Polarized Neutron Diffraction as a Tool for Mapping Molecular Magnetic Anisotropy: Local Susceptibility Tensors in CoII Complexes

Polarized neutron diffraction (PND) experiments were carried out at low temperature to characterize with high precision the local magnetic anisotropy in two paramagnetic high‐spin cobalt(II) complexes, namely [CoII(dmf)6](BPh4)2 (1) and [CoII2(sym‐hmp)2](BPh4)2 (2), in which dmf=N,N‐dimethylformamid...

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