Magnetic graphene for microwave absorbing application: Towards the lightest graphene-based absorber
Application of graphene derived nanomaterial in microwave absorption has been limited by the issue of excessively high dielectric loss. To address this issue, instead of resorting to burdensome compositing with metal and ceramic particles, we put forward the idea of approaching impedance match by tr...
Gespeichert in:
| Veröffentlicht in: | Carbon (New York) 2017-12, Vol.125, p.630-639 |
|---|---|
| Hauptverfasser: | , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 639 |
|---|---|
| container_issue | |
| container_start_page | 630 |
| container_title | Carbon (New York) |
| container_volume | 125 |
| creator | Quan, L. Qin, F.X. Estevez, D. Wang, H. Peng, H.X. |
| description | Application of graphene derived nanomaterial in microwave absorption has been limited by the issue of excessively high dielectric loss. To address this issue, instead of resorting to burdensome compositing with metal and ceramic particles, we put forward the idea of approaching impedance match by transforming graphene from diamagnetic to ferromagnetic and meanwhile suppress the conductivity. In this study, we synthesized the Nitrogen-doped graphene (NG) by a facile hydrothermal method with graphene oxide (GO) and urea as precursors. In comparison with GO and reduced GO (rGO), the nitrogen doping along with reduction process boosted the magnetism via a Ruderman-Kittel-Kasuya-Yosida (RKKY) mechanism. Pyrrolic-N has been found to dominate the magnetic property induced, which cooperates with the suppression of conductivity to benefit the absorption performance. The reflection loss of nitrogen doped graphene can achieve −11.3 dB absorption maximum at 12.7 GHz and an absorption bandwidth of 12.2–14.3 GHz (reflection loss |
| doi_str_mv | 10.1016/j.carbon.2017.09.101 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_1970948028</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><els_id>S0008622317309843</els_id><sourcerecordid>1970948028</sourcerecordid><originalsourceid>FETCH-LOGICAL-c400t-9ba911523924bcb7ee6c8256b1dc95a2bcbf6f5872da458ab9764ffef37f8d8e3</originalsourceid><addsrcrecordid>eNp9UMtOwzAQtBBIlMIfcIjEOcF2XjYHJFTxkoq4lLNlO-vUURsHOy3i73EUxJHTamd3ZncGoWuCM4JJddtlWnrl-oxiUmeYT-gJWhBW52nOODlFC4wxSytK83N0EUIX24KRYoH0m2x7GK1OWi-HLfSQGOeTvdXefckjJFIF55Xt20QOw85qOVrX3yWbOPVNSMYtJDvbbkcI459EqmSA5pcK_hKdGbkLcPVbl-jj6XGzeknX78-vq4d1qguMx5QryQkpac5pobSqASrNaFkp0mheShoxU5mS1bSRRcmk4nVVGAMmrw1rGORLdDPrDt59HuJDonMH38eTgvAa84JhyuJWMW9FhyF4MGLwdi_9tyBYTHGKTsxxiilOgfmERtr9TIPo4GjBi6At9Boa60GPonH2f4EfGDaCFA</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1970948028</pqid></control><display><type>article</type><title>Magnetic graphene for microwave absorbing application: Towards the lightest graphene-based absorber</title><source>ScienceDirect Journals (5 years ago - present)</source><creator>Quan, L. ; Qin, F.X. ; Estevez, D. ; Wang, H. ; Peng, H.X.</creator><creatorcontrib>Quan, L. ; Qin, F.X. ; Estevez, D. ; Wang, H. ; Peng, H.X.</creatorcontrib><description>Application of graphene derived nanomaterial in microwave absorption has been limited by the issue of excessively high dielectric loss. To address this issue, instead of resorting to burdensome compositing with metal and ceramic particles, we put forward the idea of approaching impedance match by transforming graphene from diamagnetic to ferromagnetic and meanwhile suppress the conductivity. In this study, we synthesized the Nitrogen-doped graphene (NG) by a facile hydrothermal method with graphene oxide (GO) and urea as precursors. In comparison with GO and reduced GO (rGO), the nitrogen doping along with reduction process boosted the magnetism via a Ruderman-Kittel-Kasuya-Yosida (RKKY) mechanism. Pyrrolic-N has been found to dominate the magnetic property induced, which cooperates with the suppression of conductivity to benefit the absorption performance. The reflection loss of nitrogen doped graphene can achieve −11.3 dB absorption maximum at 12.7 GHz and an absorption bandwidth of 12.2–14.3 GHz (reflection loss < −10 dB) at a thickness of 3 mm, which proves to be favourable with respective to the density as compared to existing graphene-based absorbers.
[Display omitted]</description><identifier>ISSN: 0008-6223</identifier><identifier>EISSN: 1873-3891</identifier><identifier>DOI: 10.1016/j.carbon.2017.09.101</identifier><language>eng</language><publisher>New York: Elsevier Ltd</publisher><subject>Absorbers ; Conductivity ; Diamagnetism ; Dielectric loss ; Dielectrics ; Ferromagnetism ; Graphene ; Magnetic properties ; Magnetism ; Microwave absorption ; Nanomaterials ; Nitrogen ; Reflection</subject><ispartof>Carbon (New York), 2017-12, Vol.125, p.630-639</ispartof><rights>2017 Elsevier Ltd</rights><rights>Copyright Elsevier BV Dec 2017</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c400t-9ba911523924bcb7ee6c8256b1dc95a2bcbf6f5872da458ab9764ffef37f8d8e3</citedby><cites>FETCH-LOGICAL-c400t-9ba911523924bcb7ee6c8256b1dc95a2bcbf6f5872da458ab9764ffef37f8d8e3</cites><orcidid>0000-0002-7971-764X</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.carbon.2017.09.101$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3548,27923,27924,45994</link.rule.ids></links><search><creatorcontrib>Quan, L.</creatorcontrib><creatorcontrib>Qin, F.X.</creatorcontrib><creatorcontrib>Estevez, D.</creatorcontrib><creatorcontrib>Wang, H.</creatorcontrib><creatorcontrib>Peng, H.X.</creatorcontrib><title>Magnetic graphene for microwave absorbing application: Towards the lightest graphene-based absorber</title><title>Carbon (New York)</title><description>Application of graphene derived nanomaterial in microwave absorption has been limited by the issue of excessively high dielectric loss. To address this issue, instead of resorting to burdensome compositing with metal and ceramic particles, we put forward the idea of approaching impedance match by transforming graphene from diamagnetic to ferromagnetic and meanwhile suppress the conductivity. In this study, we synthesized the Nitrogen-doped graphene (NG) by a facile hydrothermal method with graphene oxide (GO) and urea as precursors. In comparison with GO and reduced GO (rGO), the nitrogen doping along with reduction process boosted the magnetism via a Ruderman-Kittel-Kasuya-Yosida (RKKY) mechanism. Pyrrolic-N has been found to dominate the magnetic property induced, which cooperates with the suppression of conductivity to benefit the absorption performance. The reflection loss of nitrogen doped graphene can achieve −11.3 dB absorption maximum at 12.7 GHz and an absorption bandwidth of 12.2–14.3 GHz (reflection loss < −10 dB) at a thickness of 3 mm, which proves to be favourable with respective to the density as compared to existing graphene-based absorbers.
[Display omitted]</description><subject>Absorbers</subject><subject>Conductivity</subject><subject>Diamagnetism</subject><subject>Dielectric loss</subject><subject>Dielectrics</subject><subject>Ferromagnetism</subject><subject>Graphene</subject><subject>Magnetic properties</subject><subject>Magnetism</subject><subject>Microwave absorption</subject><subject>Nanomaterials</subject><subject>Nitrogen</subject><subject>Reflection</subject><issn>0008-6223</issn><issn>1873-3891</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><recordid>eNp9UMtOwzAQtBBIlMIfcIjEOcF2XjYHJFTxkoq4lLNlO-vUURsHOy3i73EUxJHTamd3ZncGoWuCM4JJddtlWnrl-oxiUmeYT-gJWhBW52nOODlFC4wxSytK83N0EUIX24KRYoH0m2x7GK1OWi-HLfSQGOeTvdXefckjJFIF55Xt20QOw85qOVrX3yWbOPVNSMYtJDvbbkcI459EqmSA5pcK_hKdGbkLcPVbl-jj6XGzeknX78-vq4d1qguMx5QryQkpac5pobSqASrNaFkp0mheShoxU5mS1bSRRcmk4nVVGAMmrw1rGORLdDPrDt59HuJDonMH38eTgvAa84JhyuJWMW9FhyF4MGLwdi_9tyBYTHGKTsxxiilOgfmERtr9TIPo4GjBi6At9Boa60GPonH2f4EfGDaCFA</recordid><startdate>201712</startdate><enddate>201712</enddate><creator>Quan, L.</creator><creator>Qin, F.X.</creator><creator>Estevez, D.</creator><creator>Wang, H.</creator><creator>Peng, H.X.</creator><general>Elsevier Ltd</general><general>Elsevier BV</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8FD</scope><scope>JG9</scope><orcidid>https://orcid.org/0000-0002-7971-764X</orcidid></search><sort><creationdate>201712</creationdate><title>Magnetic graphene for microwave absorbing application: Towards the lightest graphene-based absorber</title><author>Quan, L. ; Qin, F.X. ; Estevez, D. ; Wang, H. ; Peng, H.X.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c400t-9ba911523924bcb7ee6c8256b1dc95a2bcbf6f5872da458ab9764ffef37f8d8e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><topic>Absorbers</topic><topic>Conductivity</topic><topic>Diamagnetism</topic><topic>Dielectric loss</topic><topic>Dielectrics</topic><topic>Ferromagnetism</topic><topic>Graphene</topic><topic>Magnetic properties</topic><topic>Magnetism</topic><topic>Microwave absorption</topic><topic>Nanomaterials</topic><topic>Nitrogen</topic><topic>Reflection</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Quan, L.</creatorcontrib><creatorcontrib>Qin, F.X.</creatorcontrib><creatorcontrib>Estevez, D.</creatorcontrib><creatorcontrib>Wang, H.</creatorcontrib><creatorcontrib>Peng, H.X.</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><jtitle>Carbon (New York)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Quan, L.</au><au>Qin, F.X.</au><au>Estevez, D.</au><au>Wang, H.</au><au>Peng, H.X.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Magnetic graphene for microwave absorbing application: Towards the lightest graphene-based absorber</atitle><jtitle>Carbon (New York)</jtitle><date>2017-12</date><risdate>2017</risdate><volume>125</volume><spage>630</spage><epage>639</epage><pages>630-639</pages><issn>0008-6223</issn><eissn>1873-3891</eissn><abstract>Application of graphene derived nanomaterial in microwave absorption has been limited by the issue of excessively high dielectric loss. To address this issue, instead of resorting to burdensome compositing with metal and ceramic particles, we put forward the idea of approaching impedance match by transforming graphene from diamagnetic to ferromagnetic and meanwhile suppress the conductivity. In this study, we synthesized the Nitrogen-doped graphene (NG) by a facile hydrothermal method with graphene oxide (GO) and urea as precursors. In comparison with GO and reduced GO (rGO), the nitrogen doping along with reduction process boosted the magnetism via a Ruderman-Kittel-Kasuya-Yosida (RKKY) mechanism. Pyrrolic-N has been found to dominate the magnetic property induced, which cooperates with the suppression of conductivity to benefit the absorption performance. The reflection loss of nitrogen doped graphene can achieve −11.3 dB absorption maximum at 12.7 GHz and an absorption bandwidth of 12.2–14.3 GHz (reflection loss < −10 dB) at a thickness of 3 mm, which proves to be favourable with respective to the density as compared to existing graphene-based absorbers.
[Display omitted]</abstract><cop>New York</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.carbon.2017.09.101</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0002-7971-764X</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0008-6223 |
| ispartof | Carbon (New York), 2017-12, Vol.125, p.630-639 |
| issn | 0008-6223 1873-3891 |
| language | eng |
| recordid | cdi_proquest_journals_1970948028 |
| source | ScienceDirect Journals (5 years ago - present) |
| subjects | Absorbers Conductivity Diamagnetism Dielectric loss Dielectrics Ferromagnetism Graphene Magnetic properties Magnetism Microwave absorption Nanomaterials Nitrogen Reflection |
| title | Magnetic graphene for microwave absorbing application: Towards the lightest graphene-based absorber |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-11T11%3A38%3A32IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Magnetic%20graphene%20for%20microwave%20absorbing%20application:%20Towards%20the%20lightest%20graphene-based%20absorber&rft.jtitle=Carbon%20(New%20York)&rft.au=Quan,%20L.&rft.date=2017-12&rft.volume=125&rft.spage=630&rft.epage=639&rft.pages=630-639&rft.issn=0008-6223&rft.eissn=1873-3891&rft_id=info:doi/10.1016/j.carbon.2017.09.101&rft_dat=%3Cproquest_cross%3E1970948028%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1970948028&rft_id=info:pmid/&rft_els_id=S0008622317309843&rfr_iscdi=true |