Determination of Heavy Metals in a Highly Porous Sorptive Filter Material of Road Runoff Treatment Systems with LA-ICP-MS
To remove heavy metal contaminations from road runoff prior to discharge into surface water or groundwater, highly porous sorptive filter materials are used. One effective material is a technical product based on granular ferric hydroxide. To specify the removal mechanisms, lab-scale column experime...
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| description | To remove heavy metal contaminations from road runoff prior to discharge into surface water or groundwater, highly porous sorptive filter materials are used. One effective material is a technical product based on granular ferric hydroxide. To specify the removal mechanisms, lab-scale column experiments were performed preloading the material with Cd, Cu, Ni, Pb, and Zn. To identify removal mechanisms and the distribution of heavy metals in the material, investigations with scanning electron microscope (SEM)/energy-dispersive X-ray spectroscopy (EDX) and laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS) were performed. With SEM/EDX, only Pb was detectable; all other heavy metals were not represented on the surface of the particles. To determine the intrusion of the metals, LA-ICP-MS was used. Thereby, the high porosity necessitated a special data evaluation that enabled the determination of the heavy metal removal and the leaching of other elements from the filter material as a function of depth. The measured depth profiles varied for each element and correlated with the metal mobility. |
| doi_str_mv | 10.1007/s11270-017-3515-1 |
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One effective material is a technical product based on granular ferric hydroxide. To specify the removal mechanisms, lab-scale column experiments were performed preloading the material with Cd, Cu, Ni, Pb, and Zn. To identify removal mechanisms and the distribution of heavy metals in the material, investigations with scanning electron microscope (SEM)/energy-dispersive X-ray spectroscopy (EDX) and laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS) were performed. With SEM/EDX, only Pb was detectable; all other heavy metals were not represented on the surface of the particles. To determine the intrusion of the metals, LA-ICP-MS was used. Thereby, the high porosity necessitated a special data evaluation that enabled the determination of the heavy metal removal and the leaching of other elements from the filter material as a function of depth. The measured depth profiles varied for each element and correlated with the metal mobility.</description><identifier>ISSN: 0049-6979</identifier><identifier>EISSN: 1573-2932</identifier><identifier>DOI: 10.1007/s11270-017-3515-1</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Ablation ; Analytical methods ; Atmospheric Protection/Air Quality Control/Air Pollution ; Cadmium ; Climate Change/Climate Change Impacts ; Contamination ; Copper ; Earth and Environmental Science ; Environment ; Environmental monitoring ; Evaluation ; Ferric hydroxide ; Groundwater ; Heavy metals ; Hydrogeology ; Hydroxides ; Inductively coupled plasma mass spectrometry ; Intrusion ; Laser ablation ; Lasers ; Leaching ; Lead ; Mass spectrometry ; Mass spectroscopy ; Metals ; Nickel ; Particle physics ; Porosity ; Porous materials ; Profiles ; Removal ; Roads ; Runoff ; Scanning electron microscopy ; Soil Science & Conservation ; Spectroscopy ; Surface runoff ; Surface water ; Surface-groundwater relations ; Water purification ; Water Quality/Water Pollution ; Water resources ; X-ray spectroscopy ; X-rays ; Zinc</subject><ispartof>Water, air, and soil pollution, 2017-09, Vol.228 (9), p.1, Article 331</ispartof><rights>Springer International Publishing AG 2017</rights><rights>COPYRIGHT 2017 Springer</rights><rights>Water, Air, & Soil Pollution is a copyright of Springer, 2017.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c355t-2ad1dc63af3ad6d3ad23514af5f35de0b9eaa9bb3274c8320c843933b39084563</citedby><cites>FETCH-LOGICAL-c355t-2ad1dc63af3ad6d3ad23514af5f35de0b9eaa9bb3274c8320c843933b39084563</cites><orcidid>0000-0002-2002-2026</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11270-017-3515-1$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11270-017-3515-1$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Hilbig, H.</creatorcontrib><creatorcontrib>Huber, M.</creatorcontrib><creatorcontrib>Gmell, A.</creatorcontrib><creatorcontrib>Heinz, D.</creatorcontrib><title>Determination of Heavy Metals in a Highly Porous Sorptive Filter Material of Road Runoff Treatment Systems with LA-ICP-MS</title><title>Water, air, and soil pollution</title><addtitle>Water Air Soil Pollut</addtitle><description>To remove heavy metal contaminations from road runoff prior to discharge into surface water or groundwater, highly porous sorptive filter materials are used. One effective material is a technical product based on granular ferric hydroxide. To specify the removal mechanisms, lab-scale column experiments were performed preloading the material with Cd, Cu, Ni, Pb, and Zn. To identify removal mechanisms and the distribution of heavy metals in the material, investigations with scanning electron microscope (SEM)/energy-dispersive X-ray spectroscopy (EDX) and laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS) were performed. With SEM/EDX, only Pb was detectable; all other heavy metals were not represented on the surface of the particles. To determine the intrusion of the metals, LA-ICP-MS was used. Thereby, the high porosity necessitated a special data evaluation that enabled the determination of the heavy metal removal and the leaching of other elements from the filter material as a function of depth. The measured depth profiles varied for each element and correlated with the metal mobility.</description><subject>Ablation</subject><subject>Analytical methods</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Cadmium</subject><subject>Climate Change/Climate Change Impacts</subject><subject>Contamination</subject><subject>Copper</subject><subject>Earth and Environmental Science</subject><subject>Environment</subject><subject>Environmental monitoring</subject><subject>Evaluation</subject><subject>Ferric hydroxide</subject><subject>Groundwater</subject><subject>Heavy metals</subject><subject>Hydrogeology</subject><subject>Hydroxides</subject><subject>Inductively coupled plasma mass spectrometry</subject><subject>Intrusion</subject><subject>Laser ablation</subject><subject>Lasers</subject><subject>Leaching</subject><subject>Lead</subject><subject>Mass spectrometry</subject><subject>Mass spectroscopy</subject><subject>Metals</subject><subject>Nickel</subject><subject>Particle physics</subject><subject>Porosity</subject><subject>Porous materials</subject><subject>Profiles</subject><subject>Removal</subject><subject>Roads</subject><subject>Runoff</subject><subject>Scanning electron microscopy</subject><subject>Soil Science & Conservation</subject><subject>Spectroscopy</subject><subject>Surface runoff</subject><subject>Surface water</subject><subject>Surface-groundwater relations</subject><subject>Water purification</subject><subject>Water Quality/Water Pollution</subject><subject>Water resources</subject><subject>X-ray 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One effective material is a technical product based on granular ferric hydroxide. To specify the removal mechanisms, lab-scale column experiments were performed preloading the material with Cd, Cu, Ni, Pb, and Zn. To identify removal mechanisms and the distribution of heavy metals in the material, investigations with scanning electron microscope (SEM)/energy-dispersive X-ray spectroscopy (EDX) and laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS) were performed. With SEM/EDX, only Pb was detectable; all other heavy metals were not represented on the surface of the particles. To determine the intrusion of the metals, LA-ICP-MS was used. Thereby, the high porosity necessitated a special data evaluation that enabled the determination of the heavy metal removal and the leaching of other elements from the filter material as a function of depth. 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| subjects | Ablation Analytical methods Atmospheric Protection/Air Quality Control/Air Pollution Cadmium Climate Change/Climate Change Impacts Contamination Copper Earth and Environmental Science Environment Environmental monitoring Evaluation Ferric hydroxide Groundwater Heavy metals Hydrogeology Hydroxides Inductively coupled plasma mass spectrometry Intrusion Laser ablation Lasers Leaching Lead Mass spectrometry Mass spectroscopy Metals Nickel Particle physics Porosity Porous materials Profiles Removal Roads Runoff Scanning electron microscopy Soil Science & Conservation Spectroscopy Surface runoff Surface water Surface-groundwater relations Water purification Water Quality/Water Pollution Water resources X-ray spectroscopy X-rays Zinc |
| title | Determination of Heavy Metals in a Highly Porous Sorptive Filter Material of Road Runoff Treatment Systems with LA-ICP-MS |
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