Quantum‐chemical perspective of nanoscale Raman spectroscopy with the three‐dimensional phonon confinement model

Raman spectroscopy of crystalline/molecular systems is well grounded with quantum‐chemical calculations and group theory, making it a unique tool for material characterization. For the ‘intermediate’ case of nanometer‐scale systems, however, the application of Raman spectroscopy is limited by the la...

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