Kinetic, Equilibrium, and Thermodynamic Analyses of Ni(II) Biosorption from Aqueous Solution by Acorn Shell of Quercus crassipes
Exposure to divalent nickel [Ni(II)] poses a significant risk to human health. The present study was conducted to evaluate the biosorption capacity of acorn shell of Quercus crassipes Humb. & Bonpl. (QCS) for removal of Ni(II) ions from aqueous solutions in terms of kinetics, equilibrium, and th...
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| description | Exposure to divalent nickel [Ni(II)] poses a significant risk to human health. The present study was conducted to evaluate the biosorption capacity of acorn shell of
Quercus crassipes
Humb. & Bonpl. (QCS) for removal of Ni(II) ions from aqueous solutions in terms of kinetics, equilibrium, and thermodynamics. Batch biosorption studies showed that the Ni(II) biosorption behavior of QCS is strongly dependent on solution pH, shaking contact time, initial Ni(II) concentration, and temperature. Specifically, Ni(II) biosorption was found to increase with increasing solution pH, contact time, initial Ni(II) concentration, and temperature. Modeling of the Ni(II) biosorption kinetic and equilibrium data showed that the best agreement of experimental data was achieved with the pseudo-second-order kinetics model and the Freundlich isotherm model, respectively. The calculated thermodynamic parameters indicated that the Ni(II) biosorption process was endothermic, non-spontaneous, and chemical in nature. Fourier-transform infrared (FTIR) spectroscopy analysis showed that acidic functional groups, namely hydroxyl, carbonyl, and carboxyl functional groups, present on the QCS surface are likely to be involved in the biosorption of Ni(II) ions. The performance of QCS was compared with those of other reported biosorbents in terms of the efficiency of Ni(II) removal from aqueous solutions, revealing that QCS is highly effective in terms of its biosorption capacity. These findings indicate that QCS can be used as a low-cost, highly effective, and environmentally friendly alternative biosorbent for the detoxification of Ni(II)-contaminated water and wastewater. |
| doi_str_mv | 10.1007/s11270-018-3775-4 |
| format | Article |
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Quercus crassipes
Humb. & Bonpl. (QCS) for removal of Ni(II) ions from aqueous solutions in terms of kinetics, equilibrium, and thermodynamics. Batch biosorption studies showed that the Ni(II) biosorption behavior of QCS is strongly dependent on solution pH, shaking contact time, initial Ni(II) concentration, and temperature. Specifically, Ni(II) biosorption was found to increase with increasing solution pH, contact time, initial Ni(II) concentration, and temperature. Modeling of the Ni(II) biosorption kinetic and equilibrium data showed that the best agreement of experimental data was achieved with the pseudo-second-order kinetics model and the Freundlich isotherm model, respectively. The calculated thermodynamic parameters indicated that the Ni(II) biosorption process was endothermic, non-spontaneous, and chemical in nature. Fourier-transform infrared (FTIR) spectroscopy analysis showed that acidic functional groups, namely hydroxyl, carbonyl, and carboxyl functional groups, present on the QCS surface are likely to be involved in the biosorption of Ni(II) ions. The performance of QCS was compared with those of other reported biosorbents in terms of the efficiency of Ni(II) removal from aqueous solutions, revealing that QCS is highly effective in terms of its biosorption capacity. These findings indicate that QCS can be used as a low-cost, highly effective, and environmentally friendly alternative biosorbent for the detoxification of Ni(II)-contaminated water and wastewater.</description><identifier>ISSN: 0049-6979</identifier><identifier>EISSN: 1573-2932</identifier><identifier>DOI: 10.1007/s11270-018-3775-4</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Analytical methods ; Aqueous solutions ; Atmospheric Protection/Air Quality Control/Air Pollution ; Biosorption ; Capacity ; Carbonyl compounds ; Carbonyls ; Climate Change/Climate Change Impacts ; Detoxification ; Earth and Environmental Science ; Endothermic reactions ; Environment ; Environmental monitoring ; Equilibrium ; Fourier transforms ; Functional groups ; Health aspects ; Hydrogeology ; Infrared analysis ; Ions ; Kinetics ; Mathematical models ; Modelling ; Nickel ; pH effects ; Quercus ; Removal ; Shaking ; Soil Science & Conservation ; Solutions ; Temperature ; Thermodynamics ; Wastewater ; Water pollution ; Water Quality/Water Pollution</subject><ispartof>Water, air, and soil pollution, 2018-04, Vol.229 (4), p.1-17, Article 119</ispartof><rights>Springer International Publishing AG, part of Springer Nature 2018</rights><rights>COPYRIGHT 2018 Springer</rights><rights>Water, Air, & Soil Pollution is a copyright of Springer, (2018). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c355t-7280221c487f11604f3648b3689f9fb3d1e38ab8d8799fc1bd704d355eee21c73</citedby><cites>FETCH-LOGICAL-c355t-7280221c487f11604f3648b3689f9fb3d1e38ab8d8799fc1bd704d355eee21c73</cites><orcidid>0000-0002-8470-0711</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11270-018-3775-4$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11270-018-3775-4$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Aranda-García, E.</creatorcontrib><creatorcontrib>Cristiani-Urbina, E.</creatorcontrib><title>Kinetic, Equilibrium, and Thermodynamic Analyses of Ni(II) Biosorption from Aqueous Solution by Acorn Shell of Quercus crassipes</title><title>Water, air, and soil pollution</title><addtitle>Water Air Soil Pollut</addtitle><description>Exposure to divalent nickel [Ni(II)] poses a significant risk to human health. The present study was conducted to evaluate the biosorption capacity of acorn shell of
Quercus crassipes
Humb. & Bonpl. (QCS) for removal of Ni(II) ions from aqueous solutions in terms of kinetics, equilibrium, and thermodynamics. Batch biosorption studies showed that the Ni(II) biosorption behavior of QCS is strongly dependent on solution pH, shaking contact time, initial Ni(II) concentration, and temperature. Specifically, Ni(II) biosorption was found to increase with increasing solution pH, contact time, initial Ni(II) concentration, and temperature. Modeling of the Ni(II) biosorption kinetic and equilibrium data showed that the best agreement of experimental data was achieved with the pseudo-second-order kinetics model and the Freundlich isotherm model, respectively. The calculated thermodynamic parameters indicated that the Ni(II) biosorption process was endothermic, non-spontaneous, and chemical in nature. Fourier-transform infrared (FTIR) spectroscopy analysis showed that acidic functional groups, namely hydroxyl, carbonyl, and carboxyl functional groups, present on the QCS surface are likely to be involved in the biosorption of Ni(II) ions. The performance of QCS was compared with those of other reported biosorbents in terms of the efficiency of Ni(II) removal from aqueous solutions, revealing that QCS is highly effective in terms of its biosorption capacity. These findings indicate that QCS can be used as a low-cost, highly effective, and environmentally friendly alternative biosorbent for the detoxification of Ni(II)-contaminated water and wastewater.</description><subject>Analytical methods</subject><subject>Aqueous solutions</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Biosorption</subject><subject>Capacity</subject><subject>Carbonyl compounds</subject><subject>Carbonyls</subject><subject>Climate Change/Climate Change Impacts</subject><subject>Detoxification</subject><subject>Earth and Environmental Science</subject><subject>Endothermic reactions</subject><subject>Environment</subject><subject>Environmental monitoring</subject><subject>Equilibrium</subject><subject>Fourier transforms</subject><subject>Functional groups</subject><subject>Health aspects</subject><subject>Hydrogeology</subject><subject>Infrared analysis</subject><subject>Ions</subject><subject>Kinetics</subject><subject>Mathematical models</subject><subject>Modelling</subject><subject>Nickel</subject><subject>pH effects</subject><subject>Quercus</subject><subject>Removal</subject><subject>Shaking</subject><subject>Soil Science & Conservation</subject><subject>Solutions</subject><subject>Temperature</subject><subject>Thermodynamics</subject><subject>Wastewater</subject><subject>Water pollution</subject><subject>Water Quality/Water 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of Quercus crassipes</atitle><jtitle>Water, air, and soil pollution</jtitle><stitle>Water Air Soil Pollut</stitle><date>2018-04-01</date><risdate>2018</risdate><volume>229</volume><issue>4</issue><spage>1</spage><epage>17</epage><pages>1-17</pages><artnum>119</artnum><issn>0049-6979</issn><eissn>1573-2932</eissn><abstract>Exposure to divalent nickel [Ni(II)] poses a significant risk to human health. The present study was conducted to evaluate the biosorption capacity of acorn shell of
Quercus crassipes
Humb. & Bonpl. (QCS) for removal of Ni(II) ions from aqueous solutions in terms of kinetics, equilibrium, and thermodynamics. Batch biosorption studies showed that the Ni(II) biosorption behavior of QCS is strongly dependent on solution pH, shaking contact time, initial Ni(II) concentration, and temperature. Specifically, Ni(II) biosorption was found to increase with increasing solution pH, contact time, initial Ni(II) concentration, and temperature. Modeling of the Ni(II) biosorption kinetic and equilibrium data showed that the best agreement of experimental data was achieved with the pseudo-second-order kinetics model and the Freundlich isotherm model, respectively. The calculated thermodynamic parameters indicated that the Ni(II) biosorption process was endothermic, non-spontaneous, and chemical in nature. Fourier-transform infrared (FTIR) spectroscopy analysis showed that acidic functional groups, namely hydroxyl, carbonyl, and carboxyl functional groups, present on the QCS surface are likely to be involved in the biosorption of Ni(II) ions. The performance of QCS was compared with those of other reported biosorbents in terms of the efficiency of Ni(II) removal from aqueous solutions, revealing that QCS is highly effective in terms of its biosorption capacity. These findings indicate that QCS can be used as a low-cost, highly effective, and environmentally friendly alternative biosorbent for the detoxification of Ni(II)-contaminated water and wastewater.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s11270-018-3775-4</doi><tpages>17</tpages><orcidid>https://orcid.org/0000-0002-8470-0711</orcidid></addata></record> |
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| ispartof | Water, air, and soil pollution, 2018-04, Vol.229 (4), p.1-17, Article 119 |
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| subjects | Analytical methods Aqueous solutions Atmospheric Protection/Air Quality Control/Air Pollution Biosorption Capacity Carbonyl compounds Carbonyls Climate Change/Climate Change Impacts Detoxification Earth and Environmental Science Endothermic reactions Environment Environmental monitoring Equilibrium Fourier transforms Functional groups Health aspects Hydrogeology Infrared analysis Ions Kinetics Mathematical models Modelling Nickel pH effects Quercus Removal Shaking Soil Science & Conservation Solutions Temperature Thermodynamics Wastewater Water pollution Water Quality/Water Pollution |
| title | Kinetic, Equilibrium, and Thermodynamic Analyses of Ni(II) Biosorption from Aqueous Solution by Acorn Shell of Quercus crassipes |
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