Reactive co-sputter deposition of nanostructured cermet anodes for solid oxide fuel cells

The impact of a nanostructured NiO/yttria-stabilized zirconia (NiO/YSZ) and NiO/gadolinia-doped ceria (NiO/GDC) anode functional layers on low- and intermediate-temperature solid oxide fuel cell (SOFC) performance is investigated. NiO/YSZ and NiO/GDC thin films were reactively sputter-deposited by p...

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Veröffentlicht in:Japanese Journal of Applied Physics 2018-01, Vol.57 (1S), p.1
Hauptverfasser: Ionov, Igor V., Solovyev, Andrey A., Shipilova, Anna V., Lebedynskiy, Alexey M., Smolyanskiy, Egor A., Lauk, Alexander L., Semenov, Vyacheslav A.
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container_issue 1S
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container_title Japanese Journal of Applied Physics
container_volume 57
creator Ionov, Igor V.
Solovyev, Andrey A.
Shipilova, Anna V.
Lebedynskiy, Alexey M.
Smolyanskiy, Egor A.
Lauk, Alexander L.
Semenov, Vyacheslav A.
description The impact of a nanostructured NiO/yttria-stabilized zirconia (NiO/YSZ) and NiO/gadolinia-doped ceria (NiO/GDC) anode functional layers on low- and intermediate-temperature solid oxide fuel cell (SOFC) performance is investigated. NiO/YSZ and NiO/GDC thin films were reactively sputter-deposited by pulsed direct current magnetron sputtering from the Ni, Zr-Y, and Ce-Gd targets onto commercial NiO/YSZ substrates. Anode-supported SOFCs based on magnetron sputtered YSZ and GDC electrolytes (∼4 µm) with and without the nanostructured anode layers are fabricated. A direct comparison of the YSZ- and GDC-based SOFCs in temperature range of 600-800 and 400-600 °C is made. The performance of cells with the nanostructured anode layers significantly increases as compared to that of the cell without it, especially at lower temperatures. Increase of cells performance was achieved by reduction of the total area-specific resistance by 26-30%.
doi_str_mv 10.7567/JJAP.57.01AF07
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NiO/YSZ and NiO/GDC thin films were reactively sputter-deposited by pulsed direct current magnetron sputtering from the Ni, Zr-Y, and Ce-Gd targets onto commercial NiO/YSZ substrates. Anode-supported SOFCs based on magnetron sputtered YSZ and GDC electrolytes (∼4 µm) with and without the nanostructured anode layers are fabricated. A direct comparison of the YSZ- and GDC-based SOFCs in temperature range of 600-800 and 400-600 °C is made. The performance of cells with the nanostructured anode layers significantly increases as compared to that of the cell without it, especially at lower temperatures. 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subjects Anodes
Cerium gadolinium oxides
Cerium oxides
Cermets
Direct current
Electrolytic cells
Gadolinium
Gadolinium oxides
Magnetron sputtering
Nanostructure
Nickel oxides
Solid oxide fuel cells
Substrates
Thin films
Yttria-stabilized zirconia
Yttrium oxide
Zirconium dioxide
title Reactive co-sputter deposition of nanostructured cermet anodes for solid oxide fuel cells
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