Simultaneous production of biocrude oil and recovery of nutrients and metals from human feces via hydrothermal liquefaction
[Display omitted] •Fast degradation of human waste and energy recovery via hydrothermal liquefaction.•Biocrude, nutrients and metals in human waste are physically separated via HTL.•Max. liquefied fraction was 87.89%, and highest biocrude yield was 34.44%•HTL is promising for treatment from human wa...
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Veröffentlicht in: | Energy conversion and management 2017-02, Vol.134, p.340-346 |
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creator | Lu, Jianwen Zhang, Jiaren Zhu, Zhangbing Zhang, Yuanhui Zhao, Yu Li, Ruirui Watson, Jamison Li, Baoming Liu, Zhidan |
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•Fast degradation of human waste and energy recovery via hydrothermal liquefaction.•Biocrude, nutrients and metals in human waste are physically separated via HTL.•Max. liquefied fraction was 87.89%, and highest biocrude yield was 34.44%•HTL is promising for treatment from human wastes, and other wet biowastes.
Hydrothermal liquefaction (HTL) is a thermochemical process specifically suitable for treating wet wastes. This study investigated its potential for the production of biocrude oil and the recovery of nutrients and metals from human feces via HTL. Specifically, the effects of temperature (260°C, 300°C, 340°C), retention time (10min, 30min, 50min) and total solid (TS) content (5%, 15%, 25%) were studied. The maximum liquefied fraction was 87.89% and the highest biocrude yield reached 34.44% with a higher heating value of 40.29MJ/kg. Experimental results showed that 54% of carbon in the human feces was migrated to the biocrude oil while 72% of nitrogen was released to the aqueous phase. In addition, most of heavy and alkaline-earth metal elements in the human feces, including Ca (89%), Mg (81%), Al (88%), Fe (72%) and Zn (94%) were distributed in the solid residue, whereas K (89%) and Na (73%) were mainly dissolved into the aqueous phase. This study demonstrated that the efficient degradation of human waste via HTL without any pretreatment and its potential for the valorization in biocrude oil as well as separated nutrients and metals. |
doi_str_mv | 10.1016/j.enconman.2016.12.052 |
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•Fast degradation of human waste and energy recovery via hydrothermal liquefaction.•Biocrude, nutrients and metals in human waste are physically separated via HTL.•Max. liquefied fraction was 87.89%, and highest biocrude yield was 34.44%•HTL is promising for treatment from human wastes, and other wet biowastes.
Hydrothermal liquefaction (HTL) is a thermochemical process specifically suitable for treating wet wastes. This study investigated its potential for the production of biocrude oil and the recovery of nutrients and metals from human feces via HTL. Specifically, the effects of temperature (260°C, 300°C, 340°C), retention time (10min, 30min, 50min) and total solid (TS) content (5%, 15%, 25%) were studied. The maximum liquefied fraction was 87.89% and the highest biocrude yield reached 34.44% with a higher heating value of 40.29MJ/kg. Experimental results showed that 54% of carbon in the human feces was migrated to the biocrude oil while 72% of nitrogen was released to the aqueous phase. In addition, most of heavy and alkaline-earth metal elements in the human feces, including Ca (89%), Mg (81%), Al (88%), Fe (72%) and Zn (94%) were distributed in the solid residue, whereas K (89%) and Na (73%) were mainly dissolved into the aqueous phase. This study demonstrated that the efficient degradation of human waste via HTL without any pretreatment and its potential for the valorization in biocrude oil as well as separated nutrients and metals.</description><identifier>ISSN: 0196-8904</identifier><identifier>EISSN: 1879-2227</identifier><identifier>DOI: 10.1016/j.enconman.2016.12.052</identifier><language>eng</language><publisher>Oxford: Elsevier Ltd</publisher><subject>Alkaline earth metals ; Aluminum ; Biocrude oil ; Calcium ; Calorific value ; Carbon ; Feces ; Human feces ; Human wastes ; Hydrothermal liquefaction ; Iron ; Liquefaction ; Materials recovery ; Metal distribution ; Metals ; Nutrients ; Oil wastes ; Pretreatment ; Retention time ; Temperature effects ; Waste treatment ; Zinc</subject><ispartof>Energy conversion and management, 2017-02, Vol.134, p.340-346</ispartof><rights>2016 Elsevier Ltd</rights><rights>Copyright Elsevier Science Ltd. Feb 15, 2017</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c491t-7f42e71da089b4e2db50a7348487db1fb83855d29a8bb1633ba81daab6a6df4b3</citedby><cites>FETCH-LOGICAL-c491t-7f42e71da089b4e2db50a7348487db1fb83855d29a8bb1633ba81daab6a6df4b3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0196890416311475$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3537,27901,27902,65306</link.rule.ids></links><search><creatorcontrib>Lu, Jianwen</creatorcontrib><creatorcontrib>Zhang, Jiaren</creatorcontrib><creatorcontrib>Zhu, Zhangbing</creatorcontrib><creatorcontrib>Zhang, Yuanhui</creatorcontrib><creatorcontrib>Zhao, Yu</creatorcontrib><creatorcontrib>Li, Ruirui</creatorcontrib><creatorcontrib>Watson, Jamison</creatorcontrib><creatorcontrib>Li, Baoming</creatorcontrib><creatorcontrib>Liu, Zhidan</creatorcontrib><title>Simultaneous production of biocrude oil and recovery of nutrients and metals from human feces via hydrothermal liquefaction</title><title>Energy conversion and management</title><description>[Display omitted]
•Fast degradation of human waste and energy recovery via hydrothermal liquefaction.•Biocrude, nutrients and metals in human waste are physically separated via HTL.•Max. liquefied fraction was 87.89%, and highest biocrude yield was 34.44%•HTL is promising for treatment from human wastes, and other wet biowastes.
Hydrothermal liquefaction (HTL) is a thermochemical process specifically suitable for treating wet wastes. This study investigated its potential for the production of biocrude oil and the recovery of nutrients and metals from human feces via HTL. Specifically, the effects of temperature (260°C, 300°C, 340°C), retention time (10min, 30min, 50min) and total solid (TS) content (5%, 15%, 25%) were studied. The maximum liquefied fraction was 87.89% and the highest biocrude yield reached 34.44% with a higher heating value of 40.29MJ/kg. Experimental results showed that 54% of carbon in the human feces was migrated to the biocrude oil while 72% of nitrogen was released to the aqueous phase. In addition, most of heavy and alkaline-earth metal elements in the human feces, including Ca (89%), Mg (81%), Al (88%), Fe (72%) and Zn (94%) were distributed in the solid residue, whereas K (89%) and Na (73%) were mainly dissolved into the aqueous phase. This study demonstrated that the efficient degradation of human waste via HTL without any pretreatment and its potential for the valorization in biocrude oil as well as separated nutrients and metals.</description><subject>Alkaline earth metals</subject><subject>Aluminum</subject><subject>Biocrude oil</subject><subject>Calcium</subject><subject>Calorific value</subject><subject>Carbon</subject><subject>Feces</subject><subject>Human feces</subject><subject>Human wastes</subject><subject>Hydrothermal liquefaction</subject><subject>Iron</subject><subject>Liquefaction</subject><subject>Materials recovery</subject><subject>Metal distribution</subject><subject>Metals</subject><subject>Nutrients</subject><subject>Oil wastes</subject><subject>Pretreatment</subject><subject>Retention time</subject><subject>Temperature effects</subject><subject>Waste treatment</subject><subject>Zinc</subject><issn>0196-8904</issn><issn>1879-2227</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><recordid>eNqFkMtqGzEUhkVJoU7SVyiCrmciaW6aXYtpk4IhizZrocsRlpmRXEljMHn5aux0nZUQ57-c8yH0hZKaEto_HGrwOvhZ-pqVf01ZTTr2AW0oH8aKMTbcoA2hY1_xkbSf0G1KB0JI05F-g15_u3mZsvQQloSPMZhFZxc8DhYrF3RcDODgJiy9wRF0OEE8r0O_5OjA53SZzJDllLCNYcb7payCLWhI-OQk3p9NDHkPcZYTntzfBay8dNyjj7a44PPbe4defv74s32qds-Pv7bfd5VuR5qrwbYMBmok4aNqgRnVETk0LW_5YBS1ije86wwbJVeK9k2jJC9qqXrZG9uq5g59veaW80p7yuIQluhLpWCEtWsQbYqqv6p0DClFsOIY3SzjWVAiVtDiIP6DFitoQZkooIvx29UI5YaTgyiSLmQ0GFeAZWGCey_iH8_GjdA</recordid><startdate>20170215</startdate><enddate>20170215</enddate><creator>Lu, Jianwen</creator><creator>Zhang, Jiaren</creator><creator>Zhu, Zhangbing</creator><creator>Zhang, Yuanhui</creator><creator>Zhao, Yu</creator><creator>Li, Ruirui</creator><creator>Watson, Jamison</creator><creator>Li, Baoming</creator><creator>Liu, Zhidan</creator><general>Elsevier Ltd</general><general>Elsevier Science Ltd</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7ST</scope><scope>7TB</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>H8D</scope><scope>KR7</scope><scope>L7M</scope><scope>SOI</scope></search><sort><creationdate>20170215</creationdate><title>Simultaneous production of biocrude oil and recovery of nutrients and metals from human feces via hydrothermal liquefaction</title><author>Lu, Jianwen ; Zhang, Jiaren ; Zhu, Zhangbing ; Zhang, Yuanhui ; Zhao, Yu ; Li, Ruirui ; Watson, Jamison ; Li, Baoming ; Liu, Zhidan</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c491t-7f42e71da089b4e2db50a7348487db1fb83855d29a8bb1633ba81daab6a6df4b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><topic>Alkaline earth metals</topic><topic>Aluminum</topic><topic>Biocrude oil</topic><topic>Calcium</topic><topic>Calorific value</topic><topic>Carbon</topic><topic>Feces</topic><topic>Human feces</topic><topic>Human wastes</topic><topic>Hydrothermal liquefaction</topic><topic>Iron</topic><topic>Liquefaction</topic><topic>Materials recovery</topic><topic>Metal distribution</topic><topic>Metals</topic><topic>Nutrients</topic><topic>Oil wastes</topic><topic>Pretreatment</topic><topic>Retention time</topic><topic>Temperature effects</topic><topic>Waste treatment</topic><topic>Zinc</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Lu, Jianwen</creatorcontrib><creatorcontrib>Zhang, Jiaren</creatorcontrib><creatorcontrib>Zhu, Zhangbing</creatorcontrib><creatorcontrib>Zhang, Yuanhui</creatorcontrib><creatorcontrib>Zhao, Yu</creatorcontrib><creatorcontrib>Li, Ruirui</creatorcontrib><creatorcontrib>Watson, Jamison</creatorcontrib><creatorcontrib>Li, Baoming</creatorcontrib><creatorcontrib>Liu, Zhidan</creatorcontrib><collection>CrossRef</collection><collection>Environment Abstracts</collection><collection>Mechanical & Transportation Engineering Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Aerospace Database</collection><collection>Civil Engineering Abstracts</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Environment Abstracts</collection><jtitle>Energy conversion and management</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lu, Jianwen</au><au>Zhang, Jiaren</au><au>Zhu, Zhangbing</au><au>Zhang, Yuanhui</au><au>Zhao, Yu</au><au>Li, Ruirui</au><au>Watson, Jamison</au><au>Li, Baoming</au><au>Liu, Zhidan</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Simultaneous production of biocrude oil and recovery of nutrients and metals from human feces via hydrothermal liquefaction</atitle><jtitle>Energy conversion and management</jtitle><date>2017-02-15</date><risdate>2017</risdate><volume>134</volume><spage>340</spage><epage>346</epage><pages>340-346</pages><issn>0196-8904</issn><eissn>1879-2227</eissn><abstract>[Display omitted]
•Fast degradation of human waste and energy recovery via hydrothermal liquefaction.•Biocrude, nutrients and metals in human waste are physically separated via HTL.•Max. liquefied fraction was 87.89%, and highest biocrude yield was 34.44%•HTL is promising for treatment from human wastes, and other wet biowastes.
Hydrothermal liquefaction (HTL) is a thermochemical process specifically suitable for treating wet wastes. This study investigated its potential for the production of biocrude oil and the recovery of nutrients and metals from human feces via HTL. Specifically, the effects of temperature (260°C, 300°C, 340°C), retention time (10min, 30min, 50min) and total solid (TS) content (5%, 15%, 25%) were studied. The maximum liquefied fraction was 87.89% and the highest biocrude yield reached 34.44% with a higher heating value of 40.29MJ/kg. Experimental results showed that 54% of carbon in the human feces was migrated to the biocrude oil while 72% of nitrogen was released to the aqueous phase. In addition, most of heavy and alkaline-earth metal elements in the human feces, including Ca (89%), Mg (81%), Al (88%), Fe (72%) and Zn (94%) were distributed in the solid residue, whereas K (89%) and Na (73%) were mainly dissolved into the aqueous phase. This study demonstrated that the efficient degradation of human waste via HTL without any pretreatment and its potential for the valorization in biocrude oil as well as separated nutrients and metals.</abstract><cop>Oxford</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.enconman.2016.12.052</doi><tpages>7</tpages><oa>free_for_read</oa></addata></record> |
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subjects | Alkaline earth metals Aluminum Biocrude oil Calcium Calorific value Carbon Feces Human feces Human wastes Hydrothermal liquefaction Iron Liquefaction Materials recovery Metal distribution Metals Nutrients Oil wastes Pretreatment Retention time Temperature effects Waste treatment Zinc |
title | Simultaneous production of biocrude oil and recovery of nutrients and metals from human feces via hydrothermal liquefaction |
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