Study of atmospheric CO2 and CH4 at Longfengshan WMO/GAW regional station: The variations, trends, influence of local sources/sinks, and transport

Atmospheric CO2 and CH4 have been continuously measured since 2009 at Longfengshan WMO/GAW station(LFS) in China. Variations of the mole fractions, influence of long-distance transport, effects of local sources/sinks and the characteristics of synoptic scale variations have been studied based on the...

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Veröffentlicht in:Science China. Earth sciences 2017-10, Vol.60 (10), p.1886-1895
Hauptverfasser: Fang, ShuangXi, Tans, Pieter P., Yao, Bo, Luan, Tian, Wu, YanLing, Yu, DaJiang
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container_issue 10
container_start_page 1886
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creator Fang, ShuangXi
Tans, Pieter P.
Yao, Bo
Luan, Tian
Wu, YanLing
Yu, DaJiang
description Atmospheric CO2 and CH4 have been continuously measured since 2009 at Longfengshan WMO/GAW station(LFS) in China. Variations of the mole fractions, influence of long-distance transport, effects of local sources/sinks and the characteristics of synoptic scale variations have been studied based on the records from 2009 to 2013. Both the CO2 and CH4 mole fractions display increasing trends in the last five years, with growth rates of 3.1±0.02 ppm yr^-1 for CO2 and 8±0.04 ppb yr^-1(standard error, 1-σ)for CH4. In summer, the regional CO2 mole fractions are apparently lower than the Marine Boundary Layer reference, with the lowest value of.13.6±0.7 ppm in July, while the CH4 values are higher than the MBL reference, with the maximum of 139±6 ppb.From 9 to 17(Local time, LT) in summer, the atmospheric CO2 mole fractions at 10 m a.g.l. are always lower than at 80 m, with a mean difference of.1.1±0.2 ppm, indicating that the flask sampling approach deployed may underestimate the background mole fractions in summer. In winter, anthropogenic emissions dominate the regional CO2 and CH4 mole fractions. Cluster analysis of backward trajectories shows that atmospheric CO2 and CH4 at LFS are influenced by anthropogenic emissions from the southwest(Changchun and Jilin city) all year. The synoptic scale variations indicate that the northeastern China plain acts as an important source of atmospheric CO2 and CH4 in winter.
doi_str_mv 10.1007/s11430-016-9066-3
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Variations of the mole fractions, influence of long-distance transport, effects of local sources/sinks and the characteristics of synoptic scale variations have been studied based on the records from 2009 to 2013. Both the CO2 and CH4 mole fractions display increasing trends in the last five years, with growth rates of 3.1±0.02 ppm yr^-1 for CO2 and 8±0.04 ppb yr^-1(standard error, 1-σ)for CH4. In summer, the regional CO2 mole fractions are apparently lower than the Marine Boundary Layer reference, with the lowest value of.13.6±0.7 ppm in July, while the CH4 values are higher than the MBL reference, with the maximum of 139±6 ppb.From 9 to 17(Local time, LT) in summer, the atmospheric CO2 mole fractions at 10 m a.g.l. are always lower than at 80 m, with a mean difference of.1.1±0.2 ppm, indicating that the flask sampling approach deployed may underestimate the background mole fractions in summer. In winter, anthropogenic emissions dominate the regional CO2 and CH4 mole fractions. Cluster analysis of backward trajectories shows that atmospheric CO2 and CH4 at LFS are influenced by anthropogenic emissions from the southwest(Changchun and Jilin city) all year. The synoptic scale variations indicate that the northeastern China plain acts as an important source of atmospheric CO2 and CH4 in winter.</description><identifier>ISSN: 1674-7313</identifier><identifier>EISSN: 1869-1897</identifier><identifier>DOI: 10.1007/s11430-016-9066-3</identifier><language>eng</language><publisher>Beijing: Science China Press</publisher><subject>Anthropogenic factors ; Atmosphere ; Boundary layers ; Carbon dioxide ; Carbon dioxide atmospheric concentrations ; CH4 ; Cluster analysis ; Earth and Environmental Science ; Earth Sciences ; Emissions ; Growth rate ; Human influences ; Methane ; Regional analysis ; Regions ; Research Paper ; Sinkholes ; Standard error ; Summer ; Temperature ; Trajectory analysis ; Transport ; Transportation ; Trends ; Variation ; Winter ; WMO ; 区域站 ; 大气CO2 ; 天气尺度 ; 摩尔分数 ; 水沟 ; 运输</subject><ispartof>Science China. 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Earth sciences</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Fang, ShuangXi</au><au>Tans, Pieter P.</au><au>Yao, Bo</au><au>Luan, Tian</au><au>Wu, YanLing</au><au>Yu, DaJiang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Study of atmospheric CO2 and CH4 at Longfengshan WMO/GAW regional station: The variations, trends, influence of local sources/sinks, and transport</atitle><jtitle>Science China. Earth sciences</jtitle><stitle>Sci. China Earth Sci</stitle><addtitle>SCIENCE CHINA Earth Sciences</addtitle><date>2017-10-01</date><risdate>2017</risdate><volume>60</volume><issue>10</issue><spage>1886</spage><epage>1895</epage><pages>1886-1895</pages><issn>1674-7313</issn><eissn>1869-1897</eissn><abstract>Atmospheric CO2 and CH4 have been continuously measured since 2009 at Longfengshan WMO/GAW station(LFS) in China. Variations of the mole fractions, influence of long-distance transport, effects of local sources/sinks and the characteristics of synoptic scale variations have been studied based on the records from 2009 to 2013. Both the CO2 and CH4 mole fractions display increasing trends in the last five years, with growth rates of 3.1±0.02 ppm yr^-1 for CO2 and 8±0.04 ppb yr^-1(standard error, 1-σ)for CH4. In summer, the regional CO2 mole fractions are apparently lower than the Marine Boundary Layer reference, with the lowest value of.13.6±0.7 ppm in July, while the CH4 values are higher than the MBL reference, with the maximum of 139±6 ppb.From 9 to 17(Local time, LT) in summer, the atmospheric CO2 mole fractions at 10 m a.g.l. are always lower than at 80 m, with a mean difference of.1.1±0.2 ppm, indicating that the flask sampling approach deployed may underestimate the background mole fractions in summer. In winter, anthropogenic emissions dominate the regional CO2 and CH4 mole fractions. Cluster analysis of backward trajectories shows that atmospheric CO2 and CH4 at LFS are influenced by anthropogenic emissions from the southwest(Changchun and Jilin city) all year. The synoptic scale variations indicate that the northeastern China plain acts as an important source of atmospheric CO2 and CH4 in winter.</abstract><cop>Beijing</cop><pub>Science China Press</pub><doi>10.1007/s11430-016-9066-3</doi><tpages>10</tpages></addata></record>
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source SpringerLink Journals; Alma/SFX Local Collection
subjects Anthropogenic factors
Atmosphere
Boundary layers
Carbon dioxide
Carbon dioxide atmospheric concentrations
CH4
Cluster analysis
Earth and Environmental Science
Earth Sciences
Emissions
Growth rate
Human influences
Methane
Regional analysis
Regions
Research Paper
Sinkholes
Standard error
Summer
Temperature
Trajectory analysis
Transport
Transportation
Trends
Variation
Winter
WMO
区域站
大气CO2
天气尺度
摩尔分数
水沟
运输
title Study of atmospheric CO2 and CH4 at Longfengshan WMO/GAW regional station: The variations, trends, influence of local sources/sinks, and transport
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