Paper-based electrochemical sensor for on-site detection of the sulphur mustard
Herein, we report a novel paper-based electrochemical sensor for on-site detection of sulphur mustards. This sensor was conceived combining office paper-based electrochemical sensor with choline oxidase enzyme to deliver a sustainable sensing tool. The mustard agent detection relies on the evaluatio...
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| Veröffentlicht in: | Environmental science and pollution research international 2021-05, Vol.28 (20), p.25069-25080 |
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| creator | Colozza, Noemi Kehe, Kai Popp, Tanja Steinritz, Dirk Moscone, Danila Arduini, Fabiana |
| description | Herein, we report a novel paper-based electrochemical sensor for on-site detection of sulphur mustards. This sensor was conceived combining office paper-based electrochemical sensor with choline oxidase enzyme to deliver a sustainable sensing tool. The mustard agent detection relies on the evaluation of inhibition degree of choline oxidase, which is reversibly inhibited by sulphur mustards, by measuring the enzymatic by-product H
2
O
2
in chronoamperometric mode. A nanocomposite constituted of Prussian Blue nanoparticles and Carbon Black was used as working electrode modifier to improve the electroanalytical performances. This bioassay was successfully applied for the measurement of a sulphur mustard, Yprite, obtaining a detection limit in the millimolar range (LOD = 0.9 mM). The developed sensor, combined with a portable and easy-to-use instrumentation, can be applied for a fast and cost-effective detection of sulphur mustards. |
| doi_str_mv | 10.1007/s11356-018-2545-6 |
| format | Article |
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2
O
2
in chronoamperometric mode. A nanocomposite constituted of Prussian Blue nanoparticles and Carbon Black was used as working electrode modifier to improve the electroanalytical performances. This bioassay was successfully applied for the measurement of a sulphur mustard, Yprite, obtaining a detection limit in the millimolar range (LOD = 0.9 mM). The developed sensor, combined with a portable and easy-to-use instrumentation, can be applied for a fast and cost-effective detection of sulphur mustards.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-018-2545-6</identifier><identifier>PMID: 29934830</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Bioassays ; Black carbon ; Carbon black ; Chemical sensors ; Choline ; Choline oxidase ; Earth and Environmental Science ; Ecotoxicology ; Electrochemistry ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Environmental Sciences ; Environmental Sciences & Ecology ; Hydrogen peroxide ; Instrumentation ; Life Sciences & Biomedicine ; Mustard gas ; Nanocomposites ; Nanoparticles ; Onsite ; Oxidase ; Pigments ; Research Article ; Science & Technology ; Sensors ; Sulfur ; Waste Water Technology ; Water Management ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2021-05, Vol.28 (20), p.25069-25080</ispartof><rights>Springer-Verlag GmbH Germany, part of Springer Nature 2018</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, (2018). All Rights Reserved.</rights><rights>Springer-Verlag GmbH Germany, part of Springer Nature 2018.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>true</woscitedreferencessubscribed><woscitedreferencescount>13</woscitedreferencescount><woscitedreferencesoriginalsourcerecordid>wos000655219700012</woscitedreferencesoriginalsourcerecordid><citedby>FETCH-LOGICAL-c437t-98df439c8cf15480b08aaed93c7062fdd8d5fca608ffe78c5d78750dc003efb43</citedby><cites>FETCH-LOGICAL-c437t-98df439c8cf15480b08aaed93c7062fdd8d5fca608ffe78c5d78750dc003efb43</cites><orcidid>0000-0002-9028-3870 ; 0000-0002-2073-5683 ; 0000-0002-5497-6557</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-018-2545-6$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-018-2545-6$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>315,782,786,27931,27932,39265,41495,42564,51326</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/29934830$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Colozza, Noemi</creatorcontrib><creatorcontrib>Kehe, Kai</creatorcontrib><creatorcontrib>Popp, Tanja</creatorcontrib><creatorcontrib>Steinritz, Dirk</creatorcontrib><creatorcontrib>Moscone, Danila</creatorcontrib><creatorcontrib>Arduini, Fabiana</creatorcontrib><title>Paper-based electrochemical sensor for on-site detection of the sulphur mustard</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>ENVIRON SCI POLLUT R</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Herein, we report a novel paper-based electrochemical sensor for on-site detection of sulphur mustards. This sensor was conceived combining office paper-based electrochemical sensor with choline oxidase enzyme to deliver a sustainable sensing tool. The mustard agent detection relies on the evaluation of inhibition degree of choline oxidase, which is reversibly inhibited by sulphur mustards, by measuring the enzymatic by-product H
2
O
2
in chronoamperometric mode. A nanocomposite constituted of Prussian Blue nanoparticles and Carbon Black was used as working electrode modifier to improve the electroanalytical performances. This bioassay was successfully applied for the measurement of a sulphur mustard, Yprite, obtaining a detection limit in the millimolar range (LOD = 0.9 mM). The developed sensor, combined with a portable and easy-to-use instrumentation, can be applied for a fast and cost-effective detection of sulphur mustards.</description><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Bioassays</subject><subject>Black carbon</subject><subject>Carbon black</subject><subject>Chemical sensors</subject><subject>Choline</subject><subject>Choline oxidase</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Electrochemistry</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Environmental Sciences</subject><subject>Environmental Sciences & Ecology</subject><subject>Hydrogen peroxide</subject><subject>Instrumentation</subject><subject>Life Sciences & Biomedicine</subject><subject>Mustard 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R</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2021-05-01</date><risdate>2021</risdate><volume>28</volume><issue>20</issue><spage>25069</spage><epage>25080</epage><pages>25069-25080</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Herein, we report a novel paper-based electrochemical sensor for on-site detection of sulphur mustards. This sensor was conceived combining office paper-based electrochemical sensor with choline oxidase enzyme to deliver a sustainable sensing tool. The mustard agent detection relies on the evaluation of inhibition degree of choline oxidase, which is reversibly inhibited by sulphur mustards, by measuring the enzymatic by-product H
2
O
2
in chronoamperometric mode. A nanocomposite constituted of Prussian Blue nanoparticles and Carbon Black was used as working electrode modifier to improve the electroanalytical performances. This bioassay was successfully applied for the measurement of a sulphur mustard, Yprite, obtaining a detection limit in the millimolar range (LOD = 0.9 mM). The developed sensor, combined with a portable and easy-to-use instrumentation, can be applied for a fast and cost-effective detection of sulphur mustards.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>29934830</pmid><doi>10.1007/s11356-018-2545-6</doi><tpages>12</tpages><orcidid>https://orcid.org/0000-0002-9028-3870</orcidid><orcidid>https://orcid.org/0000-0002-2073-5683</orcidid><orcidid>https://orcid.org/0000-0002-5497-6557</orcidid></addata></record> |
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| subjects | Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Bioassays Black carbon Carbon black Chemical sensors Choline Choline oxidase Earth and Environmental Science Ecotoxicology Electrochemistry Environment Environmental Chemistry Environmental Health Environmental science Environmental Sciences Environmental Sciences & Ecology Hydrogen peroxide Instrumentation Life Sciences & Biomedicine Mustard gas Nanocomposites Nanoparticles Onsite Oxidase Pigments Research Article Science & Technology Sensors Sulfur Waste Water Technology Water Management Water Pollution Control |
| title | Paper-based electrochemical sensor for on-site detection of the sulphur mustard |
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