M.</creator><creator>Gao, Y.</creator><creator>He, D. X.</creator><creator>Jiang, M.</creator><creator>Wang, J.</creator><general>Springer International Publishing</general><general>Springer</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20180801</creationdate><title>Preparation, adsorption and recognition properties of uranyl ion-imprinted marine facultative fungus mainly modified by phytic acid and tetraethyl silicate</title><author>Zhang, W. ; Tan, N. ; Hou, D. ; Lin, Y. W. ; Yan, X. M. ; Gao, Y. ; He, D. X. ; Jiang, M. ; Wang, J.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c355t-c1ed2fef096af921d4d3f19db3ca9e2d2d4edc117442ec34483c6a08e109500d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Adsorption</topic><topic>Analysis</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Crosslinking</topic><topic>Diagnostic Radiology</topic><topic>Experiments</topic><topic>Fungi</topic><topic>Hadrons</topic><topic>Heavy Ions</topic><topic>Imprinted polymers</topic><topic>Inorganic Chemistry</topic><topic>Kinetic equations</topic><topic>Nuclear Chemistry</topic><topic>Nuclear Physics</topic><topic>Optimization</topic><topic>Phosphates</topic><topic>Physical Chemistry</topic><topic>Phytic acid</topic><topic>Response surface methodology</topic><topic>Selectivity</topic><topic>Silicates</topic><topic>Sol-gel processes</topic><topic>Sorption</topic><topic>Tetraethyl orthosilicate</topic><topic>Uranium</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, W.</creatorcontrib><creatorcontrib>Tan, N.</creatorcontrib><creatorcontrib>Hou, D.</creatorcontrib><creatorcontrib>Lin, Y. W.</creatorcontrib><creatorcontrib>Yan, X. M.</creatorcontrib><creatorcontrib>Gao, Y.</creatorcontrib><creatorcontrib>He, D. X.</creatorcontrib><creatorcontrib>Jiang, M.</creatorcontrib><creatorcontrib>Wang, J.</creatorcontrib><collection>CrossRef</collection><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhang, W.</au><au>Tan, N.</au><au>Hou, D.</au><au>Lin, Y. W.</au><au>Yan, X. M.</au><au>Gao, Y.</au><au>He, D. X.</au><au>Jiang, M.</au><au>Wang, J.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Preparation, adsorption and recognition properties of uranyl ion-imprinted marine facultative fungus mainly modified by phytic acid and tetraethyl silicate</atitle><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle><stitle>J Radioanal Nucl Chem</stitle><date>2018-08-01</date><risdate>2018</risdate><volume>317</volume><issue>2</issue><spage>701</spage><epage>714</epage><pages>701-714</pages><issn>0236-5731</issn><eissn>1588-2780</eissn><abstract>Uranyl ion-imprinted polymers (U(VI)-IIPs) were successfully prepared by combining phytic acid as the functional monomer, uranyl ion (UO
2
2+
) as the template, and tetraethyl silicate (TEOS) as the cross-linker with the marine facultative fungus
Fusarium
sp. #ZZF51 addicted to U (VI) mycelium through the ion-imprinted sol–gel method. Single-factor experiments were performed to optimize the preparation conditions and the prepared materials were better characterized with FTIR, SEM and BET meter. The optimum adsorption conditions were explored by single-factor experiments and BBD response surface method in detail. The adsorption–desorption recycling and adsorption selectivity experiments revealed that U(VI)-IIPs had a good stability and selectivity. The U (VI) adsorption process of U(VI)-IIPs was better described by the pseudo-second order kinetic equation and Langmuir isotherm model.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s10967-018-5937-7</doi><tpages>14</tpages></addata></record> |
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| ispartof | Journal of radioanalytical and nuclear chemistry, 2018-08, Vol.317 (2), p.701-714 |
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| language | eng |
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| source | Springer Nature - Complete Springer Journals |
| subjects | Adsorption Analysis Chemistry Chemistry and Materials Science Crosslinking Diagnostic Radiology Experiments Fungi Hadrons Heavy Ions Imprinted polymers Inorganic Chemistry Kinetic equations Nuclear Chemistry Nuclear Physics Optimization Phosphates Physical Chemistry Phytic acid Response surface methodology Selectivity Silicates Sol-gel processes Sorption Tetraethyl orthosilicate Uranium |
| title | Preparation, adsorption and recognition properties of uranyl ion-imprinted marine facultative fungus mainly modified by phytic acid and tetraethyl silicate |
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